| 1. |
- Guenot, Diego, et al.
(författare)
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Photoemission time delay measurements and calculations close to the 3s ionization cross section minimum in ar
- 2012
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Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 85:5, s. 053424-
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Tidskriftsartikel (refereegranskat)abstract
- We present experimental measurements and theoretical calculations of photoionization time delays from the 3s and 3p shells in Ar in the photon energy range of 32-42 eV. The experimental measurements are performed by interferometry using attosecond pulse trains and the infrared laser used for their generation. The theoretical approach includes intershell correlation effects between the 3s and 3p shells within the framework of the random-phase approximation with exchange. The connection between single-photon ionization and the two-color two-photon ionization process used in the measurement is established using the recently developed asymptotic approximation for the complex transition amplitudes of laser-assisted photoionization. We compare and discuss the theoretical and experimental results, especially in the region where strong intershell correlations in the 3s -> kp channel lead to an induced Cooper minimum in the 3s ionization cross section.
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| 2. |
- Louisy, Maite, et al.
(författare)
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Gating attosecond pulses in a noncollinear geometry
- 2015
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Ingår i: Optica. - 2334-2536. ; 2:6, s. 563-566
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Tidskriftsartikel (refereegranskat)abstract
- The efficient generation of isolated attosecond pulses (IAPs), giving access to ultrafast electron dynamics in various systems, is a key challenge in attosecond science. IAPs can be produced by confining the extreme ultraviolet emission generated by an intense laser pulse to a single field half-cycle or, as shown recently, by employing angular streaking methods. Here, we experimentally demonstrate the angular streaking of attosecond pulse trains in a noncollinear geometry, leading to the emission of angularly separated IAPs. The noncollinear geometry simplifies the separation of the fundamental laser field and the generated pulses, making this scheme promising for intracavity attosecond pulse generation, thus opening new possibilities for high-repetition-rate attosecond sources. (C) 2015 Optical Society of America
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| 3. |
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| 4. |
- Gisselbrecht, Mathieu, et al.
(författare)
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Exploring single-photon ionization on the attosecond time scale
- 2012
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Ingår i: XXVII International Conference on Photonic, Electronic and Atomic Collisions (Icpeac 2011), Pts 1-15. - : IOP Publishing. - 1742-6588 .- 1742-6596. ; 388, s. 032025-032025
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Konferensbidrag (refereegranskat)abstract
- One of the fundamental processes in nature is the photoelectric effect in which an electron is ripped away from its atom via the interaction with a photon. This process was long believed to be instantaneous but with the development of attosecond pulses (1 as 10(-18) s) we can finally get an insight into its dynamic. Here we measure a delay in ionization time between two differently bound electrons. The outgoing electrons are created via ionization with a train of attosecond pulses and we probe their relative delay with a synchronized infrared laser. We demonstrate how this probe field influences the measured delays and show that this contribution can be estimated with a universal formula, which allows us to extract field free atomic data..
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| 5. |
- Guenot, Diego, et al.
(författare)
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Measurements of relative photoemission time delays in noble gas atoms
- 2014
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Ingår i: Journal of Physics B. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 47:24, s. 245602-
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Tidskriftsartikel (refereegranskat)abstract
- We determine relative photoemission time delays between valence electrons in different noble gas atoms (Ar, Ne and He) in an energy range between 31 and 37 eV. The atoms are ionized by an attosecond pulse train synchronized with an infrared laser field and the delays are measured using an interferometric technique. We compare our results with calculations using the random phase approximation with exchange and multi-configurational Hartree-Fock. We also investigate the influence of the different ionization angular channels.
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| 6. |
- Klünder, Kathrin, et al.
(författare)
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Probing Single-Photon Ionization on the Attosecond Time Scale
- 2011
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Ingår i: Physical Review Letters. - 1079-7114. ; 106:14
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Tidskriftsartikel (refereegranskat)abstract
- We study photoionization of argon atoms excited by attosecond pulses using an interferometric measurement technique. We measure the difference in time delays between electrons emitted from the 3s(2) and from the 3p(6) shell, at different excitation energies ranging from 32 to 42 eV. The determination of photoemission time delays requires taking into account the measurement process, involving the interaction with a probing infrared field. This contribution can be estimated using a universal formula and is found to account for a substantial fraction of the measured delay.
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| 7. |
- Lopez, Rodrigo, et al.
(författare)
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Time-resolved ellipticity gating of high-order harmonic emission
- 2004
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Ingår i: Physical Review A. ; 69, s. 1-053811
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Tidskriftsartikel (refereegranskat)abstract
- We present time-resolved cross-correlation measurements of extreme ultraviolet (xuv) pulses generated as high-order harmonics of intense 35 fs pulses, using a short (12 fs) probe pulse. We modulate the ellipticity of the laser driving the generation process such that the polarization is linear for short times around the temporal peak of the pulse. Since harmonic generation is strongly suppressed for very small amounts of driving laser ellipticity, the emission of xuv radiation can therefore be confined to times much shorter than the laser pulse duration. In addition, our setup allows us to continuously confine the xuv emission as well as to determine its frequency sweep during the pulse.
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| 8. |
- Sola, I. J., et al.
(författare)
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Temporal and spectral studies of high-order harmonics generated by polarization-modulated infrared fields
- 2006
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Ingår i: Physical Review A (Atomic, Molecular and Optical Physics). - 1050-2947. ; 74:1
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Tidskriftsartikel (refereegranskat)abstract
- The temporal confinement of high harmonic generation (HHG) via modulation of the polarization of the fundamental pulse is studied in both temporal and spectral domains. In the temporal domain, a collinear cross-correlation setup using a 40 fs IR pump for the HHG and a 9 fs IR pulse to probe the generated emission is used to measure the XUV pulse duration. The observed temporal confinement is found to be consistent with theoretical predictions. An increased confinement is observed when a 9 fs pulse is used to generate the harmonics. An important spectral broadening, including a continuum background, is also measured. Theoretical calculations show that with 10 fs driving pulses, either one or two main attosecond pulses are created depending on the value of the carrier envelope phase.
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| 9. |
- Zair, A, et al.
(författare)
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Time-resolved measurements of high order harmonics confined by polarization gating
- 2004
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Ingår i: Applied Physics B. - : Springer Science and Business Media LLC. - 0946-2171 .- 1432-0649. ; 78:7-8, s. 869-872
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Tidskriftsartikel (refereegranskat)abstract
- We investigate the temporal confinement of high order harmonic pulses generated by a femtosecond (fs) infrared (IR) pulse with a time varying polarization. We use a set of two birefringent quartz plates to modulate the IR polarization. It produces a short temporal gate of linear polarization where harmonics are efficiently generated during a small fraction of the IR pulse. By rotating one of the plates, the gate width can be continuously varied between 70 fs down to 7 fs. The XUV pulse duration is measured by cross-correlation with a probe IR pulse of 12 fs. When the gate width is decreased, a clear temporal confinement of the XUV emission is observed through the cross correlation signal. This experiment is the first direct experimental evidence in the temporal domain that the polarization gating technique can be used to significantly shorten the harmonic pulse duration.
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