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KL double core hole pre-edge states of HCl
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- Koulentianos, Dimitris, 1987 (author)
- Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, Origovagen 6B, SE-41296 Gothenburg, Sweden.;UPMC Univ Paris 06, CNRS, Sorbonne Univ, Lab Chim Phys Mat & Rayonnement,UMR 7614, F-75005 Paris 05, France.
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- Puettner, R. (author)
- Free Univ Berlin, Fachbereich Phys, Arnimallee 14, D-14195 Berlin, Germany.
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- Goldsztejn, G. (author)
- UPMC Univ Paris 06, CNRS, Sorbonne Univ, Lab Chim Phys Mat & Rayonnement,UMR 7614, F-75005 Paris 05, France.;Max Born Inst, Max Born Str 2A, D-12489 Berlin, Germany.
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- 2018
- 2018
- English.
- In: Physical Chemistry Chemical Physics. - : Royal Society of Chemistry (RSC). - 1463-9076 .- 1463-9084. ; 20:4
- Journal article (peer-reviewed)
Abstract
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- The formation of double core hole pre-edge states of the form $1s^{-1}2p^{-1}(^{1,3}\text{P})\sigmaup^*,n\ell$ for HCl, located on the binding energy scale as deep as 3 keV, has been investigated by means of a high resolution single channel electron spectroscopy technique recently developed for the hard x-ray region. A detailed spectroscopic assignment is performed based on \textit{ab initio} quantum chemical calculations and by using a sophisticated fit model comprising regular Rydberg series. Quantum defects for the different Rydberg series are extracted and the energies for the associated double core hole ionization continua are extrapolated. Dynamical information such as the lifetime width of these double-core-hole pre-edge states and the slope of the related dissociative potential energy curves are also obtained. In addition, $1s^{-1}2p^{-1}V^{-1}n\ell\lambdaup n^{\prime}\ell^{\prime}\lambdaup^{\prime}$ double shake-up transitions and double core hole states of the form $1s^{-1}2s^{-1}(^{1,3}\text{S})\sigmaup^*,4s$ are observed.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
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- Puettner, R.
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- Marchenko, T.
- Travnikova, O.
- Journel, L.
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- Guillemin, R.
- Ceolin, D.
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- Simon, M.
- Feifel, Raimund
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