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A-site alloying-guided universal design of noble metal-based MAX phases

Li, Youbing (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Zhu, Shuairu (författare)
Zhejiang Institute of Tianjin University, 85 Zhongguan West Road, Ningbo, 315201, Zhejiang, China
Le, Jia-Bo (författare)
Key Laboratory of Advanced Fuel Cell and Electrolyzer Technology of Zhejiang Province, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, 315201, China
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Lu, Jun (författare)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Wang, Xue (författare)
Key Laboratory of Advanced Fuel Cell and Electrolyzer Technology of Zhejiang Province, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, 315201, China
Chen, Lu (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Ding, Haoming (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Chen, Ke (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Li, Mian (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Du, Shiyu (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Wang, Hui (författare)
Zhejiang Institute of Tianjin University, 85 Zhongguan West Road, Ningbo, 315201, Zhejiang, China
Zhang, Runnan (författare)
Zhejiang Institute of Tianjin University, 85 Zhongguan West Road, Ningbo, 315201, Zhejiang, China
Persson, Per O. Å. (författare)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Hultman, Lars (författare)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Eklund, Per (författare)
Linköpings universitet,Tunnfilmsfysik,Tekniska fakulteten
Kuang, Yongbo (författare)
Key Laboratory of Advanced Fuel Cell and Electrolyzer Technology of Zhejiang Province, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, 315201, China; Center of Materials Science and Optoelectronics Engineering, University of the Chinese Academy of Sciences, 19(A) Yuquan Road, Beijing, 100049, China
Chai, Zhifang (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
Huang, Qing (författare)
Engineering Laboratory of Advanced Energy Materials, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Zhejiang, Ningbo, 315201, China; Qianwan Institute of CNiTECH, Ningbo, 315336, China
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 (creator_code:org_t)
Cell Press, 2024
2024
Engelska.
Ingår i: Matter. - : Cell Press. - 2590-2393 .- 2590-2385. ; 7:2, s. 523-538
Relaterad länk:
https://liu.diva-por... (primary) (Raw object)
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https://urn.kb.se/re...
https://doi.org/10.1...
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  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
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  • Mn+1AXn (MAX) phases have attracted significant attention due to their structural diversity and potential applications. Designing MAX phases with single-atom-thick A layers featuring 4d/5d-orbital electronic elements is interesting work. Here, we present a comprehensive report on noble metal-based M2(A1-xA′x)C (M = V, Ti, Nb; A = Al, Sn, In, Ga, Ge; A′ = Ru, Rh, Pd, Ir, Pt, Au and combinations thereof; 0 < x ≤ 0.4) phases featuring A sublayers of 4d/5d-orbital electronic elements through an A-site alloying strategy. The chemical composition of MAX phases can be adjusted by selecting different M- and A-site elements, with morphology tailored by distinct C sources. Furthermore, the V2(Sn0.8Pt0.2)C (15.7 wt % Pt) catalyst showed better performance for hydrogen evolution reaction compared to the commercial Pt/C (20 wt % Pt) electrode. This study highlights the prospects of A-site alloying for the design of novel MAX phases with unique properties and promising applications in electrocatalysis and beyond.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

Nyckelord

alloying strategy; hydrogen evolution reaction; MAP1: Discovery; MAX phases; noble metal

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