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Voltammetric and spectroscopic characterization of early intermediates in the Co(II)-polypyridyl-catalyzed reduction of water
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- Singh, Wangkheimayum Marjit (author)
- Uppsala universitet,Molekylär biomimetik
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- Mirmohades, Mohammad (author)
- Uppsala universitet,Fysikalisk kemi
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- Jane, Reuben T. (author)
- Uppsala universitet,Molekylär biomimetik
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- Royal Society of Chemistry (RSC), 2013
- 2013
- English.
- In: Chemical Communications. - : Royal Society of Chemistry (RSC). - 1359-7345 .- 1364-548X. ; 49:77, s. 8638-8640
- Journal article (peer-reviewed)
Abstract
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- Early intermediates of catalytic water reduction by a Co(II)-polypyridyl species have been characterized. Electrochemical detection of the Co(III)-hydride and time-resolved spectroscopic detection of the Co(I)-ligand intermediates provide an understanding of their reactivity in electrolytic or light-driven reduction of protons to hydrogen.
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