Local atomic configuration approach to the nonmonotonic concentration dependence of magnetic properties of Ni(2)Mn(1+x)Z(1-x) (Z = In, Sn, Sb) Heusler alloys

• The Ni(2)Mn(1+x)Z(1-x) Heusler alloys, where Z = In, Sn, Sb are attractive candidates for shape memory applications. The effect is directly related to their magnetic properties. We have studied these systems by ab-initio calculations and experiments, focusing on magnetic moments and exchange-bias fields. The calculations indicate that the composition dependence of the total magnetic moment is due to competing ferro-magnetic and antiferromagnetic alignment between Mn atoms on different sublattices and with different local environments. This phenomenon can also explain the composition dependence of the exchange-bias effect. (C) 2020 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)

NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

Nyckelord

Heusler phases; Ferromagnetic shape memory alloy; Magnetic thin films; Magnetic structure; Ab initio calculation

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