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Irreversible Network Transformation in a Dynamic Porous Host Catalyzed by Sulfur Dioxide
- Yang, Sihai (author)
-
- Liu, Leifeng (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Sun, Junliang (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK)
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- Thomas, K. Mark (author)
- Davies, Andrew J. (author)
- George, Michael W. (author)
- Blake, Alexander J. (author)
- Hill, Adrian H. (author)
- Fitch, Andrew N. (author)
- Tang, Chiu C. (author)
- Schroeder, Martin (author)
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- (creator_code:org_t)
- 2013-03-25
- 2013
- English.
- In: Journal of the American Chemical Society. - : American Chemical Society (ACS). - 0002-7863 .- 1520-5126. ; 135:13, s. 4954-4957
- Journal article (peer-reviewed)
Abstract
Subject headings
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- Porous NOTT-202a shows exceptionally high uptake of SO2, 13.6 mmol g(-1) (87.0 wt %) at 268 K and 1.0 bar, representing the highest value reported to date for a framework material. NOTT-202a undergoes a distinct irreversible framework phase transition upon SO2 uptake at 268-283 K to give NOTT-202b which has enhanced stability due to the formation of strong pi...pi interactions between interpenetrated networks.
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
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- ref (subject category)
- art (subject category)
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