| 1. |
- Sobek, Anna, et al.
(författare)
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Organic matter degradation causes enrichment of organic pollutants in hadal sediments
- 2023
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Ingår i: Nature Communications. - 2041-1723. ; 14
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Tidskriftsartikel (refereegranskat)abstract
- Burial of persistent organic pollutants (POPs) such as polychlorinated biphenyls (PCBs) in deep-sea sediments contributes to 60% of their historical emissions. Yet, empirical data on their occurrence in the deep-ocean is scarce. Estimates of the deep-ocean POP sink are therefore uncertain. Hadal trenches, representing the deepest part of the ocean, are hotspots for organic carbon burial and decomposition. POPs favorably partition to organic carbon, making trenches likely significant sinks for contaminants. Here we show that PCBs occur in both hadal (7720–8085 m) and non-hadal (2560–4050 m) sediment in the Atacama Trench. PCB concentrations normalized to sediment dry weight were similar across sites while those normalized to sediment organic carbon increased exponentially as the inert organic carbon fraction of the sediment increased in degraded hadal sediments. We suggest that the unique deposition dynamics and elevated turnover of organic carbon in hadal trenches increase POP concentrations in the deepest places on Earth.
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| 2. |
- Ferraro, Mattia, et al.
(författare)
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Multi-century reconstruction of environmental conditions in Lurefjorden, Norway.
- 2024
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Ingår i: 24th Nordic Geological Winter Meeting, 10-12th Jan, 2024, Gothenburg, Sweden.
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Konferensbidrag (övrigt vetenskapligt/konstnärligt)abstract
- Benthic foraminiferal assemblages are identified to reconstruct changes in environmental conditions over the last few centuries in Lurefjorden, a western Norwegian fjord. From ca. 1970 until present days the relative abundance of Brizalina skagerrakkensis, an efficient bio-indicator for organic matter fluxes, is enhanced relative to the preceding time interval. Hence, our results suggest that there is an increase of the organic matter within the Lurefjorden basin in the last 50 years. Over the same period, there is also an increase in the absolute abundance of agglutinated species, indicating lower oxygen concentration in the water. A lowering of the oxygen concentrations may have taken place as a response of a greater oxygen consumption caused by a higher organic matter supply in the water column. Accoridng to Aksnes (2009), Lurefjorden was subject to an increased freshening of Norwegian coastal waters (NCW), which has led to a decrease in sunlight penetration into the water column, affecting the oxygen levels and the behavior of marine life within the basin, between 1935 and 2007. Furthermore, we used diversity indices to study the ecological status of the area, showing significant growth in diversity, abundance, and richness within the benthic foraminiferal community over the past 50 years. Our observations highlight that an increase in the input of organic matter over the last century has led to a change in the benthic foraminifera community in the Lurefjorden basin.
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| 3. |
- Barthel, Roland, 1967, et al.
(författare)
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Similarity-based approaches in hydrogeology: proposal of a new concept for data-scarce groundwater resource characterization and prediction
- 2021
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Ingår i: Hydrogeology Journal. - : Springer Science and Business Media LLC. - 1435-0157 .- 1431-2174. ; 29:5, s. 1693-1709
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Tidskriftsartikel (refereegranskat)abstract
- A new concept is proposed for describing, analysing and predicting the dynamic behaviour of groundwater resources based on classification and similarity. The concept makes use of the ideas put forward by the “PUB” (predictions in ungauged basins) initiative in surface-water hydrology. One of the approaches developed in PUB uses the principle that similar catchments, exposed to similar weather conditions, will generate a similar discharge response at the catchment outlet. This way, models developed for well-observed catchments can be used to make predictions for ungauged catchments with similar properties (topography, land use, etc.). The concept proposed here applies the same idea to groundwater systems, with the goal to make predictions of the dynamic behaviour of groundwater in poorly observed systems using similarities to well-observed and understood systems. This paper gives an overview of the main ideas, the methodological background, the progress so far, and the challenges that the authors regard as most crucial for further development. One of the main goals of this article is thus to raise interest for this new concept within the groundwater community. There are a multitude of highly interesting aspects to investigate, and a community effort, as with PUB, is required. A second goal is to foster and exchange ideas between the groundwater and surface water research communities who, while often working on similar problems, have often missed the opportunity to learn from each other.
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| 4. |
- Chan, Phoebe, et al.
(författare)
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Freshening of the Alaska Coastal Current recorded by coralline algal Ba/Ca ratios
- 2011
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Ingår i: Journal of Geophysical Research-Biogeosciences. - 0148-0227. ; 116
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Tidskriftsartikel (refereegranskat)abstract
- Arctic Ocean freshening can exert a controlling influence on global climate, triggering strong feedbacks on ocean-atmospheric processes and affecting the global cycling of the world's oceans. Glacier-fed ocean currents such as the Alaska Coastal Current are important sources of freshwater for the Bering Sea shelf, and may also influence the Arctic Ocean freshwater budget. Instrumental data indicate a multiyear freshening episode of the Alaska Coastal Current in the early 21st century. It is uncertain whether this freshening is part of natural multidecadal climate variability or a unique feature of anthropogenically induced warming. In order to answer this, a better understanding of past variations in the Alaska Coastal Current is needed. However, continuous long-term high-resolution observations of the Alaska Coastal Current have only been available for the last 2 decades. In this study, specimens of the long-lived crustose coralline alga Clathromorphum nereostratum were collected within the pathway of the Alaska Coastal Current and utilized as archives of past temperature and salinity. Results indicate that coralline algal Mg/Ca ratios provide a 60 year record of sea surface temperatures and track changes of the Pacific Decadal Oscillation, a pattern of decadal-to-multidecadal ocean-atmosphere climate variability centered over the North Pacific. Algal Ba/Ca ratios (used as indicators of coastal freshwater runoff) are inversely correlated to instrumentally measured Alaska Coastal Current salinity and record the period of freshening from 2001 to 2006. Similar multiyear freshening events are not evident in the earlier portion of the 60 year Ba/Ca record. This suggests that the 21st century freshening of the Alaska Coastal Current is a unique feature related to increasing glacial melt and precipitation on mainland Alaska.
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| 5. |
- Gamboa, G., et al.
(författare)
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Mg/Ca ratios in coralline algae record northwest Atlantic temperature variations and North Atlantic Oscillation relationships
- 2010
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Ingår i: Journal of Geophysical Research-Oceans. - 0148-0227. ; 115
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Tidskriftsartikel (refereegranskat)abstract
- [1] Climate variability in the North Atlantic has been linked in part to the North Atlantic Oscillation (NAO). The NAO influences marine ecosystems in the northwestern Atlantic and transport variability of the cold Labrador Current. Understanding historic patterns of NAO variability requires long-term and high-resolution climate records that are not available from instrumental data. Here we present the first century-scale proxy record of sea surface temperature (SST) variability from the Newfoundland shelf, a region from which other annual-resolution shallow marine proxies are unavailable. The 116 year record was obtained from three sites along the eastern Newfoundland shelf using laser ablation inductively coupled mass spectrometry-determined Mg/Ca ratios in the crustose coralline alga Clathromorphum compactum. The alga is characterized by a high Mg-calcite skeleton exhibiting annual growth increments and a century-scale lifespan. Results indicate positive correlations between interannual variations in Mg/Ca ratios and both station-based and gridded instrumental SST. In addition, the record shows high spatial correlations to SST across the Newfoundland shelf and the Gulf of St. Lawrence. Before 1950 the Mg/Ca proxy record reveals significant departures from gridded temperature records. While the Newfoundland shelf is generally considered a region of negative correlations to the NAO, the algal time series as well as a recent modeling study suggest a variable negative relationship with the NAO which is strongest after similar to 1960 and before the mid-1930s.
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| 6. |
- Nygren, Michelle, et al.
(författare)
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Exploring groundwater drought responsiveness in lowland post‑glacial environments
- 2022
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Ingår i: Hydrogeology Journal. - : Springer Science and Business Media LLC. - 1431-2174 .- 1435-0157. ; 30, s. 1937-1961
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Tidskriftsartikel (refereegranskat)abstract
- Groundwater drought response to meteorological forcing depends on initial hydrological conditions. This makes it difficult to characterise groundwater droughts and identify the drought vulnerability of aquifers. The objective is to increase the understanding of groundwater memory and response to meteorological forcing in lowland post-glacial environments. Eighty-one groundwater hydrographs are analysed, using the standardised groundwater level index (SGI) and the precipitation index. Memory and response times are assessed using auto- and cross-correlation functions. Response time is estimated by comparing two approaches: (1) the traditional use of the maximum cross-correlation, and (2) the alternative use of the cross-correlation slope. Results are interpreted for different hydrogeological settings. The analysis showed that sand aquifers have the longest memory and response times, particularly in confined settings where the memory could be over 4 years. Silts and tills have relatively short memories and response times, at less than 1 year, though median values for silt are higher than for unconfined sand aquifers. In this study, estimating response time using the correlation slope is superior at capturing the initial response time of groundwater to precipitation. However, the results showed that groundwater anomalies in lowland post-glacial environments are sometimes more influenced by climate teleconnections than concurrent forcing. This emphasises the need for a holistic approach for the characterisation and projection of groundwater drought, as it develops in simultaneous response to meteorological forcing at different timescales.
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| 7. |
- Gomez-Gener, L., et al.
(författare)
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Global carbon dioxide efflux from rivers enhanced by high nocturnal emissions
- 2021
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Ingår i: Nature Geoscience. - : Springer Science and Business Media LLC. - 1752-0894 .- 1752-0908. ; 14, s. 289-294
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Tidskriftsartikel (refereegranskat)abstract
- Carbon dioxide (CO2) emissions to the atmosphere from running waters are estimated to be four times greater than the total carbon (C) flux to the oceans. However, these fluxes remain poorly constrained because of substantial spatial and temporal variability in dissolved CO2 concentrations. Using a global compilation of high-frequency CO2 measurements, we demonstrate that nocturnal CO2 emissions are on average 27% (0.9 gC m(-2) d(-1)) greater than those estimated from diurnal concentrations alone. Constraints on light availability due to canopy shading or water colour are the principal controls on observed diel (24 hour) variation, suggesting this nocturnal increase arises from daytime fixation of CO2 by photosynthesis. Because current global estimates of CO2 emissions to the atmosphere from running waters (0.65-1.8 PgC yr(-1)) rely primarily on discrete measurements of dissolved CO2 obtained during the day, they substantially underestimate the magnitude of this flux. Accounting for night-time CO2 emissions may elevate global estimates from running waters to the atmosphere by 0.20-0.55 PgC yr(-1). Failing to account for emission differences between day and night will lead to an underestimate of global CO2 emissions from rivers by up to 0.55 PgC yr(-1), according to analyses of high-frequency CO2 measurements.
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| 8. |
- Wurzbacher, Christian, 1980, et al.
(författare)
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Poorly known microbial taxa dominate the microbiome of permafrost thaw ponds.
- 2017
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Ingår i: The ISME journal. - : Springer Science and Business Media LLC. - 1751-7370 .- 1751-7362. ; 11:8, s. 1938-1941
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Tidskriftsartikel (refereegranskat)abstract
- In the transition zone of the shifting permafrost border, thaw ponds emerge as hotspots of microbial activity, processing the ancient carbon freed from the permafrost. We analyzed the microbial succession across a gradient of recently emerged to older ponds using three molecular markers: one universal, one bacterial and one fungal. Age was a major modulator of the microbial community of the thaw ponds. Surprisingly, typical freshwater taxa comprised only a small fraction of the community. Instead, thaw ponds of all age classes were dominated by enigmatic bacterial and fungal phyla. Our results on permafrost thaw ponds lead to a revised perception of the thaw pond ecosystem and their microbes, with potential implications for carbon and nutrient cycling in this increasingly important class of freshwaters.
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| 9. |
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| 10. |
- Rämö, Robert, et al.
(författare)
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Sediment Remediation Using Activated Carbon: Effects of Sorbent Particle Size and Resuspension on Sequestration of Metals and Organic Contaminants.
- 2022
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Ingår i: Environmental toxicology and chemistry. - : Wiley. - 1552-8618 .- 0730-7268. ; 41:4, s. 1096-1110
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Tidskriftsartikel (refereegranskat)abstract
- Thin-layer capping using activated carbon (AC) has been described as a cost-effective in situ sediment remediation method for organic contaminants. In this study, we compare the capping efficiency of powdered AC (PAC) against granular AC (GAC) using contaminated sediment from Oskarshamn harbor, Sweden. The effects of resuspension on contaminant retention and cap integrity were also studied. Intact sediment cores were collected from the outer harbor and brought to the laboratory. Three thin-layer caps, consisting of PAC or GAC mixed with clay, or clay only, were added to the sediment surface. Resuspension was created using a motor-driven paddle to simulate propeller wash from ship traffic. Passive samplers were placed in the sediment and in the water column to measure the sediment-to-water release of PAHs, PCBs, and metals. Our results show that a thin-layer cap with PAC reduced sediment-to-water fluxes of PCBs by 57 % under static conditions and 91 % under resuspension. Thin-layer capping with GAC was less effective than PAC, but reduced fluxes of high-molecular weight PAHs. Thin-layer capping with AC was less effective in retaining metals, except for Cd, which release was significantly reduced by PAC. Resuspension generally decreased water concentrations of dissolved cationic metals, perhaps due to sorption to suspended sediment particles. Sediment resuspension in treatments without capping increased fluxes of PCBs with log Kow > 7 and PAHs with log Kow 5 6, but resuspension reduced PCB and PAH fluxes through the PAC thin-layer cap. Overall, PAC performed better than GAC, but adverse effects on the benthic community and transport of PAC to non-target areas are drawbacks that favor the use of GAC. This article is protected by copyright. All rights reserved.© 2022 The Authors. Environmental Toxicology and Chemistry published by Wiley Periodicals LLC on behalf of SETAC.
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