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Träfflista för sökning "WFRF:(Niklasson B) ;pers:(Johansson B)"

Sökning: WFRF:(Niklasson B) > Johansson B

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1.
  • Abrikosov, IA, et al. (författare)
  • Order-N Green's function technique for local environment effects in alloys
  • 1996
  • Ingår i: PHYSICAL REVIEW LETTERS. - : AMER INST PHYSICS. ; 76:22, s. 4203-4206
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • We have developed a new approach to the calculations of ground state properties of large crystalline systems with arbitrary atomic configurations based on a Green's function technique in conjunction with a self-consistent effective medium for the underlyi
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3.
  • Henk, J, et al. (författare)
  • Magnetic structure and anisotropy of ultra-thin Ni films on Cu(001)
  • 1998
  • Ingår i: PHILOSOPHICAL MAGAZINE B-PHYSICS OF CONDENSED MATTER STATISTICAL MECHANICS ELECTRONIC OPTICAL AND MAGNETIC PROPERTIES. - : TAYLOR & FRANCIS LTD. - 0141-8637. ; 78:5-6, s. 585-589
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • Both magnetic structure and magnetic anisotropy energy (MAE) are calculated for fee and fct Ni films on Cu(001) for thicknesses from I to 10 monolayers (ML). The transition from in-plane to perpendicular anisotropy can be attributed to the volume contribu
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4.
  • Henk, J, et al. (författare)
  • Magnetism and anisotropy of ultrathin Ni films on Cu(001)
  • 1999
  • Ingår i: PHYSICAL REVIEW B-CONDENSED MATTER. - : AMERICAN PHYSICAL SOC. - 0163-1829. ; 59:14, s. 9332-9341
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • Both magnetic structure and magnetic-anisotropy energies are calculated for cubic and tetragonal Ni films on Cu(001) for thicknesses from 1 to 10 monolayers. The magnetic reorientation transition from in-plane to perpendicular anisotropy can be attributed
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7.
  • Johansson, Malin B., et al. (författare)
  • Electronic and optical properties of nanocrystalline WO3 thin films studied by optical spectroscopy and density functional calculations
  • 2013
  • Ingår i: Journal of Physics. - : IOP Publishing. - 0953-8984 .- 1361-648X. ; 25:20, s. 205502-
  • Tidskriftsartikel (refereegranskat)abstract
    • The optical and electronic properties of nanocrystalline WO3 thin films prepared by reactive dc magnetron sputtering at different total pressures (P-tot) were studied by optical spectroscopy and density functional theory (DFT) calculations. Monoclinic films prepared at low P-tot show absorption in the near infrared due to polarons, which is attributed to a strained film structure. Analysis of the optical data yields band-gap energies E-g approximate to 3.1 eV, which increase with increasing P-tot by 0.1 eV, and correlate with the structural modifications of the films. The electronic structures of triclinic delta-WO3, and monoclinic gamma- and epsilon-WO3 were calculated using the Green function with screened Coulomb interaction (GW approach), and the local density approximation. The delta-WO3 and gamma-WO3 phases are found to have very similar electronic properties, with weak dispersion of the valence and conduction bands, consistent with a direct band-gap. Analysis of the joint density of states shows that the optical absorption around the band edge is composed of contributions from forbidden transitions (>3 eV) and allowed transitions (>3.8 eV). The calculations show that E-g in epsilon-WO3 is higher than in the delta-WO3 and gamma-WO3 phases, which provides an explanation for the P-tot dependence of the optical data.
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8.
  • Johansson, Malin B., et al. (författare)
  • Optical properties of nanocrystalline WO3 and WO3-x thin films prepared by DC magnetron sputtering
  • 2014
  • Ingår i: Journal of Applied Physics. - : American Institute of Physics (AIP). - 0021-8979 .- 1089-7550. ; 115:21, s. 213510-
  • Tidskriftsartikel (refereegranskat)abstract
    • The optical properties of tungsten trioxide thin films prepared by DC magnetron sputtering, withdifferent oxygen vacancy (Vo) concentration, have been studied by spectrophotometry andphotoluminescence (PL) emission spectroscopy. Absorption and PL spectra show that the filmsexhibit similar band gap energies, Eg 2.9 eV. The absorption spectra of the films show twopronounced absorption bands in the near-infrared region. One peak (P1) is located atapproximately 0.7 eV, independent of Vo concentration. A second peak (P2) shifts from 0.96 eV to1.16 eV with decreasing Vo concentration. Peak P1 is assigned to polaron absorption due totransitions between tungsten sites (W5þ!W6þ), or an optical transition from a neutral vacancystate to the conduction band, Vo0!W6þ. The origin of peak P2 is more uncertain but may involveþ1 and þ2 charged vacancy sites. The PL spectra show several emission bands in the range 2.07 to3.10 eV in the more sub-stoichiometric and 2.40 to 3.02 eV in the less sub-stoichiometric films.The low energy emission bands agree well with calculated optical transition energies of oxygenvacancy sites, with dominant contribution from neutral and singly charged vacancies in the lesssub-stoichiometric films, and additional contributions from doubly charged vacancy sites in themore sub-stoichiometric films.
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9.
  • Johansson, Malin B, 1972-, et al. (författare)
  • Porous Fractals of MAPbI3 Perovskite : Characterization of Crystal Grain Formation by Irreversible Diffusion-Limited Aggregation
  • 2018
  • Konferensbidrag (refereegranskat)abstract
    • Isopropanol solution based methylammonium lead triiodide (MAPbI3) is studied during the crystallization process. The crystal growth starts in an unstable suspension far from equilibrium by forming different dendritic patterns and terminates with aggregation of stable cubic crystalline grains into fractal clusters. Using transmission electron microscopy (TEM), the time evolution of a newly mixed suspension was studied over a period of two weeks at room temperature and a sequence of the morphological changes was observed. The crystallization process started with single dendritic growth exhibiting branches at 90 degrees angles to one another. After 4 hours, a multi-dendritic growth pattern and a transformation into small crystalline quantum dots were observed. After a week, clusters of crystal grains were formed into a fractal pattern and these patterns appear to be stable also during the second week. Electron and x-ray diffraction revealed the crystallinity of the quantum dots and the clusters of micrometer-sized crystals. Scanning transmission electron microscope (STEM) together with energy dispersive X-ray spectroscopy (EDS) showed that newly formed large grains, from a one hour old solution, displayed a core-shell structure with higher percentage of Pb atoms as compared to iodine at the surface. In the inner core of the grains the percentage of iodine was slightly higher. The electron diffraction (ED) scan over the newly formed grains revealed a polycrystalline surface whereas the inner part had a single crystal pattern. The same solution, now one-week-old, contained grains with only single crystal patterns in the ED scan and showed no core-shell character or polycrystalline surface. The measured percentage of iodine atoms compared to lead was 2:1 throughout the cross section, which is a quantitative value within the measurement. It can be concluded from these measurements that the suspension approaches higher crystallinity of the perovskite grains in an irreversible process, where the perovskite grains are insoluble in isopropanol. The perovskite material has also been characterized with scanning electron microscopy (SEM) and photoluminescence (PL) mapping where both techniques showed a very porous crystalline material. The PL mapping revealed two peaks at 730 and 760 nm for a thin film spin coated from a newly mixed solution, while a film deposited from a one week old solution showed three peaks, the last one at 830 nm. Because of the high crystallinity, it is suggested that all three peaks are due to band-to-band transitions and not due to localized states. These data will be analyzed further; however, the results contain information of the content of quantum dots versus larger crystals, as well as displaying emission intensity variations at different positions of the grains. The purpose with this project is to understand these phenomena of crystal growth. A new mesoporous perovskite material has been designed for optoelectronic purposes.
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10.
  • Johansson, Malin B, et al. (författare)
  • Structural and optical properties of visible active photocatalytic WO3 thin films prepared by reactive dc magnetron sputtering
  • 2012
  • Ingår i: Journal of Materials Research. - : Springer Science and Business Media LLC. - 0884-2914 .- 2044-5326. ; 27:24, s. 3130-3140
  • Tidskriftsartikel (refereegranskat)abstract
    • Nanostructured tungsten trioxide films were prepared by reactive dc magnetron sputteringat different working pressures P-tot = 1-4 Pa. The films were characterized by scanning electron microscopy, x-ray diffraction, Rutherford backscattering spectroscopy, Raman spectroscopy, and ultraviolet-visible spectrophotometry. The films were found to exhibit predominantly monoclinic structures and have similar band gap, E-g approximate to 2.8 eV, with a pronounced Urbach tail extending down to 2.5 eV. At low P-tot, strained film structures formed, which were slightly reduced and showed polaron absorption in the near-infrared region. The photodegradation rate of stearic acid was found to correlate with the stoichiometry and polaron absorption. This is explained by a recombination mechanism, whereby photoexcited electron-hole pairs recombine with polaron states in the band gap. The quantum yield decreased by 50% for photon energies close to E-g due to photoexcitations to band gap states lying below the O-2 affinity level.
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  • Resultat 1-10 av 26

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