| 1. |
- Biemont, E, et al.
(författare)
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Core-polarization effects and radiative lifetime measurements in PrIII
- 2001
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Ingår i: Physical Review A (Atomic, Molecular and Optical Physics). - 1050-2947. ; 64:2
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Tidskriftsartikel (refereegranskat)abstract
- New radiative lifetimes of eight levels in Pr III have been measured using the time-resolved laser-induced fluorescence method. A tunable frequency-doubled dye laser with 1-ns pulse duration was used to excite selectively doubly ionized praseodymium in a laser-produced plasma. The experimental results agree generally well with theoretical data, provided core-polarization effects are considered in the calculations in an adequate way.
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| 2. |
- Biemont, E, et al.
(författare)
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Doubly ionized thorium: Laser lifetime measurements and transition probability determination of interest in cosmochronology
- 2002
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Ingår i: Astrophysical Journal. - : American Astronomical Society. - 0004-637X .- 1538-4357. ; 567:2, s. 1276-1283
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Tidskriftsartikel (refereegranskat)abstract
- The first lifetime measurements have been performed for six levels of doubly ionized thorium, an important cosmochronometer in astrophysics for estimating the age of the Galaxy. The levels, belonging to the 5f(2), 5f7p, 7s7p, and 6d7p configurations of Th III, have been measured by the time-resolved laser-induced fluorescence method and compared with relativistic Hartree-Fock calculations including configuration interaction and core-polarization effects. Taking advantage of the excellent agreement between theory and experiment, a first set of transition probabilities of astrophysical interest has been deduced for this ion from a combination of the experimental lifetimes and of the theoretical branching fractions.
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| 3. |
- Biemont, E, et al.
(författare)
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Experimental and theoretical energy levels, transition probabilities and radiative lifetimes in YbIII
- 2001
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Ingår i: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 34:10, s. 1869-1876
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Tidskriftsartikel (refereegranskat)abstract
- The analysis of the spectrum of Yb rn has been extended allowing us to establish 11 new energy level values. In addition, radiative lifetimes of two excited states of Yb III have been measured for the first time using time-resolved laser-induced fluorescence following two-photon excitation. The good agreement between experimental results and semi-empirical calculations performed with the relativistic Hartree-Fock method including core-polarization effects allows the determination of transition probabilities for 15 lines.
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| 4. |
- Biemont, E, et al.
(författare)
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Experimental lifetime determination in neutral praseodymium (Pr I) and neodymium (Nd I)
- 2004
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Ingår i: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 37:7, s. 1381-1389
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Tidskriftsartikel (refereegranskat)abstract
- Radiative lifetime measurements have been performed, with a time-resolved laser-induced fluorescence technique, for 18 even-parity levels of Pr I and 15 odd-parity levels of Nd I. The new results are compared with the few experimental data available in the literature and good agreement is found. However, fragmentary knowledge of the spectra prevents reliable calculation of branching fractions and calls for additional laboratory efforts in order to provide the astrophysicists with reliable transition probabilities needed for investigating the magnetic fields in chemically peculiar stars.
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| 5. |
- Biemont, E, et al.
(författare)
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Lifetime measurements and calculations in LaI
- 2004
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Ingår i: European Physical Journal D. Atomic, Molecular, Optical and Plasma Physics. - : Springer Science and Business Media LLC. - 1434-6060. ; 30:2, s. 157-162
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Tidskriftsartikel (refereegranskat)abstract
- Radiative lifetime measurements have been performed, with a time-resolved laser-induced fluorescence technique, for 20 odd-parity levels of La I belonging to the configurations 5d(2)6p, 5d6s6p and 4f5d6s. The new results are compared with the few experimental data available in the literature and with theoretical calculations including configuration interaction effects. The agreement theory-experiment is generally satisfying but discrepancies are observed for some levels emphasizing the difficulty to get a reliable theoretical model in such a heavy and complex neutral element.
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| 6. |
- Biemont, E, et al.
(författare)
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Lifetime measurements and calculations in singly ionized ytterbium
- 2002
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Ingår i: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075. ; 35:22, s. 4743-4749
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Tidskriftsartikel (refereegranskat)abstract
- New radiative lifetimes, measured by time-resolved laser-induced fluorescence spectroscopy, are reported for five Rydberg states of singly ionized ytterbium. Free Yb+ ions were produced in a laser-induced plasma. The experimental results have been compared with HFR calculations, taking core-polarization effects into account, and a good agreement (within 25%) between theory and experiment is observed for four levels. HFR results are also proposed for np (n less than or equal to 7) and nf (n less than or equal to 8) Rydberg states and compared with available data.
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| 7. |
- Biemont, E, et al.
(författare)
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Lifetime measurements for doubly ionized uranium
- 2002
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Ingår i: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 35:7, s. 1701-1705
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Tidskriftsartikel (refereegranskat)abstract
- The first lifetime measurements for doubly ionized uranium are reported in the present work. They relate to five levels belonging to the configurations 5f(2)6d(2), 5f(2)6d7s and 5f(3)7p and have been obtained with a time-resolved laser-induced-fluorescence technique, the ions being produced by laser ablation of a uranium oxide target.
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| 8. |
- Biemont, E, et al.
(författare)
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Lifetimes along perturbed Rydberg series in neutral thallium
- 2005
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Ingår i: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 38:19, s. 3547-3558
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Tidskriftsartikel (refereegranskat)abstract
- Radiative lifetimes of 15 Tl I levels belonging to the 6s(2)ns(2)S(1/2) (n = 7-14) and 6s(2)nd(2)D(3/2) Rydberg series (n = 6-12) have been measured using a time-resolved laser-induced fluorescence technique. All the measured levels have been excited from the ground state 6s(2)6p(2)P(1/2)(0) (odd parity) with a single-step excitation process. The general perturbation of the ns series by the 6s6p(2) configuration and the corresponding modification of the lifetimes are adequately reproduced by a theoretical model including core-polarization effects and combined with a least-squares fit to the observed energy levels. The general behaviour of the lifetime values for the 6s(2)np odd levels along the Rydberg series is also well reproduced. The use of the multiconfiguration quantum defect theory has allowed us to obtain lifetime values along the 6s(2)ns(2)S(1/2) series up to levels with n = 31.
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| 9. |
- Biemont, E, et al.
(författare)
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Measurement of radiative lifetimes and determination of transition probabilities of astrophysical interest in HoIII
- 2001
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Ingår i: Monthly Notices of the Royal Astronomical Society. - : Oxford University Press (OUP). - 1365-2966 .- 0035-8711. ; 328:4, s. 1085-1090
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Tidskriftsartikel (refereegranskat)abstract
- Lifetimes of six levels belonging to the 4f(10)6p configuration of Ho III have been measured for the first time using the time-resolved laser-induced fluorescence method. They are compared with multiconfigurational pseudo-relativistic Hartree-Fock calculations. A very good agreement is found. Using the experimental lifetimes and theoretical branching fractions, a first set of transition probabilities of astrophysical interest has been obtained for this ion.
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| 10. |
- Biémont, E, et al.
(författare)
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Radiative lifetime and oscillator strength determinations in Sm III
- 2003
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Ingår i: Astronomy & Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 399:1, s. 343-349
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Tidskriftsartikel (refereegranskat)abstract
- Radiative lifetimes of 6 levels belonging to the4f5(6Hdeg,6Fdeg)5d configuration of Sm III have beenmeasured for the first time using a time-resolved laser-inducedfluorescence technique. Experimental data have been compared withsemi-empirical calculations. The agreement is excellent for 4 levelswith 6Fdeg as a parent term. Larger discrepancies(53 and 37) are observed for 2 levels with 6Hdegand 6Fdeg, respectively, as a parent term and areexplainable by strong mixing and cancellation effects occurring in theline strength calculations which are responsible of instabilitiesoccurring in the lifetimes considered as a function of J value withinthe term. Branching ratios for the lines depopulating the levels ofinterest have been measured by Fourier transform spectroscopy. A firstset of oscillator strengths has been deduced for this ion.
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