| 1. |
- Börjesson, Gunnar, et al.
(författare)
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A national landfill methane budget for Sweden based on field measurements, and an evaluation of IPCC models
- 2009
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Ingår i: Tellus, Series B: Chemical and Physical Meteorology. - : Stockholm University Press. - 1600-0889 .- 0280-6509. ; 61:2, s. 424-435
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Tidskriftsartikel (refereegranskat)abstract
- Seven Swedish landfills were investigated from 2001 to 2003. On each landfill, a measure of the total methane production was calculated from data on: (1) methane emissions (leakage); (2) methane oxidation and (3) from gas recovery. Methane emissions were determined via a tracer gas (N2O) release-based remote sensing method. N2O and CH4 were measured with an Fourier Transform infrared detector at a distance of more than 1 km downwind from the landfills. Methane oxidation in the landfill covers was measured with the stable carbon isotope method. The efficiency in gas recovery systems proved to be highly variable, but on an average, 51% of the produced landfill gas was captured. A first-order decay model, based on four fractions (waste from households and parks, sludges and industrial waste), showed that the use of a degradable organic carbon fraction (DOCf) value of 0.54, in accordance with the default value for DOCf of 0.50 in the latest IPCC model, gave an emission estimate similar to the official national reports.
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| 2. |
- Aiuppa, A., et al.
(författare)
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Gas measurements from the Costa Rica-Nicaragua volcanic segment suggest possible along-arc variations in volcanic gas chemistry
- 2014
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Ingår i: Earth and Planetary Science Letters. - : Elsevier BV. - 1385-013X .- 0012-821X. ; 407, s. 134-147
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Tidskriftsartikel (refereegranskat)abstract
- Obtaining accurate estimates of the CO2 output from arc volcanism requires a precise understanding of the potential along-arc variations in volcanic gas chemistry, and ultimately of the magmatic gas signature of each individual arc segment. In an attempt to more fully constrain the magmatic gas signature of the Central America Volcanic Arc (CAVA), we present here the results of a volcanic gas survey performed during March and April 2013 at five degassing volcanoes within the Costa Rica-Nicaragua volcanic segment (CNVS). Observations of the volcanic gas plume made with a multicomponent gas analyzer system (Multi-GAS) have allowed characterization of the CO2/SO2-ratio signature of the plumes at Pads (0.30 +/- 0.06, mean +/- SD), Rincon de la Vieja (27.0 +/- 15.3), and Turrialba (2.2 +/- 0.8) in Costa Rica, and at Telica (3.0 +/- 0.9) and San Cristobal (4.2 +/- 1.3) in Nicaragua (all ratios on molar basis). By scaling these plume compositions to simultaneously measured SO2 fluxes, we estimate that the CO2 outputs at CNVS volcanoes range from low (25.5 +/- 11.0 tons/day at Pods) to moderate (918 to 1270 tons/day at Turrialba). These results add a new information to the still fragmentary volcanic CO2 output data set, and allow estimating the total CO2 output from the CNVS at 2835 1364 tons/day. Our novel results, with previously available information about gas emissions in Central America, are suggestive of distinct volcanic gas CO2/S-T (= SO2 + H2S)-ratio signature for magmatic volatiles in Nicaragua (similar to 3) relative to Costa Rica (similar to 0.5-1.0). We also provide additional evidence for the earlier theory relating the CO2-richer signature of Nicaragua volcanism to increased contributions from slab-derived fluids, relative to more-MORB-like volcanism in Costa Rica. The sizeable along-arc variations in magmatic gas chemistry that the present study has suggested indicate that additional gas observations are urgently needed to more-precisely confine the volcanic CO2 from the CAVA, and from global arc volcanism.
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| 3. |
- Aiuppa, Sandro, et al.
(författare)
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Tracking formation of a lava lake from ground and space: Masaya volcano (Nicaragua), 2015-2017
- 2018
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Ingår i: Geochemistry, Geophysics, Geosystems. - 1525-2027. ; 19:2, s. 496-515
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Tidskriftsartikel (refereegranskat)abstract
- A vigorously degassing lava lake appeared inside the Santiago pit crater of Masaya volcano (Nicaragua) in December 2015, after years of degassing with no (or minor) incandescence. Here, we present an unprecedented-long (3 years) and continuous volcanic gas record that instrumentally characterizes the (re)activation of the lava-lake. Our results show that, before appearance of the lake, the volcanic gas plume composition became unusually CO2-rich, as testified by high CO2/SO2 ratios (mean, 12.2±6.3) and low H2O/CO2 ratios (mean, 2.3±1.3). The volcanic CO2 flux also peaked in November 2015 (mean, 81.3±40.6 kg/s; maximum, 247 kg/s). Using results of magma degassing models and budgets, we interpret this elevated CO2 degassing as sourced by degassing of a volatile-rich fast-convecting (3.6-5.2 m3·s-1) magma, supplying CO2-rich gas bubbles from minimum equivalent depths of 0.36-1.4 km. We propose this elevated gas bubbles supply destabilized the shallow (<1 km) Masaya magma reservoir, leading to upward migration of vesicular (buoyant) resident magma, and ultimately to (re)formation of the lava lake. At onset of lava lake activity on 11 December 2015 (constrained by satellite-based (MODIS) thermal observations), the gas emissions transitioned to more SO2-rich composition, and the SO2 flux increased by a factor ~40 % (11.4±5.2 kg/s) relative to background degassing (8.0 kg/s), confirming faster than normal (4.4 vs. ~3 m3·s-1) shallow magma convection. Elevated shallow magma circulation is also supported by gradual increase in irradiated thermal energy, captured by MODIS, from which we calculate that 0.4-0.8 m3·s-1 of magma have been surface-emplaced since December 2015.
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| 4. |
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| 5. |
- Arellano, Santiago, 1981, et al.
(författare)
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Long-term monitoring of SO2 quiescent degassing from Nyiragongo’s lava lake
- 2017
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Ingår i: Journal of African Earth Sciences. - : Elsevier BV. - 1879-1956 .- 1464-343X .- 0899-5362. ; 134, s. 866-873
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Tidskriftsartikel (refereegranskat)abstract
- The activity of open-vent volcanoes with an active lava-lake, such as Nyiragongo, is characterized by persistent degassing, thus continuous monitoring of the rate, volume and fate of their gas emissions is of great importance to understand their geophysical state and their potential impact. We report results of SO2 emission measurements from Nyiragongo conducted between 2004 and 2012 with a network of ground-based scanning-DOAS (Differential Optical Absorption Spectroscopy) remote sensors. The mean SO2 emission rate is found to be 13 ± 9 kg s−1, similar to that observed in 1959. Daily emission rate has a distribution close to log-normal and presents large inter-day variability, reflecting the dynamics of percolation of magma batches of heterogeneous size distribution and changes in the effective permeability of the lava lake. The degassed S content is found to be between 1000 and 2000 ppm from these measurements and the reported magma flow rates sustaining the lava lake. The inter-annual trend and plume height statistics indicate stability of a quiescently degassing lava lake during the period of study.
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| 6. |
- Arellano, Santiago, 1981, et al.
(författare)
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New developments on remote sensing studies of volcanic gas emissions by solar infrared spectroscopy
- 2011
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Ingår i: 11th IAVCEI-CCVG Gas Workshop, September 1 - 10, 2011, Kamchatka, Russia.
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Konferensbidrag (refereegranskat)abstract
- In this contribution, we will present some recent developments made by our group on the application of solar occultation remote sensing to the measurement of volcanic gas emissions in the infrared spectral region. These include the automation of Fourier Transform Spectrometers (FTS) and novel methods for radiation collection and spectrometric analysis.Solar FTS is a proven and versatile method for measuring volcanogenic gases. However, its relatively high cost and complexity on data collection and analysis have precluded its wider use by observatories as a permanent monitoring tool. We will present some results of a field experimentperformed at Popocatépetl volcano (Mexico) within the FIEL-VOLCAN project in April 2010, to show the feasibility of automating a solar FTS on volcanic settings to measure SO2/HCl molar ratios. The system includes a compact solar tracker for automatic radiation collection from a stationary point as well as an embedded computer for data acquisition. Data is evaluated off-line by using e.g., the Chalmers-QESOF program.Further simplifications of the transfer optics and spectroscopic analysis have been investigatedby our group and their operation principles and preliminary results will be presented.
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| 9. |
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| 10. |
- Arellano, Santiago, 1981, et al.
(författare)
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Prospects of a global network for studies of volcanic plumes
- 2009
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Ingår i: CEV-IAVCEI Workshop on Advances in studies of volcanic plumes and pyroclastic density currents, Clermont-Ferrand, France, Oct. 2009..
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Konferensbidrag (övrigt vetenskapligt/konstnärligt)
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