| 1. |
- Jacobsson, T. Jesper, 1984-, et al.
(författare)
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An open-access database and analysis tool for perovskite solar cells based on the FAIR data principles
- 2022
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Ingår i: Nature Energy. - : Springer Nature. - 2058-7546. ; 7:1, s. 107-115
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Tidskriftsartikel (refereegranskat)abstract
- Large datasets are now ubiquitous as technology enables higher-throughput experiments, but rarely can a research field truly benefit from the research data generated due to inconsistent formatting, undocumented storage or improper dissemination. Here we extract all the meaningful device data from peer-reviewed papers on metal-halide perovskite solar cells published so far and make them available in a database. We collect data from over 42,400 photovoltaic devices with up to 100 parameters per device. We then develop open-source and accessible procedures to analyse the data, providing examples of insights that can be gleaned from the analysis of a large dataset. The database, graphics and analysis tools are made available to the community and will continue to evolve as an open-source initiative. This approach of extensively capturing the progress of an entire field, including sorting, interactive exploration and graphical representation of the data, will be applicable to many fields in materials science, engineering and biosciences.
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| 2. |
- Cheng, W., et al.
(författare)
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Medial reward and lateral non-reward orbitofrontal cortex circuits change in opposite directions in depression
- 2016
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Ingår i: Brain. - : Oxford University Press. - 0006-8950 .- 1460-2156. ; 139:12, s. 3296-3309
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Tidskriftsartikel (refereegranskat)abstract
- The first brain-wide voxel-level resting state functional connectivity neuroimaging analysis of depression is reported, with 421 patients with major depressive disorder and 488 control subjects. Resting state functional connectivity between different voxels reflects correlations of activity between those voxels and is a fundamental tool in helping to understand the brain regions with altered connectivity and function in depression. One major circuit with altered functional connectivity involved the medial orbitofrontal cortex Brodmann area 13, which is implicated in reward, and which had reduced functional connectivity in depression with memory systems in the parahippocampal gyrus and medial temporal lobe, especially involving the perirhinal cortex Brodmann area 36 and entorhinal cortex Brodmann area 28. The Hamilton Depression Rating Scale scores were correlated with weakened functional connectivity of the medial orbitofrontal cortex Brodmann area 13. Thus in depression there is decreased reward-related and memory system functional connectivity, and this is related to the depressed symptoms. The lateral orbitofrontal cortex Brodmann area 47/12, involved in non-reward and punishing events, did not have this reduced functional connectivity with memory systems. Second, the lateral orbitofrontal cortex Brodmann area 47/12 had increased functional connectivity with the precuneus, the angular gyrus, and the temporal visual cortex Brodmann area 21. This enhanced functional connectivity of the non-reward/punishment system (Brodmann area 47/12) with the precuneus (involved in the sense of self and agency), and the angular gyrus (involved in language) is thus related to the explicit affectively negative sense of the self, and of self-esteem, in depression. A comparison of the functional connectivity in 185 depressed patients not receiving medication and 182 patients receiving medication showed that the functional connectivity of the lateral orbitofrontal cortex Brodmann area 47/12 with these three brain areas was lower in the medicated than the unmedicated patients. This is consistent with the hypothesis that the increased functional connectivity of the lateral orbitofrontal cortex Brodmann area 47/12 is related to depression. Relating the changes in cortical connectivity to our understanding of the functions of different parts of the orbitofrontal cortex in emotion helps to provide new insight into the brain changes related to depression.
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| 3. |
- Bayrak Pehlivan, Ilknur, et al.
(författare)
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Scalable and thermally-integrated solar water-splitting modules using Ag-doped Cu(In,Ga)Se2 and NiFe layered double hydroxide nanocatalysts
- 2022
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Ingår i: Journal of Materials Chemistry A. - : Royal Society of Chemistry. - 2050-7488 .- 2050-7496. ; 10:22, s. 12079-12091
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Tidskriftsartikel (refereegranskat)abstract
- Photovoltaic (PV) electrolysis is an important and powerful technology for environmentally-friendly fuel production based on solar energy. By directly coupling solar cell materials to electrochemical systems to perform water electrolysis, solar energy can be converted into hydrogen fuel utilizing locally-generated heat and avoid losses from DC-DC convertors and power grid transmission. Although there have been significant contributions to the photoelectrochemical and PV-electrolysis field using isolated laboratory cells, the capacity to upscale and retain high levels of efficiency in larger modules remains a critical issue for widespread use and application. In this study, we develop thermally-integrated, solar-driven water-splitting device modules using AgCu(In,Ga)Se2 (ACIGS) and an alkaline electrolyzer system with NiFe-layered double hydroxide (LDH) nanocatalysts with devices of 82-100 cm2 area. The Ga-content in the ACIGS solar cells is tuned to achieve an optimal voltage for the catalyst system, and the average efficiencies and durability of the PV-electrolyzer were tested in up to seven-day indoor and 21 day outdoor operations. We achieved a solar-to-hydrogen (STH) module efficiency of 13.4% from gas volume measurements for the system with a six-cell CIGS-electrolyzer module with an active area of 82.3 cm2 and a 17.27% PV module efficiency under 100 mW cm−2 illumination, and thus 77% electricity-to-hydrogen efficiency at one full sun. Outdoor tests under mid-Europeen winter conditions exhibited an STH efficiency between 10 and 11% after the initial activation at the installation site in Jülich, Germany, in December 2020, despite challenging outdoor-test weather conditions, including sub-zero temperatures.
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| 4. |
- Chen, G., et al.
(författare)
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Energy-Cascaded Upconversion in an Organic Dye-Sensitized Core/Shell Fluoride Nanocrystal
- 2015
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Ingår i: Nano letters (Print). - : American Chemical Society (ACS). - 1530-6984 .- 1530-6992. ; 15:11, s. 7400-7407
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Tidskriftsartikel (refereegranskat)abstract
- Lanthanide-doped upconversion nanoparticles hold promises for bioimaging, solar cells, and volumetric displays. However, their emission brightness and excitation wavelength range are limited by the weak and narrowband absorption of lanthanide ions. Here, we introduce a concept of multistep cascade energy transfer, from broadly infrared-harvesting organic dyes to sensitizer ions in the shell of an epitaxially designed core/shell inorganic nanostructure, with a sequential nonradiative energy transfer to upconverting ion pairs in the core. We show that this concept, when implemented in a core-shell architecture with suppressed surface-related luminescence quenching, yields multiphoton (three-, four-, and five-photon) upconversion quantum efficiency as high as 19% (upconversion energy conversion efficiency of 9.3%, upconversion quantum yield of 4.8%), which is about ∼100 times higher than typically reported efficiency of upconversion at 800 nm in lanthanide-based nanostructures, along with a broad spectral range (over 150 nm) of infrared excitation and a large absorption cross-section of 1.47 × 10-14 cm2 per single nanoparticle. These features enable unprecedented three-photon upconversion (visible by naked eye as blue light) of an incoherent infrared light excitation with a power density comparable to that of solar irradiation at the Earth surface, having implications for broad applications of these organic-inorganic core/shell nanostructures with energy-cascaded upconversion.
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| 5. |
- Ma, Y., et al.
(författare)
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Theoretical research on flow instability in parallel channels under motion conditions
- 2013
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Ingår i: Proceedings of the 21st International Conference on Nuclear Engineering --2013. - : ASME Press. - 9780791855812
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Konferensbidrag (refereegranskat)abstract
- In motion conditions, in addition to gravitational acceleration, a new acceleration was developed and it was added to the thermal hydraulics characteristics in flow channels. The additional acceleration leads to the different thermal hydraulic characteristics and will trigger the flow oscillation and even flow instability in parallel channels. In order to study the effect of the additional acceleration on the flow oscillation, the corresponding physical models are established in this work. Through the deduction of the mathematical model, the code for flow instability under motion conditions with Gear algorithm is developed. The flow oscillation curves, critical power, marginal stability boundary (MSB) are obtained. After comparison and analysis, it is found that some motion conditions lead to flow periodic oscillation. Different flow passage position results in different oscillation amplitudes. The marginal stability boundaries (MSB) under different motion conditions fit well, that is, the effect of motion conditions on MSB is small. Number of channels has little effect; however, channel arrangement influences the flow in every channel. These conclusions are of great significance in marine reactor design.
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| 6. |
- Neff, Curtis W., et al.
(författare)
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Coupled resonator optical waveguide structures with highly dispersive media
- 2006
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Ingår i: Optoeletronic Materials and Devices, Pts 1 and 2. - BELLINGHAM, WA : SPIE-INT SOC OPTICAL ENGINEERING. - 0819464473 ; , s. U316-U324
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Konferensbidrag (refereegranskat)abstract
- Enhanced slow light propagation is predicted in a coupled resonator optical waveguide structure possessing highly dispersive elements using the finite-difference time-domain method. The group velocity is shown to be below 0.01c(0).
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| 7. |
- Neff, Curtis W., et al.
(författare)
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Coupled resonator optical waveguide structures with highly dispersive media
- 2007
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Ingår i: Optics Express. - 1094-4087. ; 15:16, s. 10362-10369
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Tidskriftsartikel (refereegranskat)abstract
- Analysis of photonic crystal coupled resonator optical waveguide (CROW) structures with a highly dispersive background medium is presented. A finite-difference time-domain algorithm was employed which contains an exact representation of the permittivity of a three-level atomic system which exhibits electromagnetically induced transparency (EIT). We find that the coupling strength between nearest-neighbor cavities in the CROW decreases with increasing steepness of the background dispersion, which is continuously tunable as it is directly related to the control field Rabi frequency. The weaker coupling decreases the speed of pulse propagation through the waveguide. In addition, due to the dispersive nature of the EIT background, the CROW band shape is tuned around a fixed k-point. Thus, the EIT background enables dynamic tunability of the CROW band shape and the group velocity in the structure at a fixed operating point in momentum space.
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| 8. |
- Neff, Curtis W., et al.
(författare)
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Modelling electromagnetically induced transparency media using the finite-difference time-domain method
- 2007
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Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 9
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Tidskriftsartikel (refereegranskat)abstract
- Time-domain electromagnetic modelling of complex structures which include both non-dispersive media and media exhibiting electromagnetically induced transparency (EIT) require a general, robust calculation method such as finite-difference time-domain (FDTD). We propose a complex-valued, exact two-pole representation of the permittivity of a three-level system which is suitable for integration into the FDTD algorithm via the auxiliary differential equation method. Our calculation model confirmed reported results which were calculated with an approximate representation of the EIT permittivity. Additionally, propagation calculations which mimic slow light experiments were performed. A major advantage of our representation is the ease with which changes in the control field Rabi frequency can be implemented by using a time-dependent permittivity.
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| 9. |
- Qiu, Min, et al.
(författare)
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Nanostructured plasmonic devices and their applications
- 2013
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Ingår i: 2013 IEEE 6th International Conference on Advanced Infocomm Technology, ICAIT 2013. - : IEEE. - 9781479904655 ; , s. 79-80
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Konferensbidrag (refereegranskat)abstract
- In this talk, we will review our recent works on nanostructured plasmonic devices, and their applications in high performance light absorption, photothermal effects, and partly in photonic integrations.
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| 10. |
- Ruan, Zhichao, et al.
(författare)
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Ideal cylindrical cloak : Perfect but sensitive to tiny perturbations
- 2007
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Ingår i: Physical Review Letters. - 0031-9007 .- 1079-7114. ; 99:11
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Tidskriftsartikel (refereegranskat)abstract
- A cylindrical wave expansion method is developed to obtain the scattering field for an ideal two-dimensional cylindrical invisibility cloak. A near-ideal model of the invisibility cloak is set up to solve the boundary problem at the inner boundary of the cloak shell. We confirm that a cloak with the ideal material parameters is a perfect invisibility cloak by systematically studying the change of the scattering coefficients from the near-ideal case to the ideal one. However, because of the slow convergence of the zeroth-order scattering coefficients, a tiny perturbation on the cloak would induce a noticeable field scattering and penetration.
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