| 1. |
- Erny, Christian, et al.
(författare)
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Metrology of high-order harmonics for free-electron laser seeding
- 2011
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 13
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Tidskriftsartikel (refereegranskat)abstract
- We examine the characteristics of high-order harmonics generated with 800 nm, 25 mJ, 160 fs laser pulses in an Ar gas cell with the objective of seeding a free electron laser. We measure the energy per pulse and per harmonic, the energy jitter, the divergence and the position stability of the harmonic beam. We perform ab initio numerical simulations based on integration of the time-dependent Schrodinger equation and of the wave equation within the slowly varying envelope approximation. The results reproduce the experimental measurements to better than a factor of two. The interaction of a frequency comb of harmonic fields with an electron bunch in an undulator is examined with a simple model consisting of calculating the energy modulation owing to the seed-electron interaction. The model indicates that the undulator acts as a spectral filter selecting a given harmonic.
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| 2. |
- Gabrysch, Markus, et al.
(författare)
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XUV-induced transient phase gratings for probing ultra-fast carrier generation and recombination processes in wide-bandgap semiconductors
- 2013
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Ingår i: Annalen der Physik. - : Wiley. - 0003-3804 .- 1521-3889. ; 525:1-2, s. 59-65
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Tidskriftsartikel (refereegranskat)abstract
- A method for probing the temporal evolution of ultra-fast carrier generation and recombination processes in wide-bandgap semiconductors, e.g. diamond, is described. Two extreme ultraviolet (pump) pulses produced by high-order harmonic generation in Argon gas (with a photon energy of 32 eV) are superimposed on a sample with a small angle between them, inducing periodic changes in the refractive index of the material causing it to act as a transient diffraction grating. A delayed synchronized infrared (probe) pulse gets diffracted on the induced phase grating and is detected in the first diffraction order. By varying the time-delay between pump and probe, the full temporal evolution of the free carrier generation and recombination processes can be resolved. Feasibility calculations and the first steps towards experimental implementation are presented.
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| 3. |
- He, Xinkui, et al.
(författare)
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Spatial and spectral properties of the high-order harmonic emission in argon for seeding applications
- 2009
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Ingår i: Physical Review A (Atomic, Molecular and Optical Physics). - 1050-2947. ; 79:6
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Tidskriftsartikel (refereegranskat)abstract
- We characterize and control the harmonic emission in the spectral and spatial domains in order to define in which conditions the harmonic radiation can be a high-quality seed for soft x-ray and x-ray free-electron lasers. The length of the gas cell, where harmonics are generated, was optimized and the energy per pulse was determined in absolute value with a calibrated x-ray photodiode. The beam spatial profile was measured and, in some conditions, a very collimated beam with a half-angle divergence below 1 mrad could be obtained. We also show that increasing the intensity of the fundamental laser field leads to a considerable broadening of the bandwidth of the harmonic radiation, allowing us to cover a large spectral range. This effect is due to fundamental reshaping leading to an efficient phase matching of both short- and long-trajectory contributions.
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| 4. |
- Mikkelsen, Anders, et al.
(författare)
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Photoemission electron microscopy using extreme ultraviolet attosecond pulse trains
- 2009
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Ingår i: Review of Scientific Instruments. - : AIP Publishing. - 1089-7623 .- 0034-6748. ; 80:12
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Tidskriftsartikel (refereegranskat)abstract
- We report the first experiments carried out on a new imaging setup, which combines the high spatial resolution of a photoemission electron microscope (PEEM) with the temporal resolution of extreme ultraviolet (XUV) attosecond pulse trains. The very short pulses were provided by high-harmonic generation and used to illuminate lithographic structures and Au nanoparticles, which, in turn, were imaged with a PEEM resolving features below 300 nm. We argue that the spatial resolution is limited by the lack of electron energy filtering in this particular demonstration experiment. Problems with extensive space charge effects, which can occur due to the low probe pulse repetition rate and extremely short duration, are solved by reducing peak intensity while maintaining a sufficient average intensity to allow imaging. Finally, a powerful femtosecond infrared (IR) beam was combined with the XUV beam in a pump-probe setup where delays could be varied from subfemtoseconds to picoseconds. The IR pump beam could induce multiphoton electron emission in resonant features on the surface. The interaction between the electrons emitted by the pump and probe pulses could be observed. (C) 2009 American Institute of Physics. [doi:10.1063/1.3263759]
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| 5. |
- Rudawski, Piotr, et al.
(författare)
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A high-flux high-order harmonic source.
- 2013
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Ingår i: Review of Scientific Instruments. - : AIP Publishing. - 1089-7623 .- 0034-6748. ; 84:7
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Tidskriftsartikel (refereegranskat)abstract
- We develop and implement an experimental strategy for the generation of high-energy high-order harmonics (HHG) in gases for studies of nonlinear processes in the soft x-ray region. We generate high-order harmonics by focusing a high energy Ti:Sapphire laser into a gas cell filled with argon or neon. The energy per pulse is optimized by an automated control of the multiple parameters that influence the generation process. This optimization procedure allows us to obtain energies per pulse and harmonic order as high as 200 nJ in argon and 20 nJ in neon, with good spatial properties, using a loose focusing geometry (f#≈400) and a 20 mm long medium. We also theoretically examine the macroscopic conditions for absorption-limited conversion efficiency and optimization of the HHG pulse energy for high-energy laser systems.
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| 6. |
- Schwenke, Jörg, et al.
(författare)
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Digital in-line holography on amplitude and phase objects prepared with electron beam lithography.
- 2012
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Ingår i: Journal of Microscopy. - : Wiley. - 0022-2720. ; 247:2, s. 196-201
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Tidskriftsartikel (refereegranskat)abstract
- We report on the fabrication and characterization of amplitude and phase samples consisting of well defined Au or Al features formed on ultrathin silicon nitride membranes. The samples were manufactured using electron beam lithography, metallization and a lift-off technique, which allow precise lateral control and thickness of the metal features. The fabricated specimens were evaluated by conventional microscopy, atomic force microscopy and with the digital in-line holography set-up at the Lund Laser Centre. The latter uses high-order harmonic generation as a light source, and is capable of recovering both the shape and phase shifting properties of the samples. We report on the details of the sample production and on the imaging tests with the holography set-up.
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| 7. |
- Schwenke, Jörg, et al.
(författare)
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Digital in-line holography with a single high-order harmonic pulse
- 2009
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Ingår i: Holography : Advances and Modern Trends - Advances and Modern Trends. - : SPIE. - 9780819476326 ; 7358
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Konferensbidrag (refereegranskat)abstract
- In this paper, we review the optimization and characterization of a high-order harmonic generation (HHG) source for application in coherence imaging, and the use of this light source in a digital in-line holography setup. The high-order harmonic beam is generated by focusing a powerful infrared beam into an Ar gas cell. The length of the cell and the focusing parameters are optimized to maximize the HHG output. By spectrally filtering and focusing the generated harmonic beam and positioning a 2D detector, we obtain a table-top light source suitable for in-line holography, capable of recording a hologram with a single 40 fs XUV pulse. The reconstructed images have a spatial resolution in the micrometer range.
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| 8. |
- Schwenke, Jörg, et al.
(författare)
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Single-shot holography using high-order harmonics
- 2008
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Ingår i: Journal of Modern Optics. - : Informa UK Limited. - 0950-0340 .- 1362-3044. ; 55:16, s. 2723-2730
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Tidskriftsartikel (refereegranskat)abstract
- This work demonstrates single-shot holography with ultrashort XUV pulses. The pulses are generated by high-harmonic generation in an Ar gas cell and focused to produce a strongly divergent reference beam suitable for in-line holography of micrometer size objects. The achieved intensity of the high-order harmonics in the XUV regime is sufficient for single-shot holography with good signal-to-noise ratio. A numerical algorithm is applied to reconstruct real images from the recorded holograms, which also includes an iterative process to reduce the twin-image blurring. Holograms and reconstructed images of microscope tips are presented and a description of the algorithm is given.
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| 9. |
- Schwenke, Jörg
(författare)
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Towards ultrafast imaging with extreme ultraviolet light sources
- 2012
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- This thesis reports experimental studies performed with two advanced coherent XUV sources with ultrashort pulse duration, high-order harmonic generation and seeded-free electron laser. High-order harmonic generation (HHG) is the generation of overtones of a fundamental laser pulse in a medium, e.g. noble gases. The emitted radiation has a high degree of transverse coherence, and pulse lengths in the attosecond regime can be achieved. We have applied the pulses to digital in-line holography, where we demonstrated imaging of micrometer-sized objects with single XUV pulses, and the reconstruction of the phase shifting properties of thin layers of material. A method to produce thin layers of arbitrary shape and thickness, on top of ultra-thin membranes, is presented. In another experiment, we used HHG pulses to eject electrons from a sample, to be imaged with a PEEM microscope. The experiment aims at combining the short temporal duration achievable with high-order harmonic generation, to the high spatial resolution of PEEM, in order to image electron density variations on prepared surfaces. A further experiment is proposed to use the XUV pulses from the HHG source to study the charge-carrier recombination processes in a wide-bandgap semiconductor. The short duration and high intensity of the XUV pulse allows us to create a transient phase grating and to probe the induced refractive index change at a variable time delay. Finally, we have also studied the feasibility to use HHG pulses as a seed laser for a seeded free-electron laser, by investigating the energy and pointing stability of the source. These studies are a preparation to implement an HHG setup at an existing seeded free-electron laser setup. The characterization of the emission of the seeded FEL is also presented. Here the coherence was tested in a double-slit experiment, and the polarization was determined with a linear polarizer.
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| 10. |
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