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Sökning: WAKA:ref > Inganäs Olle > Hamedi Mahiar > Herland Anna

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  • Hamedi, Mahiar, et al. (författare)
  • Electrochemical Devices Made from Conducting Nanowire Networks Self-Assembled from Amyloid Fibrils and Alkoxysulfonate PEDOT
  • 2008
  • Ingår i: Nano letters (Print). - 1530-6984. ; 8:6, s. 1736-1740
  • Tidskriftsartikel (refereegranskat)abstract
    • Proteins offer an almost infinite number of functions and geometries for building nanostructures. Here we have focused on amyloid fibrillar proteins as a nanowire template and shown that these fibrils can be coated with the highly conducting polymer alkoxysulfonate PEDOT through molecular self-assembly in water. Transmission electron microscopy and atomic force microscopy show that the coated fibers have a diameter around 15 nm and a length/thickness aspect ratio >1:1000 . We have further shown that networks of the conducting nanowires are electrically and electrochemically active by constructing fully functional electrochemical transistors with nanowire networks, operating at low voltages between 0 and 0.5 V.
  • Karlsson, Roger, et al. (författare)
  • Iron-Catalyzed Polymerization of Alkoxysulfonate-Functionalized 3,4-Ethylenedioxythiophene Gives Water-Soluble Poly(3,4-ethylenedioxythiophene) of High Conductivity
  • 2009
  • Ingår i: Chemistry of Materials. - American Chemical Society (ACS). - 0897-4756. ; 21:9, s. 1815-1821
  • Tidskriftsartikel (refereegranskat)abstract
    • Chemical polymerization of a 3,4-ethylenedioxythiophene derivative bearing a sulfonate group (EDOTS) is reported. The polymer, PEDOT-S, is fully water-soluble and has been produced by polymerizing EDOT-S in water, using Na2S2O8 and a catalytic amount of FeCl3. Elemental analysis and XPS measurements indicate that PEDOT-S is a material with a substantial degree of self-doping, but also contains free sulfate ions as charge-balancing counterions of the oxidized polymer. Apart from self-doping PEDOT-S, the side chains enable full water solubility of the material; DLS studies show an average cluster size of only 2 nm. Importantly, the solvation properties of the PEDOT-S are reflected in spin-coated films, which show a surface roughness of 1.2 nm and good conductivity (12 S/cm) in ambient conditions. The electro-optical properties of this material are shown with cyclic voltammetry and spectroelectrochemical experiment reveals an electrochromic contrast (similar to 48% at lambda(max) = 606 nm).
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  • Resultat 1-3 av 3
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Konradsson, Peter, (2)
Åslund, Andreas, (2)
Karlsson, Roger H, (2)
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Fahlman, Mats, (1)
Liu, Xianjie, (1)
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