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- Zhaunerchyk, Vitali, et al.
(author)
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Disentangling formation of multiple-core holes in aminophenol molecules exposed to bright X-FEL radiation
- 2015
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In: Journal of Physics B. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 48:24
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Journal article (peer-reviewed)abstract
- Competing multi-photon ionization processes, some leading to the formation of double core hole states, have been examined in 4-aminophenol. The experiments used the linac coherent light source (LCLS) x-ray free electron laser, in combination with a time-of-flight magnetic bottle electron spectrometer and the correlation analysis method of covariance mapping. The results imply that 4-aminophenol molecules exposed to the focused x-ray pulses of the LCLS sequentially absorb more than two x-ray photons, resulting in the formation of multiple core holes as well as in the sequential removal of photoelectrons and Auger electrons (so-called PAPA sequences).
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