| 1. |
- Achtert, P., et al.
(författare)
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Measurement of wind profiles by motion-stabilised ship-borne Doppler lidar
- 2015
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 8:11, s. 4993-5007
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Tidskriftsartikel (refereegranskat)abstract
- Three months of Doppler lidar wind measurements were obtained during the Arctic Cloud Summer Experiment on the icebreakerOden during the summer of 2014. Such ship-borne Doppler measurements require active stabilisation to remove the effects of ship motion. We demonstrate that the combination of a commercial Doppler lidar with a custom-made motion-stabilisation platform enables the retrieval of wind profiles in the Arctic atmospheric boundary layer during both cruising and ice-breaking with statistical uncertainties comparable to land-based measurements. This held true particularly within the atmospheric boundary layer even though the overall aerosol load was very low. Motion stabilisation was successful for high wind speeds in open water and the resulting wave conditions. It allows for the retrieval of vertical winds with a random error below 0.2 m s−1. The comparison of lidar-measured wind and radio soundings gives a mean bias of 0.3 m s−1 (2°) and a mean standard deviation of 1.1 m s−1 (12°) for wind speed (wind direction). The agreement for wind direction degrades with height. The combination of a motion-stabilised platform with a low-maintenance autonomous Doppler lidar has the potential to enable continuous long-term high-resolution ship-based wind profile measurements over the oceans.
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| 2. |
- Ausmeel, Stina, et al.
(författare)
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Methods for identifying aged ship plumes and estimating contribution to aerosol exposure downwind of shipping lanes
- 2019
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 12:8, s. 4479-4493
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Tidskriftsartikel (refereegranskat)abstract
- Ship traffic is a major source of aerosol particles, particularly near shipping lanes and harbours. In order to estimate the contribution to exposure downwind of a shipping lane, it is important to be able to measure the ship emission contribution at various distances from the source. We report on measurements of atmospheric particles 7-20 km downwind of a shipping lane in the Baltic Sea Sulfur Emission Control Area (SECA) at a coastal location in southern Sweden during a winter and a summer campaign. Each ship plume was linked to individual ship passages using a novel method based on wind field data and automatic ship identification system data (AIS), where varying wind speeds and directions were applied to calculate a plume trajectory. In a situation where AIS data are not matching measured plumes well or if AIS data are missing, we provide an alternative method with particle number concentration data. The shipping lane contribution to the particle number concentration in Falsterbo was estimated by subtracting background concentrations from the ship plume concentrations, and more than 150 plumes were analysed. We have also extrapolated the contribution to seasonal averages and provide recommendations for future similar measurements. Averaged over a season, the contribution to particle number concentration was about 18 % during the winter and 10 % during the summer, including those periods with wind directions when the shipping lane was not affecting the station. The corresponding contribution to equivalent black carbon was 1.4 %..
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| 3. |
- Backman, John, et al.
(författare)
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On Aethalometer measurement uncertainties and an instrument correction factor for the Arctic
- 2017
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 10:12, s. 5039-5062
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Tidskriftsartikel (refereegranskat)abstract
- Several types of filter-based instruments are used to estimate aerosol light absorption coefficients. Two significant results are presented based on Aethalometer measurements at six Arctic stations from 2012 to 2014. First, an alternative method of post-processing the Aethalometer data is presented, which reduces measurement noise and lowers the detection limit of the instrument more effectively than box-car averaging. The biggest benefit of this approach can be achieved if instrument drift is minimised. Moreover, by using an attenuation threshold criterion for data post-processing, the relative uncertainty from the electronic noise of the instrument is kept constant. This approach results in a time series with a variable collection time (Delta t) but with a constant relative uncertainty with regard to electronic noise in the instrument. An additional advantage of this method is that the detection limit of the instrument will be lowered at small aerosol concentrations at the expense of temporal resolution, whereas there is little to no loss in temporal resolution at high aerosol concentrations (>2.1-6.7Mm(-1) as measured by the Aethalometers). At high aerosol concentrations, minimising the detection limit of the instrument is less critical. Additionally, utilising co-located filter-based absorption photometers, a correction factor is presented for the Arctic that can be used in Aethalometer corrections available in literature. The correction factor of 3.45 was calculated for low-elevation Arctic stations. This correction factor harmonises Aethalometer attenuation coefficients with light absorption coefficients as measured by the co-located light absorption photometers. Using one correction factor for Arctic Aethalometers has the advantage that measurements between stations become more inter-comparable.
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| 4. |
- Bannan, T. J., et al.
(författare)
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A method for extracting calibrated volatility information from the FIGAERO-HR-ToF-CIMS and its experimental application
- 2019
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 12:3, s. 1429-1439
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Tidskriftsartikel (refereegranskat)abstract
- The Filter Inlet for Gases and AEROsols (FIGAERO) is an inlet specifically designed to be coupled with the Aerodyne High-Resolution Time-of-Flight Chemical Ionization Mass Spectrometer (HR-ToF-CIMS). The FIGAERO-HR-ToF-CIMS provides simultaneous molecular information relating to both the gas- and particle-phase samples and has been used to extract vapour pressures (VPs) of the compounds desorbing from the filter whilst giving quantitative concentrations in the particle phase. However, such extraction of vapour pressures of the measured particle-phase components requires use of appropriate, well-defined, reference compounds. Vapour pressures for the homologous series of polyethylene glycols (PEG) ((H-(O-CH 2 CH 2 ) n -OH) for n = 3 to n = 8), covering a range of vapour pressures (VP) (10 -1 to 10 -7 Pa) that are atmospherically relevant, have been shown to be reproduced well by a range of different techniques, including Knudsen Effusion Mass Spectrometry (KEMS). This is the first homologous series of compounds for which a number of vapour pressure measurement techniques have been found to be in agreement, indicating the utility as a calibration standard, providing an ideal set of benchmark compounds for accurate characterization of the FIGAERO for extracting vapour pressure of measured compounds in chambers and the real atmosphere. To demonstrate this, single-component and mixture vapour pressure measurements are made using two FIGAERO-HR-ToF-CIMS instruments based on a new calibration determined from the PEG series. VP values extracted from both instruments agree well with those measured by KEMS and reported values from literature, validating this approach for extracting VP data from the FIGAERO. This method is then applied to chamber measurements, and the vapour pressures of known products are estimated. © 2019 Author(s).
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| 5. |
- Baron, P., et al.
(författare)
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Simulation study for the Stratospheric Inferred Winds (SIW) sub-millimeter limb sounder
- 2018
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 11:7, s. 4545-4566
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Tidskriftsartikel (refereegranskat)abstract
- Stratospheric Inferred Winds (SIW) is a Swedish mini sub-millimeter limb sounder selected for the 2nd InnoSat platform, with launch planned for around 2022. It is intended to fill the altitude gap between 30 and 70 km in atmospheric wind measurements and also aims at pursuing the limb observations of temperature and key atmospheric constituents between 10 and 90 km when current satellite missions will probably come to an end. Line-of-sight winds are retrieved from the Doppler shift of molecular emission lines introduced by the wind field. Observations will be performed with two antennas pointing toward the limb in perpendicular directions in order to reconstruct the 2-D horizontal wind vector. Each antenna has a vertical field of view (FOV) of 5 km. The chosen spectral band, near 655 GHz, contains a dense group of strong O3 lines suitable for exploiting the small amount of wind information in stratospheric spectra. Using both sidebands of the heterodyne receiver, a large number of chemical species will be measured, including O3 isotopologues, H2O, HDO, HCl, ClO, N2O, HNO3, NO, NO2, HCN, CH3CN and HO2. This paper presents a simulation study that assesses measurement performance. The line-of-sight winds are retrieved between 30 and 90 km with the best sensitivity between 35 and 70 km, where the precision (1 σ ) is 5-10 mĝ€†sĝ'1 for a single scan. Similar performance can be obtained during day and night conditions except in the lower mesosphere, where the photo-dissociation of O3 in daytime reduces the sensitivity by 50 % near 70 km. Profiles of O3, H2O and temperature are retrieved with high precision up to 50 km ( < 1 %, < 2 %, 1 K, respectively). Systematic errors due to uncertainties in spectroscopic parameters, in the radiometer sideband ratio and in the radiance calibration process are investigated. A large wind retrieval bias of 10-30 mĝ€†sĝ'1 between 30 and 40 km could be induced by the air-broadening parameter uncertainties of O3 lines. This highlights the need for good knowledge of these parameters and for studying methods to mitigate the retrieval bias..
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| 6. |
- Bender, Stefan, et al.
(författare)
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Comparison of nitric oxide measurements in the mesosphere and lower thermosphere from ACE-FTS, MIPAS, SCIAMACHY, and SMR
- 2015
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 8:10, s. 4171-4195
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Tidskriftsartikel (refereegranskat)abstract
- We compare the nitric oxide measurements in the mesosphere and lower thermosphere (60 to 150 km) from four instruments: the Atmospheric Chemistry Experiment–Fourier Transform Spectrometer (ACE-FTS), the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), the SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY), and the Sub-Millimetre Radiometer (SMR). We use the daily zonal mean data in that altitude range for the years 2004–2010 (ACE-FTS), 2005–2012 (MIPAS), 2008–2012 (SCIAMACHY), and 2003–2012 (SMR).We first compare the data qualitatively with respect to the morphology, focussing on the major features, and then compare the time series directly and quantitatively. In three geographical regions, we compare the vertical density profiles on coincident measurement days. Since none of the instruments delivers continuous daily measurements in this altitude region, we carried out a multi-linear regression analysis. This regression analysis considers annual and semi-annual variability in the form of harmonic terms and inter-annual variability by responding linearly to the solar Lyman-α radiation index and the geomagnetic Kp index. This analysis helps to find similarities and differences in the individual data sets with respect to the inter-annual variations caused by geomagnetic and solar variability.
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| 7. |
- Brath, M., et al.
(författare)
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Retrieval of an ice water path over the ocean from ISMAR and MARSS millimeter and submillimeter brightness temperatures
- 2018
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 11:1, s. 611-632
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Tidskriftsartikel (refereegranskat)abstract
- A neural-network-based retrieval method to determine the snow ice water path (SIWP), liquid water path (LWP), and integrated water vapor (IWV) from millimeter and submillimeter brightness temperatures, measured by using airborne radiometers (ISMAR and MARSS), is presented. The neural networks were trained by using atmospheric profiles from the ICON numerical weather prediction (NWP) model and by radiative transfer simulations using the Atmospheric Radiative Transfer Simulator (ARTS). The basic performance of the retrieval method was analyzed in terms of offset (bias) and the median fractional error (MFE), and the benefit of using submillimeter channels was studied in comparison to pure microwave retrievals. The retrieval is offset-free for SIWP > 0.01kgm -2 , LWP > 0:1kgm -2 , and IWV > 3kgm -2 . The MFE of SIWP decreases from 100% at SIWPD 0.01kgm -2 to 20% at SIWPD 1kgm -2 and the MFE of LWP from 100% at LWP D 0.05kgm -2 to 30% at LWPD 1kgm -2 . The MFE of IWV for IWV > 3kgm -2 is 5 to 8%. The SIWP retrieval strongly benefits from submillimeter channels, which reduce the MFE by a factor of 2, compared to pure microwave retrievals. The IWV and the LWP retrievals also benefit from submillimeter channels, albeit to a lesser degree. The retrieval was applied to ISMAR and MARSS brightness temperatures from FAAM flight B897 on 18 March 2015 of a precipitating frontal system west of the coast of Iceland. Considering the given uncertainties, the retrieval is in reasonable agreement with the SIWP, LWP, and IWV values simulated by the ICON NWP model for that flight. A comparison of the retrieved IWV with IWV from 12 dropsonde measurements shows an offset of 0:5kgm -2 and an RMS difference of 0:8kgm -2 , showing that the retrieval of IWV is highly effective even under cloudy conditions.
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| 8. |
- Christensen, Ole Martin, 1984, et al.
(författare)
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Tomographic retrieval of water vapour and temperature around polar mesospheric clouds using Odin-SMR
- 2015
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 8:5, s. 1981-1999
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Tidskriftsartikel (refereegranskat)abstract
- A special observation mode of the Odin satellite provides the first simultaneous measurements of water vapour, temperature and polar mesospheric cloud (PMC) brightness over a large geographical area while still resolving both horizontal and vertical structures in the clouds and background atmosphere. The observation mode was activated during June, July and August of 2010 and 2011, and for latitudes between 50 and 82 degrees N. This paper focuses on the water vapour and temperature measurements carried out with Odin's sub-millimetre radiometer (SMR). The tomographic retrieval approach used provides water vapour and temperature between 75 and 90 km with a vertical resolution of about 2.5 km and a horizontal resolution of about 200 km. The precision of the measurements is estimated to 0.2 ppmv for water vapour and 2K for temperature. Due to limited information about the pressure at the measured altitudes, the results have large uncertainties (> 3 ppmv) in the retrieved water vapour. These errors, however, influence mainly the mean atmosphere retrieved for each orbit, and variations around this mean are still reliably captured by the measurements. SMR measurements are performed using two different mixer chains, denoted as frequency mode 19 and 13. Systematic differences between the two frontends have been noted. A first comparison with the Solar Occultation For Ice Experiment instrument (SOFIE) on-board the Aeronomy of Ice in the Mesosphere (AIM) satellite and the Fourier Transform Spectrometer of the Atmospheric Chemistry Experiment (ACE-FTS) on-board SCISAT indicates that the measurements using the frequency mode 19 have a significant low bias in both temperature (> 15 K) and water vapour (> 0.5 ppmv), while the measurements using frequency mode 13 agree with the other instruments considering estimated errors. PMC brightness data is provided by OSIRIS, Odin's other sensor. Combined SMR and OSIRIS data for some example orbits is considered. For these orbits, effects of PMCs on the water vapour distribution are clearly seen. Areas depleted of water vapour are found above layers with PMC, while regions of enhanced water vapour due to ice particle sedimentation are primarily placed between and under the clouds.
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| 9. |
- DeMott, Paul J., et al.
(författare)
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The Fifth International Workshop on Ice Nucleation phase 2 (FIN-02) : Laboratory intercomparison of ice nucleation measurements
- 2018
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 11:11, s. 6231-6257
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Tidskriftsartikel (refereegranskat)abstract
- The second phase of the Fifth International Ice Nucleation Workshop (FIN-02) involved the gathering of a large number of researchers at the Karlsruhe Institute of Technology's Aerosol Interactions and Dynamics of the Atmosphere (AIDA) facility to promote characterization and understanding of ice nucleation measurements made by a variety of methods used worldwide. Compared to the previous workshop in 2007, participation was doubled, reflecting a vibrant research area. Experimental methods involved sampling of aerosol particles by direct processing ice nucleation measuring systems from the same volume of air in separate experiments using different ice nucleating particle (INP) types, and collections of aerosol particle samples onto filters or into liquid for sharing amongst measurement techniques that post-process these samples. In this manner, any errors introduced by differences in generation methods when samples are shared across laboratories were mitigated. Furthermore, as much as possible, aerosol particle size distribution was controlled so that the size limitations of different methods were minimized. The results presented here use data from the workshop to assess the comparability of immersion freezing measurement methods activating INPs in bulk suspensions, methods that activate INPs in condensation and/or immersion freezing modes as single particles on a substrate, continuous flow diffusion chambers (CFDCs) directly sampling and processing particles well above water saturation to maximize immersion and subsequent freezing of aerosol particles, and expansion cloud chamber simulations in which liquid cloud droplets were first activated on aerosol particles prior to freezing. The AIDA expansion chamber measurements are expected to be the closest representation to INP activation in atmospheric cloud parcels in these comparisons, due to exposing particles freely to adiabatic cooling. The different particle types used as INPs included the minerals illite NX and potassium feldspar (K-feldspar), two natural soil dusts representative of arable sandy loam (Argentina) and highly erodible sandy dryland (Tunisia) soils, respectively, and a bacterial INP (Snomax®). Considered together, the agreement among post-processed immersion freezing measurements of the numbers and fractions of particles active at different temperatures following bulk collection of particles into liquid was excellent, with possible temperature uncertainties inferred to be a key factor in determining INP uncertainties. Collection onto filters for rinsing versus directly into liquid in impingers made little difference. For methods that activated collected single particles on a substrate at a controlled humidity at or above water saturation, agreement with immersion freezing methods was good in most cases, but was biased low in a few others for reasons that have not been resolved, but could relate to water vapor competition effects. Amongst CFDC-style instruments, various factors requiring (variable) higher supersaturations to achieve equivalent immersion freezing activation dominate the uncertainty between these measurements, and for comparison with bulk immersion freezing methods. When operated above water saturation to include assessment of immersion freezing, CFDC measurements often measured at or above the upper bound of immersion freezing device measurements, but often underestimated INP concentration in comparison to an immersion freezing method that first activates all particles into liquid droplets prior to cooling (the PIMCA-PINC device, or Portable Immersion Mode Cooling chAmber-Portable Ice Nucleation Chamber), and typically slightly underestimated INP number concentrations in comparison to cloud parcel expansions in the AIDA chamber; this can be largely mitigated when it is possible to raise the relative humidity to sufficiently high values in the CFDCs, although this is not always possible operationally. Correspondence of measurements of INPs among direct sampling and post-processing systems varied depending on the INP type. Agreement was best for Snomax® particles in the temperature regime colder than -10°C, where their ice nucleation activity is nearly maximized and changes very little with temperature. At temperatures warmer than -10°C, Snomax® INP measurements (all via freezing of suspensions) demonstrated discrepancies consistent with previous reports of the instability of its protein aggregates that appear to make it less suitable as a calibration INP at these temperatures. For Argentinian soil dust particles, there was excellent agreement across all measurement methods; measures ranged within 1 order of magnitude for INP number concentrations, active fractions and calculated active site densities over a 25 to 30°C range and 5 to 8 orders of corresponding magnitude change in number concentrations. This was also the case for all temperatures warmer than -25°C in Tunisian dust experiments. In contrast, discrepancies in measurements of INP concentrations or active site densities that exceeded 2 orders of magnitude across a broad range of temperature measurements found at temperatures warmer than -25°C in a previous study were replicated for illite NX. Discrepancies also exceeded 2 orders of magnitude at temperatures of -20 to -25°C for potassium feldspar (K-feldspar), but these coincided with the range of temperatures at which INP concentrations increase rapidly at approximately an order of magnitude per 2°C cooling for K-feldspar. These few discrepancies did not outweigh the overall positive outcomes of the workshop activity, nor the future utility of this data set or future similar efforts for resolving remaining measurement issues. Measurements of the same materials were repeatable over the time of the workshop and demonstrated strong consistency with prior studies, as reflected by agreement of data broadly with parameterizations of different specific or general (e.g., soil dust) aerosol types. The divergent measurements of the INP activity of illite NX by direct versus post-processing methods were not repeated for other particle types, and the Snomax° data demonstrated that, at least for a biological INP type, there is no expected measurement bias between bulk collection and direct immediately processed freezing methods to as warm as -10°C. Since particle size ranges were limited for this workshop, it can be expected that for atmospheric populations of INPs, measurement discrepancies will appear due to the different capabilities of methods for sampling the full aerosol size distribution, or due to limitations on achieving sufficient water supersaturations to fully capture immersion freezing in direct processing instruments. Overall, this workshop presents an improved picture of present capabilities for measuring INPs than in past workshops, and provides direction toward addressing remaining measurement issues.
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| 10. |
- Duncan, David, 1988, et al.
(författare)
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An experimental 2D-Var retrieval using AMSR2
- 2019
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 12:12, s. 6341-6359
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Tidskriftsartikel (refereegranskat)abstract
- A two-dimensional variational retrieval (2D-Var) is presented for a passive microwave imager. The overlapping antenna patterns of all frequencies from the Advanced Microwave Scanning Radiometer 2 (AMSR2) are explicitly simulated to attempt retrieval of near-surface wind speed and surface skin temperature at finer spatial scales than individual antenna beams. This is achieved, with the effective spatial resolution of retrieved parameters judged by analysis of 2D-Var averaging kernels. Sea surface temperature retrievals achieve about 30 km resolution, with wind speed retrievals at about 10 km resolution. It is argued that multi-dimensional optimal estimation permits greater use of total information content from microwave sensors than other methods, with no compromises on target resolution needed; instead, various targets are retrieved at the highest possible spatial resolution, driven by the channels' sensitivities. All AMSR2 channels can be simulated within near their published noise characteristics for observed clear-sky scenes, though calibration and emissivity model errors are key challenges. This experimental retrieval shows the feasibility of 2D-Var for cloud-free retrievals and opens the possibility of stand-alone 3D-Var retrievals of water vapour and hydrometeor fields from microwave imagers in the future. The results have implications for future satellite missions and sensor design, as spatial oversampling can somewhat mitigate the need for larger antennas in the push for higher spatial resolution.
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