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Stable Sulfuric Vapor Transport and Liquid Sulfur Growth on Transition Metal Dichalcogenides

Chareev, Dmitriy A. (författare)
Institute of Experimental Mineralogy (IEM RAS), 142432 Chernogolovka, Moscow Region, Russia; Kazan Federal University, 18 Kremlyovskaya St., 420008 Kazan, Russia; Ural Federal University, 620002 Ekaterinburg, Russia,RAS, Inst Expt Mineral IEM, Moscow 142432, Russia.;Kazan Fed Univ, Kazan 420008, Russia.;Ural Fed Univ, Ekaterinburg 620002, Russia.
Khan, Md Ezaz Hasan (författare)
University of Doha for Science and Technology, 24449 Doha, P.O. Box 24449, Qatar,Univ Doha Sci & Technol, Doha 24449, Qatar.
Karmakar, Debjani (författare)
Uppsala universitet,Materialteori
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Nekrasov, Aleksey N. (författare)
Institute of Experimental Mineralogy (IEM RAS), 142432 Chernogolovka, Moscow Region, Russia,RAS, Inst Expt Mineral IEM, Moscow 142432, Russia.
Nickolsky, Maximilian S. (författare)
Institute of Geology of Ore Deposits (IGEM RAS), 35, Staromonetnyi per., 119017 Moscow, Russia,RAS, Inst Geol Ore Deposits IGEM, Moscow 119017, Russia.
Eriksson, Olle, 1960- (författare)
Uppsala universitet,Örebro universitet,Institutionen för naturvetenskap och teknik,Department of Physics and Astronomy, Uppsala University, Box 516, SE-75120 Uppsala, Sweden; School of Science and Technology, Örebro University, SE-701 82 Örebro, Sweden,Materialteori,Örebro Univ, Sch Sci & Technol, SE-70182 Örebro, Sweden.
Delin, Anna, 1966- (författare)
KTH,Material- och nanofysik,SeRC - Swedish e-Science Research Centre,KTH Royal Inst Technol, Dept Appl Phys, SE-10691 Stockholm, Sweden.;KTH Royal Inst Technol, Swedish Esci Res Ctr, SE-10044 Stockholm, Sweden.
Vasiliev, Alexander N. (författare)
Lomonosov Moscow State University, 119991 Moscow, Russia; National University of Science and Technology “MISiS”, 119049 Moscow, Russia,Lomonosov Moscow State Univ, Moscow 119991, Russia. Natl Univ Sci & Technol MISiS, Moscow 119049, Russia.
Abdel-Hafiez, Mahmoud (författare)
Uppsala universitet,Energimaterialens fysik,Univ Doha Sci & Technol, Doha 24449, Qatar.
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Institute of Experimental Mineralogy (IEM RAS), 142432 Chernogolovka, Moscow Region, Russia; Kazan Federal University, 18 Kremlyovskaya St, 420008 Kazan, Russia; Ural Federal University, 620002 Ekaterinburg, Russia RAS, Inst Expt Mineral IEM, Moscow 142432, Russia.;Kazan Fed Univ, Kazan 420008, Russia.;Ural Fed Univ, Ekaterinburg 620002, Russia. (creator_code:org_t)
2023-03-21
2023
Engelska.
Ingår i: Crystal Growth & Design. - : ACS Publications. - 1528-7483 .- 1528-7505. ; 23:4, s. 2287-2294
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  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
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  • Transition metal dichalcogenides (TMDs) are an emergent class of low-dimensional materials with growing applications in the field of nanoelectronics. However, efficient methods for synthesizing large monocrystals of these systems are still lacking. Here, we describe an efficient synthetic route for a large number of TMDs that were obtained in quartz glass ampoules by sulfuric vapor transport and liquid sulfur. Unlike the sublimation technique, the metal enters the gas phase in the form of molecules, hence containing a greater amount of sulfur than the growing crystal. We have investigated the physical properties for a selection of these crystals and compared them to state-of-the-art findings reported in the literature. The acquired electronic properties features demonstrate the overall high quality of single crystals grown in this work as exemplified by CoS2, ReS2, NbS2, and TaS2. This new approach to synthesize high-quality TMD single crystals can alleviate many material quality concerns and is suitable for emerging electronic devices.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

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