| 1. |
- Abele, H., et al.
(author)
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Particle physics at the European Spallation Source
- 2023
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In: Physics reports. - : Elsevier. - 0370-1573 .- 1873-6270. ; 1023, s. 1-84
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Research review (peer-reviewed)abstract
- Presently under construction in Lund, Sweden, the European Spallation Source (ESS) will be the world’s brightest neutron source. As such, it has the potential for a particle physics program with a unique reach and which is complementary to that available at other facilities. This paper describes proposed particle physics activities for the ESS. These encompass the exploitation of both the neutrons and neutrinos produced at the ESS for high precision (sensitivity) measurements (searches).
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| 2. |
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| 3. |
- Ahlborg, Helene, 1980, et al.
(author)
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Provision of electricity to African households : The importance of democracy and institutional quality
- 2015
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In: Energy Policy. - : Elsevier BV. - 0301-4215 .- 1873-6777. ; 87, s. 125-135
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Journal article (peer-reviewed)abstract
- How can differences in per capita household electricity consumption across African countries be understood? Based on theories that highlight the importance of democracy and institutional quality for provision of public goods, the aim of the paper is to analyse the degree to which the level of per capita household electricity consumption in African countries can be attributed to the countries’ democratic status and their institutional quality. We rely on regression analysis employing a pooled data set for 44 African countries over the time period 1996–2009. The analysis shows that democracy and institutional quality both have significant positive effects on per capita household consumption of electricity. Our results have implications for how energy sector reforms are promoted in developing countries. At a more general level they illustrate that institution-building policy efforts are relevant also in areas where contemporary debates have tended to primarily centre on economic development, financial prerequisites and ownership issues.
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| 4. |
- Ahlström, Johan, 1990, et al.
(author)
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Economic potential for substitution of fossil fuels with liquefied biomethane in Swedish iron and steel industry – Synergy and competition with other sectors
- 2020
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In: Energy Conversion and Management. - : Elsevier Ltd. - 0196-8904 .- 1879-2227. ; 209
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Journal article (peer-reviewed)abstract
- In Sweden, the iron and steel industry (ISI) is a major source of greenhouse gas (GHG) emissions. Most of the emissions result from the use of fossil reducing agents. Nevertheless, the use of fossil fuels for other purposes must also be eliminated in order to reach the Swedish emissions reduction targets. In this study, we investigate the possibility to replace fossil gaseous and liquid fuels used for heating in the ISI, with liquefied biomethane (LBG) produced through gasification of forest residues. We hypothesize that such utilization of fuels in the Swedish ISI is insufficient to independently drive the development of large-scale LBG production, and that other sectors demanding LBG, e.g., for transportation, can be expected to influence the economic potential for the ISI to switch to LBG. The paper investigates how demand for LBG from other sectors can contribute to, or prevent, a phase-out of fossil fuels used for heating purposes in the ISI under different future energy market scenarios, with additional analysis of the impact of a CO2 emissions charge. A geographically explicit cost-minimizing biofuel production localization model is combined with heat integration and energy market scenario analysis. The results show that from a set of possible future energy market scenarios, none yielded more than a 9% replacement of fossil fuels used for heating purposes in the ISI, and only when there was also a demand for LBG from other sectors. The scenarios corresponding to a more ambitious GHG mitigation policy did not achieve higher adoption of LBG, due to corresponding higher biomass prices. A CO2 charge exceeding 200 EUR/tonCO2 would be required to achieve a full phase-out of fossil fuels used for heating purposes in the ISI. We conclude that with the current policy situation, substitution of fossil fuels by LBG will not be economically feasible for the Swedish ISI.
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| 5. |
- Ahlström, Johan, et al.
(author)
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Value chains for integrated production of liquefied bio-SNG at sawmill sites – Techno-economic and carbon footprint evaluation
- 2017
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In: Applied Energy. - : Elsevier BV. - 0306-2619 .- 1872-9118. ; 206, s. 1590-1608
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Journal article (peer-reviewed)abstract
- Industry's increasing demand for liquefied natural gas could be met in the future by liquefied methane produced from biomass feedstock (LBG - liquefied biogas). This study presents results from an investigation of value chains for integrated production of LBG at a generic sawmill site, based on gasification of sawmill waste streams and forest residues. The objective was to investigate the cost for, as well as the carbon footprint reduction associated with, production and use of LBG as a fuel. Five different LBG plant sizes were investigated in combination with three different sawmill sizes. The resulting cases differ regarding biomass feedstock composition, biomass transportation distances, LBG plant sizes, how efficiently the excess heat from the LBG plant is used, and LBG distribution distances. Pinch technology was used to quantify the heat integration opportunities and to design the process steam network. The results show that efficient use of energy within the integrated process has the largest impact on the performance of the value chain in terms of carbon footprint. The fuel production cost are mainly determined by the investment cost of the plant, as well as feedstock transportation costs, which mainly affects larger plants. Production costs are shown to range from 68 to 156 EUR/MW hfuel and the carbon footprint ranges from 175 to 250 kg GHG-eq/MW hnet biomass assuming that the product is used to substitute fossil LNG fuel. The results indicate that process integration of an indirect biomass gasifier for LBG production is an effective way for a sawmill to utilize its by-products. Integration of this type of biorefinery can be done in such a way that the plant can still cover its heating needs whilst expanding its product portfolio in a competitive way, both from a carbon footprint and cost perspective. The results also indicate that the gains associated with efficient heat integration are important to achieve an efficient value chain.
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| 6. |
- Ahmed, Mukhtiar, et al.
(author)
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Aromatic Heterocyclic Anion Based Ionic Liquids and Electrolytes
- 2023
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In: Physical Chemistry, Chemical Physics - PCCP. - : Royal Society of Chemistry. - 1463-9076 .- 1463-9084. ; 25:4, s. 3502-3512
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Journal article (peer-reviewed)abstract
- Five new ionic materials comprising fluorine-free aromatic heterocyclic anions based on pyridine and pyrazine combined with a common n-tetrabutylphosphonium cation, (P4444)+, result in two room temperature ionic liquids (RTILs), one semi-solid, and two organic ionic plastic crystals (OIPCs) with melting points >20 °C. The OIPCs showed a plastic crystalline phase, multiple solid–solid transitions, and plastic crystalline and melt phases. For both the neat RTILs and the Li+ conducting electrolytes, the nature and strength of the ion–ion interactions mainly depend on the position of the nitrogen atom with respect to the carboxylate group in the anions. Furthermore, for the RTILs the ionic conductivity is effected by the electronic structure and flexibility of the ions and the anions diffuse faster than the (P4444)+ cation, but are slowed down in the electrolytes due to the strong electrostatic interactions between the carboxylate group of the anions and the Li+, as shown both experimentally and computationally. Overall, this study describes the effect of structural tuning of aromatic anions on the ion–ion interactions and introduces new ionic materials with promising properties to be used as solid and liquid electrolytes in energy storage devices.
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| 7. |
- Ahmed, Mukhtiar, et al.
(author)
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Ionic Liquids and Electrolytes with Flexible Aromatic Anions
- 2023
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In: Chemistry - A European Journal. - : John Wiley & Sons. - 0947-6539 .- 1521-3765. ; 29:41
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Journal article (peer-reviewed)abstract
- Five new n-tetrabutylphosphonium (P4444)+ cation based ionic liquids (ILs) with oligoether substituted aromatic carboxylate anions have been synthesized. The nature and position of the oligoether chain affect thermal stability (up to 330 ºC), phase behaviour (Tg < -55 ºC) and ion transport. Furthermore, with the aim of application in lithium batteries, electrolytes were created for two of the ILs by 10 mol% doping using the corresponding Li-salts. This affects the ion diffusion negatively, from being higher and equal for cations and anions to lower for all ions and unequal. This is due to the stronger ionic interactions and formation of aggregates, primarily between the Li+ ions and the carboxylate group of the anions. Electrochemically, the electrolytes have electrochemical stability windows up to 3.5 V, giving some promise for battery application.
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| 8. |
- Ahmed, Mukhtiar, et al.
(author)
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Pyrrolidium- and Imidazolium-Based Ionic Liquids and Electrolytes with Flexible Oligoether Anions
- 2024
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In: ChemPhysChem. - : John Wiley & Sons. - 1439-7641 .- 1439-4235. ; In Press
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Journal article (peer-reviewed)abstract
- A new class of fluorine-free ionic liquids (ILs) and electrolytes based on aliphatic flexible oligoether anions, 2-(2-methoxyethoxy)acetate (MEA) and 2-[2-(2-methoxyethoxy)ethoxy]acetate (MEEA), coupled with pyrrolidinium and imidazolium cations is introduced. For the ILs with MEEA anions, Li+ conducting electrolytes are created by doping the ILs with 30 mol % of LiMEEA. The structural flexibility of the oligoether functionality in the anion results in glass transition temperatures (Tg) as low as −60 °C for the neat ILs and the electrolytes. The imidazolium-based ILs and electrolytes reveal better thermal stabilities but higher Tg and lower electrochemical stabilities than the corresponding pyrrolidinium-based analogues. All neat ILs show comparable transport properties for the cations and these decrease by the addition of lithium salt – the pyrrolidinium-based electrolyte being affected the most.
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| 9. |
- Aires, F., et al.
(author)
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Microwave hyperspectral measurements for temperature and humidity atmospheric profiling from satellite: The clear-sky case
- 2015
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In: Journal of Geophysical Research. - 0148-0227 .- 2156-2202 .- 2169-897X .- 2169-8996. ; 120:21, s. 11334-11351
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Journal article (peer-reviewed)abstract
- This study investigates the benefits of a satellite HYperspectral Microwave Sensor (HYMS) for the retrieval of atmospheric temperature and humidity profiles, in the context of numerical weather prediction (NWP). In the infrared, hyperspectral instruments have already improved the accuracy of NWP forecasts. Microwave instruments so far only provide observations for a limited number of carefully selected channels. An information content analysis is conducted here to assess the impact of hyperspectral microwave measurements on the retrieval of temperature and water vapor profiles under clear-sky conditions. It uses radiative transfer simulations over a large variety of atmospheric situations. It accounts for realistic observation (instrument and radiative transfer) noise and for a priori information assumptions compatible with NWP practices. The estimated retrieval performance of the HYMS instrument is compared to those of the microwave instruments to be deployed on board the future generation of European operational meteorological satellites (MetOp-SG). The results confirm the positive impact of a HYMS instrument on the atmospheric profiling capabilities compared to MetOp-SG. Temperature retrieval uncertainty, compared to a priori information, is reduced by 2 to 10%, depending on the atmospheric height, and improvement rates are much higher than what will be obtained with MetOp-SG. For humidity sounding these improvements can reach 30%, a significant benefit as compared to MetOp-SG results especially below 250 hPa. The results are not very sensitive to the instrument noise, under our assumptions. The main impact provided by the hyperspectral information originates from the higher resolution in the O2 band around 60 GHz. The results are presented over ocean at nadir, but similar conclusions are obtained for other incidence angles and over land. Key Points A hyperspectral MW instrument could improve temperature & humidity retrieval compared to MetOp-SG The main impact from HYMS comes from higher resolution in the O2 band around 60 GHz Hyperspectral information is not really sensitive to instrument noise.
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| 10. |
- Aires, Filipe, et al.
(author)
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Towards more realistic hypotheses for the information content analysis of cloudy/precipitating situations - Application to a hyperspectral instrument in the microwave
- 2019
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In: Quarterly Journal of the Royal Meteorological Society. - : Wiley. - 0035-9009 .- 1477-870X. ; 145:718, s. 1-14
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Journal article (peer-reviewed)abstract
- Information Content (IC) analysis can be used before an instrument is built to estimate its retrieval uncertainties and analyse their sensitivity to several factors. It is a very useful method to define/optimize satellite instruments. IC has shown its potential to compare instrument concepts in the infrared or the microwave. IC is based on some hypotheses such as the the Gaussian character of the radiative transfer (RT) and instrument errors, the first-guess errors (Gaussian character, std and correlation structure), or the linearization of the RT around a first guess. These hypotheses are easier to define for simple atmospheric situations. However, even in the clear-sky case, their complexity has never ceased to increase towards more realism, to optimize the assimilation of satellite measurements in numerical weather prediction (NWP) systems. In the cloudy/precipitating case, these hypotheses are even more difficult to define in a realistic way as many factors are still very difficult to quantify. In this study, several tools are introduced to specify more realistic IC hypotheses than the current practice. We focus on microwave observations as they are more pertinent for clouds and precipitation. Although not perfect, the proposed solutions are a new step towards more realistic IC assumptions of cloudy/precipitating scenes. A state-dependence of the RT errors is introduced, the first-guess errors have a more complex vertical structure, the IC is performed simultaneously on all the hydrometeors to take into account the contamination effect of the RT input uncertainties, and the IC is performed on a diversified set of cloudy/precipitating scenes with well-defined hydrometeor assumptions. The method presented in this study is illustrated using the HYperspectral Microwave Sensor (HYMS) instrument concept with channels between 6.9 and 874 GHz (millimetre and sub-millimetre regions). HYMS is considered as a potential next generation microwave sounder.
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