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- Chua, C., et al.
(författare)
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Observation of Coulomb blockade in nanostructured epitaxial bilayer graphene on SiC
- 2017
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Ingår i: Carbon. - : Elsevier BV. - 0008-6223 .- 1873-3891. ; 119, s. 426-430
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Tidskriftsartikel (refereegranskat)abstract
- We study electron transport in nanostructures patterned in bilayer graphene patches grown epitaxially on SiC as a function of doping, magnetic field, and temperature. Away from charge neutrality transport is only weakly modulated by changes in carrier concentration induced by a local side-gate. At low n-type doping close to charge neutrality, electron transport resembles that in exfoliated graphene nanoribbons and is well described by tunnelling of single electrons through a network of Coulomb-blockaded islands. Under the influence of an external magnetic field, Coulomb blockade resonances fluctuate around an average energy and the gap shrinks as a function of magnetic field. At charge neutrality, however, conduction is less insensitive to external magnetic fields. In this regime we also observe a stronger suppression of the conductance below T*, which we interpret as a sign of broken interlayer symmetry or strong fluctuations in the edge/potential disorder.
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- Melios, C., et al.
(författare)
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Detection of Ultralow Concentration NO2 in Complex Environment Using Epitaxial Graphene Sensors
- 2018
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Ingår i: ACS Sensors. - : American Chemical Society (ACS). - 2379-3694. ; 3:9, s. 1666-1674
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Tidskriftsartikel (refereegranskat)abstract
- We demonstrate proof-of-concept graphene sensors for environmental monitoring of ultralow concentration NO2 in complex environments. Robust detection in a wide range of NO2 concentrations, 10-154 ppb, was achieved, highlighting the great potential for graphene-based NO2 sensors, with applications in environmental pollution monitoring, portable monitors, automotive and mobile sensors for a global real-time monitoring network. The measurements were performed in a complex environment, combining NO2/synthetic air/water vapor, traces of other contaminants, and variable temperature in an attempt to fully replicate the environmental conditions of a working sensor. It is shown that the performance of the graphene-based sensor can be affected by coadsorption of NO2 and water on the surface at low temperatures (≤70 °C). However, the sensitivity to NO2 increases significantly when the sensor operates at 150 °C and the cross-selectivity to water, sulfur dioxide, and carbon monoxide is minimized. Additionally, it is demonstrated that single-layer graphene exhibits two times higher carrier concentration response upon exposure to NO2 than bilayer graphene.
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