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  • Martinsson, Johan, et al. (författare)
  • Impacts of Combustion Conditions and Photochemical Processing on the Light Absorption of Biomass Combustion Aerosol
  • 2015
  • Ingår i: Environmental Science and Technology. - : American Chemical Society (ACS). - 0013-936X .- 1520-5851. ; 49:24, s. 14663-14671
  • Tidskriftsartikel (refereegranskat)abstract
    • The aim was to identify relationships between combustion conditions, particle characteristics, and optical properties of fresh and photochemically processed emissions from biomass combustion. The combustion conditions included nominal and high burn rate operation and individual combustion phases from a conventional wood stove. Low temperature pyrolysis upon fuel addition resulted in "tar-ball" type particles dominated by organic aerosol with an absorption Angstrom exponent (AAE) of 2.5-2.7 and estimated Brown Carbon contributions of 50-70% to absorption at the climate relevant aethalometer-wavelength (520 nm). High temperature combustion during the intermediate (flaming) phase was dominated by soot agglomerates with AAE 1.0-1.2 and 85-100% of absorption at 520 nm attributed to Black Carbon. Intense photochemical processing of high burn rate flaming combustion emissions in an oxidation flow reactor led to strong formation of Secondary Organic Aerosol, with no or weak absorption. PM1 mass emission factors (mg/kg) of fresh emissions were about an order of magnitude higher for low temperature pyrolysis compared to high temperature combustion. However, emission factors describing the absorption cross section emitted per kg of fuel consumed (m(2)/kg) were of similar magnitude at 520 nm for the diverse combustion conditions investigated in this study. These results provide a link between biomass combustion conditions, emitted particle types, and their optical properties in fresh and processed plumes which can be of value for source apportionment and balanced mitigation of biomass combustion emissions from a climate and health perspective.
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  • Pagels, Joakim, et al. (författare)
  • Chemical composition and mass emission factors of candle smoke particles
  • 2009
  • Ingår i: Journal of Aerosol Science. - : Elsevier BV. - 0021-8502. ; 40:3, s. 193-208
  • Tidskriftsartikel (refereegranskat)abstract
    • The aim of this study is to investigate the physical and chemical properties of particle emissions from candle burning in indoor air. Two representative types of tapered candies were studied during steady burn, sooting burn and smouldering (upon extinction) under controlled conditions in a walk-in stainless steel chamber. Steady burn emits relatively high number emissions of ultrafine particles dominated by either phosphates or alkali nitrates. The likely source of these particles is flame retardant additives to the wick. Sooting burn in addition emits larger particles mainly consisting of agglomerated elemental carbon. This burning mode is associated with the highest mass emission factors. Particles emitted during smouldering upon extinction are dominated by organic matter. A mass closure was illustrated for the total mass concentration, the summed mass concentration from chemical analysis and the size-integrated mass concentration assessed from number distribution measurements using empirically determined effective densities for the three particle types. (C) 2008 Published by Elsevier Ltd.
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