| 1. |
- Abdul-Redah, T, et al.
(författare)
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Anomalous neutron Compton scattering in metallic hydrides: new experiments
- 2000
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Ingår i: PHYSICA B. - : ELSEVIER SCIENCE BV. - 0921-4526. ; 276, s. 824-825
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Tidskriftsartikel (refereegranskat)abstract
- The time-of-flight spectra of the neutron Compton scattering of solid palladium hydrides were measured at room temperature. This experiment, which was motivated by previous measurements on liquid H2O/D2O mixtures as mel as on niobium hydrides, showed anom
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| 2. |
- Ahlberg, Martina, et al.
(författare)
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Effect of ferromagnetic proximity on critical behavior
- 2012
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Ingår i: Physical Review B Condensed Matter. - 0163-1829 .- 1095-3795. ; 85:22, s. 224425-1-224425-6
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Tidskriftsartikel (refereegranskat)abstract
- We have investigated the magnetic phase transition in amorphous Fe93Zr7(x angstrom)/Co95Zr5(1 angstrom) multilayers, where x = 25, 50, and 75. The extremely thin CoZr layer induces magnetic order at temperatures well above the inherent ordering temperature of Fe93Zr7. The changes in the critical exponent beta, associated with the temperature dependence of the magnetization, imply a crossover from two-to three-dimensional behavior as the FeZr thickness is reduced, consistent with a substantial magnetic induction in the FeZr layers. In addition we determined the exponents delta and gamma, of the critical isotherm and the susceptibility, respectively, and their values confirm the nonuniversal character of the phase transition. Scaling of the results yields an excellent data collapse and is found to hold in the crossover regime where the universality hypothesis is not applicable.
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| 3. |
- Ahlberg, Martina, et al.
(författare)
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Influence of boundaries on magnetic ordering in Fe/V superlattices
- 2010
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Ingår i: Physical Review B. Condensed Matter and Materials Physics. - 1098-0121 .- 1550-235X. ; 81:21, s. 214429-
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Tidskriftsartikel (refereegranskat)abstract
- We study the role of surface boundaries on the magnetic properties of [Fe/V](n) superlattice structures, with n=2-10. Using the magneto-optical Kerr effect and polarized neutron reflectivity measurements, we examine the evolution of both the total and the layer-resolved magnetizations as a function of temperature. By varying n, we observe a large shift in the transition temperatures T-c and a substantial change in the total magnetization critical exponent beta. In particular, the thicker samples exhibit nonuniversal exponent values. By resolving the magnetization as a function of position within the superlattice, we show that this behavior arises from contributions of the surfaces. Furthermore, we attribute the large shift in T-c to long-ranged interactions present in the superlattice.
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| 4. |
- Ahlberg, Martina, et al.
(författare)
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Reversed interface effects in amorphous FeZr/AlZr multilayers
- 2014
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Ingår i: Physical Review B. Condensed Matter and Materials Physics. - 1098-0121 .- 1550-235X. ; 90:18, s. 184403-
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Tidskriftsartikel (refereegranskat)abstract
- We report an anomalous enhancement of the critical temperature (T-c) when the thickness (d) of the magnetic layer is decreased from 60 to 20 angstrom in amorphous FeZr/AlZr multilayers. Further reduction of the thickness causes a decrease of T-c, as expected by finite-size scaling, while the magnetic moment decreases monotonically for all values of d. The increase of the critical temperature is attributed to a reversed interface effect where local changes in the nearest-neighbor distance and coordination number gives a higher effective magnetic coupling at the interfaces compared to the interior of the layer. We have successfully described the results within a model where such interface effects are combined with finite-size scaling.
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| 5. |
- Ahlberg, Martina, et al.
(författare)
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Temperature dependence of magnetic properties in weakly exchange coupled Fe/V superlattices
- 2013
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Ingår i: Journal of Magnetism and Magnetic Materials. - : Elsevier BV. - 0304-8853 .- 1873-4766. ; 341, s. 142-147
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Tidskriftsartikel (refereegranskat)abstract
- We use Fe(3)/V(x)Fe(3)/V(x) superlattices, x = 16-27 monolayers (ML) to explore the interlayer exchange coupling (IEC) as a function of both spacer layer thickness and temperature. Fe/V is a common model system for studies addressing the IEC, but the behavior in the weakly exchange coupled regime, complemented with the temperature dependence of the magnetic properties, have remained unexplored. We observe clear regions with ferro- and antiferromagnetic coupling, which is manifested in oscillations in the saturation field, the remanence and the critical temperature. The oscillation in the interlayer coupling (J') has a period of 5.8(1) ML. This is approximate to 0.8 ML smaller than observed for Fe(7)/V(x) superlattices which illustrates the influence of the magnetic layer thickness on the interlayer coupling. The temperature dependence of the remanent magnetization was proven to be significantly affected by the strength of the ferromagnetic coupling, leading to high values of the effective critical exponent beta(eff).
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| 6. |
- Ahlberg, Martina, et al.
(författare)
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Two-dimensional XY-like amorphous Co68Fe24Zr8/Al70Zr30 multilayers
- 2011
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Ingår i: Physical Review B. Condensed Matter and Materials Physics. - 1098-0121 .- 1550-235X. ; 83:22, s. 224404-
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Tidskriftsartikel (refereegranskat)abstract
- We present an experimental realization of a magnetic two-dimensional XY system using amorphous materials. The classification of the dimensionality is based on the critical behavior of amorphous Co68Fe24Zr8(d)/Al70O30 (20 angstrom) multilayers, where d = 11 - 16 angstrom. Analysis of the remanent magnetization, the magnetic isotherms, the initial susceptibility, and the magnetic correlation length shows that the magnetic phase transition can be described by the 2D XY model. The samples are not paramagnetic above the critical temperature but are characterized by local magnetic order manifested in the field and temperature dependence of the magnetization. Furthermore, an average spin-spin interaction length of 8.1 angstrom was estimated using the thickness dependence of the Curie temperature.
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| 7. |
- Ali, Hasan, 1985-, et al.
(författare)
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Atomic resolution energy-loss magnetic chiral dichroism measurements enabled by patterned apertures
- 2020
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Ingår i: Physical Review Research. - College Park USA. - 2643-1564. ; 2:2
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Tidskriftsartikel (refereegranskat)abstract
- Electron energy-loss magnetic chiral dichroism (EMCD) has the potential to measure magnetic properties of the materials at atomic resolution but the complex distribution of magnetic signals in the zone axis and the overlapping diffraction discs at higher beam convergence angles make the EMCD signal acquisition challenging. Recently, the use of ventilator apertures to acquire the EMCD signals with atomic resolution was proposed. Here we give the experimental demonstration of several types of ventilator apertures and obtain a clear EMCD signal at beam semiconvergence angles of 5 mrad. To simplify the experimental procedures, we propose a modified ventilator aperture which not only simplifies the complex scattering conditions but reduces the influence of lens aberrations on the EMCD signal as compared to the originally proposed ventilator apertures. In addition, this modified aperture can be used to analyze magnetic crystals with various symmetries and we demonstrate this feature by acquiring EMCD signals on different zone axis orientations of an Fe crystal. With the same aperture we obtain EMCD signals with convergence angles corresponding to atomic resolution electron probes. After the theoretical demonstration of the EMCD signal on a zone axis orientation at high beam convergence angles, this work thus overcomes the experimental and methodological hurdles and enables atomic resolution EMCD on the zone axis by using apertures.
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| 8. |
- Ali, Hasan, 1985-, et al.
(författare)
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Quantitative EMCD by use of a double aperture for simultaneous acquisition of EELS
- 2019
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Ingår i: Ultramicroscopy. - : Elsevier BV. - 0304-3991 .- 1879-2723. ; 196, s. 192-196
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Tidskriftsartikel (refereegranskat)abstract
- The weak signal strength in electron magnetic circular dichroism (EMCD) measurements remains one of the main challenges in the quantification of EMCD related EELS spectra. As a consequence, small variations in peak intensity caused by changes of background intervals, choice of method for extraction of signal intensity and equally differences in sample quality can cause strong changes in the EMCD signal. When aiming for high resolution quantitative EMCD, an additional difficulty consists in the fact that the two angular resolved EELS spectra needed to obtain the EMCD signal are taken at two different instances and it cannot be guaranteed that the acquisition conditions for these two spectra are identical. Here, we present an experimental setup where we use a double hole aperture in the transmission electron microscope to obtain the EMCD signal in a single acquisition. This geometry allows for the parallel acquisition of the two electron energy loss spectra (EELS) under exactly the same conditions. We also compare the double aperture acquisition mode with the qE acquisition mode which has been previously used for parallel acquisition of EMCD. We show that the double aperture mode not only offers better signal to noise ratio as compared to qE mode but also allows for much higher acquisition times to significantly improve the signal quality which is crucial for quantitative analysis of the magnetic moments.
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| 9. |
- Ali, Hasan, 1985-, et al.
(författare)
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Simultaneous mapping of EMCD signals and crystal orientations in a transmission electron microscope
- 2021
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Ingår i: Scientific Reports. - : Springer Nature. - 2045-2322. ; 11
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Tidskriftsartikel (refereegranskat)abstract
- When magnetic properties are analysed in a transmission electron microscope using the technique of electron magnetic circular dichroism (EMCD), one of the critical parameters is the sample orientation. Since small orientation changes can have a strong impact on the measurement of the EMCD signal and such measurements need two separate measurements of conjugate EELS spectra, it is experimentally non-trivial to measure the EMCD signal as a function of sample orientation. Here, we have developed a methodology to simultaneously map the quantitative EMCD signals and the local orientation of the crystal. We analyse, both experimentally and by simulations, how the measured magnetic signals evolve with a change in the crystal tilt. Based on this analysis, we establish an accurate relationship between the crystal orientations and the EMCD signals. Our results demonstrate that a small variation in crystal tilt can significantly alter the strength of the EMCD signal. From an optimisation of the crystal orientation, we obtain quantitative EMCD measurements.
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| 10. |
- Ali, Hasan, 1985-, et al.
(författare)
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Single scan STEM-EMCD in 3-beam orientation using a quadruple aperture
- 2023
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Ingår i: Ultramicroscopy. - : Elsevier BV. - 0304-3991 .- 1879-2723. ; 251
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Tidskriftsartikel (refereegranskat)abstract
- The need to acquire multiple angle-resolved electron energy loss spectra (EELS) is one of the several critical challenges associated with electron magnetic circular dichroism (EMCD) experiments. If the experiments are performed by scanning a nanometer to atomic-sized electron probe on a specific region of a sample, the precision of the local magnetic information extracted from such data highly depends on the accuracy of the spatial registration between multiple scans. For an EMCD experiment in a 3-beam orientation, this means that the same specimen area must be scanned four times while keeping all the experimental conditions same. This is a non-trivial task as there is a high chance of morphological and chemical modification as well as non-systematic local orientation variations of the crystal between the different scans due to beam damage, contamination and spatial drift. In this work, we employ a custom-made quadruple aperture to acquire the four EELS spectra needed for the EMCD analysis in a single electron beam scan, thus removing the above-mentioned complexities. We demonstrate a quantitative EMCD result for a beam convergence angle corresponding to sub-nm probe size and compare the EMCD results for different detector geometries.
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