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Advanced opportunities and insights on the influence of nitrogen incorporation on the physico-/electro-chemical properties of robust electrocatalysts for electrocatalytic energy conversion

Chandrasekaran, Sundaram (author)
Guangxi Key Laboratory of Electrochemical and Magneto-chemical, Functional Materials, College of Chemistry and Bioengineering, Guilin University of Technology, Guilin 541004, PR China; College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen 518060, PR China
Zhang, Chenle (author)
College of Julong, Shenzhen Technology University, Shenzhen Guangdong 518118, PR China
Shu, Yiqing (author)
Key Laboratory of Optoelectronic Devices, Systems of Ministry of Education and Guangdong Province, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
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Wang, Huide (author)
Key Laboratory of Optoelectronic Devices, Systems of Ministry of Education and Guangdong Province, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
Chen, Sanming (author)
College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen 518060, PR China
Edison, Thomas Nesakumar Jebakumar Immanuel (author)
School of Chemical Engineering, Yeungnam University, Gyeongsan, Gyeongbuk 38541, Republic of Korea
Liu, Yongping (author)
Guangxi Key Laboratory of Electrochemical and Magneto-chemical, Functional Materials, College of Chemistry and Bioengineering, Guilin University of Technology, Guilin 541004, PR China
Namachivayam, Karthik (author)
Luleå tekniska universitet,Maskinelement
Misra, R.D.K. (author)
College of Engineering Metallurgical, Materials and Biomedical Engineering, University of Texas at El Paso, Texas 79968, USA
Deng, Libo (author)
College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen 518060, PR China
Yin, Peng (author)
Key Laboratory of Optoelectronic Devices, Systems of Ministry of Education and Guangdong Province, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
Ge, Yanqi (author)
Key Laboratory of Optoelectronic Devices, Systems of Ministry of Education and Guangdong Province, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
Al-Hartomy, Omar A. (author)
Department of Physics, Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia
Al-Ghamdi, Ahmed (author)
Department of Physics, Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia
Wageh, Swelm (author)
Department of Physics, Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia
Zhang, Peixin (author)
College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen 518060, PR China
Bowen, Chris (author)
Department of Mechanical Engineering, University of Bath, BA2 7AY Bath, UK
Han, Zhang (author)
Key Laboratory of Optoelectronic Devices, Systems of Ministry of Education and Guangdong Province, College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
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 (creator_code:org_t)
Elsevier, 2021
2021
English.
In: Coordination chemistry reviews. - : Elsevier. - 0010-8545 .- 1873-3840. ; 449
Related links:
https://urn.kb.se/re...
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https://doi.org/10.1...
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  • Research review (peer-reviewed)
Abstract Subject headings
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  • The use of a wide range of methods for incorporating nitrogen atoms on robust catalysts has given rise to fundamental advances in the field of energy conversion and storage. Recently, nitrogen incorporation has proven to be able to fine-tune the electron densities of exposed active sites to create high-performance electrocatalysts. The preservation of a strong interface between the local atomic coordination of nitrogen atoms on bare carbon, single metal atoms, transition metal oxides, metal chalcogenides, and MXenes during synthesis plays an important role in producing an efficient electrocatalysts. In addition, the ability of nitrogen atoms to bind with carbon or metal atoms can be influenced by processing conditions. In this regard, this review is the first comprehensive overview of the range of synthetic strategies to form nitrogen incorporated catalysts and assess their chemical, structural, physical electronic property modification and their influence on electrocatalytic ORR, OER, and HER performance. This review will describe how specific strategies have been utilized to realise effective electrocatalytic systems, including the energy conversion of nitrogen incorporated catalysts, structural coordination, and material optimization. Finally, the main challenges to be considered in future investigations in order to initiate new research efforts in this promising research area are discussed.

Subject headings

NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

Keyword

Nitrogen
N-doped carbon
Single-atom sites
N-doped metal oxides
N-doped metal chalcogenides
N-doped MXenes
ORR
OER
and HER
Maskinelement
Machine Elements

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