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Observation of Feshbach Resonances in the F + H2 → HF + H Reaction

Qiu, Minghui (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Department of Physics, Dalian Jiaotong University, P. R. China.
Ren, Zefeng (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
Che, Li (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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Dai, Dongxu (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
Harich, Steven A. (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
Wang, Xiuyan (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
Yang, Xueming (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
Xu, Chuanxiu (author)
Institute of Theoretical and Computational Chemistry, Department of Chemistry, Nanjing University
Xie, Daiqian (author)
Institute of Theoretical and Computational Chemistry, Department of Chemistry, Nanjing University
Gustafsson, Magnus (author)
Department of Chemistry and Biochemistry, University of Colorado, Boulder
Skodje, Rex T. (author)
Department of Chemistry and Biochemistry, University of Colorado, Boulder
Sun, Zhigang (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Center for Theoretical and Computational Chemistry, Dalian Institute of Chemical Physics, Dalian, Department of Computational Science, National University of Singapore
Zhang, Donghui (author)
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Center for Theoretical and Computational Chemistry, Dalian Institute of Chemical Physics, Dalian, Department of Computational Science, National University of Singapore
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State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Department of Physics, Dalian Jiaotong University, P R. China. State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China (creator_code:org_t)
American Association for the Advancement of Science (AAAS), 2006
2006
English.
In: Science. - : American Association for the Advancement of Science (AAAS). - 0036-8075 .- 1095-9203. ; 311:5766, s. 1440-1443
Related links:
https://urn.kb.se/re...
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https://doi.org/10.1...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Reaction resonances, or transiently stabilized transition-state structures, have proven highly challenging to capture experimentally. Here, we used the highly sensitive H atom Rydberg tagging time-of-flight method to conduct a crossed molecular beam scattering study of the F + H2 → HF + H reaction with full quantum-state resolution. Pronounced forward-scattered HF products in the v′ = 2 vibrational state were clearly observed at a collision energy of 0.52 kcal/mol; this was attributed to both the ground and the first excited Feshbach resonances trapped in the peculiar HF(v′ = 3)-H′ vibrationally adiabatic potential, with substantial enhancement by constructive interference between the two resonances.

Subject headings

NATURVETENSKAP  -- Fysik -- Annan fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Other Physics Topics (hsv//eng)

Keyword

Tillämpad fysik
Tillämpad fysik

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art (subject category)

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