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- Samuelsson, Göran S., et al.
(author)
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Large-scale field study on thin-layer capping of dioxin contaminated sediments in the Grenland fjords, Norway : Effects on marine benthic fauna
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Other publication (other academic/artistic)abstract
- The Grenland fjords on the South East Coast of Norway are heavily contaminated with dioxins and furans after emissions from past industrial activities. Thin layer capping with a 1.1 to 3.7 cm cap was tested as a remediation option in a large-scale in situ study in two different parts of the fjord system, in the Ormefjord at 25-30 meters depth and in the Eidangerfjord at 80-100 meters depth. Three different capping materials: Limestone gravel, Clay, and powdered activated carbon (AC) mixed into clay (AC+clay) was compared to untreated reference fields in order to evaluate their effects on contaminant sequestering and possible effects on the benthic communities. Sediment to water fluxes of contaminants were significantly reduced by the capping materials, especially with AC-clay and is reported in a companion study.This study discusses the ecological effects of the remediation 1 and 14 months post treatment. Capping with Clay and Lime had minor and short-lasting effects on benthic fauna. Capping with AC+clay, however, had led to profound and more long-lasting perturbations of the macrofauna. An initial massive decline in filter feeders and suspension feeders was observed after 1 month in the shallower Ormefjord. The negative effects got worse after 14 months and resulted in dramatic reductions of all feeding guilds. The number of species, organism abundances and biomass in the AC+clay field were ca 80-90 % lower compared to the reference fields after 14 months.The negative effects were less pronounced at the deeper (80-100 meters) location in the Eidangerfjord and were also stable with time, suggesting that the benthic community the deeper habitat was more resilient to the capping compared to the shallower community in Ormefjord.The differences in response of the two communities are hypothesized to be due to the higher macrofaunal diversity in the deeper location, as well as to differences in abiotic factors such as available food and temperature. Results from this study show that amendment with powdered AC can lead to serious perturbations of the benthic community, at least initially, i.e. one year post capping in this study. These results stresses that further long-term monitoring of these benthic communities is necessary before capping with AC+clay could be advocated as a potential remediation option.
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| 2. |
- Samuelsson, Göran S., et al.
(author)
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Reduced bioaccumulation of PCBs and PAHs by sediment fauna following in situ remediation with activated carbon in Trondheim Harbor (Norway)
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Other publication (other academic/artistic)abstract
- Thin-layer capping with activated carbon (AC) was deployed in experimental plots in Trondheim harbor, Norway, using caps containing AC+clay, AC-only or AC+sand. Intact sediment cores were collected from the in situ remediated plots to study the capping efficiency of the various AC treatments in reducing the aqueous concentrations and the bioaccumulation of polycyclic aromatic hydrocarbons (PAHs) and polychlorinated biphenyls (PCBs) in the polychaete Hediste diversicolor and the clam Abra nitida. Reduced aqueous concentrations were observed in all AC-treatments, but generally AC+clay appeared to be superior to the other tested treatments. Capping efficiency by AC+clay, in terms of reduced bioaccumulation of PAHs and PCBs, ranged between 40 % and 87% in the worms and between 67% and 97% in the clams. Sediment capped with AC-only also led to reduced bioaccumulation of PCBs, while AC+sand showed no reduction in bioaccumulation. The worms had lower relative lipid content in the AC-only treatment after exposure.
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| 5. |
- Josefsson, Sarah, 1976-, et al.
(author)
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Capping efficiency of various carbonaceous and mineral materials for in situ remediation of marine sediments contaminated with PCDD/Fs, OCS and HCB
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Other publication (other academic/artistic)abstract
- The efficiency of various thin-layer capping materials in reducing the sediment-to-water flux and benthic organism bioaccumulation of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs), hexachlorobenzene (HCB) and octachlorostyrene (OCS) was investigated in a boxcosm experiment. The influence of cap layer thickness (0.5-5 cm) and different cap materials were tested using a three-factor experimental design. The capping materials consisted of a passive carrier (coarse or fine limestone material, or a marine clay sediment), and an active material (activated carbon (AC) or kraft lignin) to sequester the contaminants and decrease their bioavailability. Macrofauna was added to the boxes to get a semi-natural bioturbation. The sediment-to-water flux was measured using passive (SPMD) samplers, and the bioaccumulation by the surface-dwelling gastropod Hinia reticulata and the deep-burrowing polychaetes Nereis spp. was determined. Results showed substantial decreases in both flux and bioaccumulation as a result of thin-layer capping. The thickness of the capping layer and the choice of active material were important factors, while the use of different types of passive materials was not statistically significant for any of the observed endpoints. Flux and bioaccumulation decreased with increased cap thickness, and could be further decreased with addition of active material. Activated carbon was more efficient than lignin, and a ~90% reduction of the flux and bioaccumulation, compared to uncapped control sediment, could be achieved with 3 cm caps with 3.3% AC (g C/g ww clay). The reduction was generally larger in the surface-dwelling H. reticulata than in Nereis spp., and the magnitude of the reduction was frequently similar between Nereis spp. and sediment-to-water fluxes. The latter was interpreted to indicate a link between Nereis spp. bioirrigation and sediment-to-water fluxes. Furthermore, the reduction in sediment-to-water flux was dependent on the hydrophobicity of the congeners, with less hydrophobic congeners achieving a larger reduction than more hydrophobic congeners.
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| 6. |
- Samuelsson, Karl, Postdoktor, et al.
(author)
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Diverse experiences by active travel: Longitudinal study reveals a persistent discrepancy across residential contexts
- 2023
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Other publication (other academic/artistic)abstract
- To inform spatial planning promoting low-carbon travel and well-being, we investigate the potential for experiential diversity by active travel across different residential contexts. We use spatiotemporal tracking and experience data from the Gävle city-region, Sweden, generated by 165 participants over the course of 15 months. Findings reveal a discrepancy between typical travel distances to locations of positive experiences (1.5–5 km) and the distances at which active travel dominates (up to 1.5 km). This discrepancy largely persists across urban, suburban, and peripheral contexts, with urban dwellers travelling further for nature experiences, whereas peripheral dwellers travel further for urbanicity experiences. These results illustrate the importance of spatial scale for promoting diverse positive experiences by active travel, regardless of residential context. Planning strategies include enhancing environmental diversity close to people’s homes and providing infrastructure that promotes switching from motorised to active travel for trips of a few kilometres.
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