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Weak Makes It Power...
Weak Makes It Powerful: The Role of Cognate Small Molecules as an Alloy Donor in 2D/1A Ternary Fullerene Solar Cells for Finely Tuned Hierarchical Morphology in Thick Active Layers
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- Fan, Qunping, 1989 (författare)
- Chalmers tekniska högskola,Chalmers University of Technology
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- Liu, Tao (författare)
- Hong Kong University of Science and Technology
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- Zhang, Ming (författare)
- Shanghai Jiao Tong University
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- Su, Wenyan (författare)
- Chalmers tekniska högskola,Chalmers University of Technology,Jinan University
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- Mendez Romero, Ulises, 1988 (författare)
- Chalmers tekniska högskola,Chalmers University of Technology
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- Yang, Tao (författare)
- Chinese Academy of Sciences
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- Geng, Xinjian (författare)
- Chalmers tekniska högskola,Chalmers University of Technology
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- Hou, Lintao (författare)
- Jinan University
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- Yu, Donghong (författare)
- Aalborg Universitet,Aalborg University
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- Liu, Feng (författare)
- Shanghai Jiao Tong University
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- Yan, He (författare)
- Hong Kong University of Science and Technology
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- Wang, Ergang, 1981 (författare)
- Chalmers tekniska högskola,Chalmers University of Technology,Zhengzhou University
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(creator_code:org_t)
- 2020-01-21
- 2020
- Engelska.
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Ingår i: Small Methods. - : Wiley. - 2366-9608. ; 4:3
- Relaterad länk:
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https://rss.onlineli...
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https://research.cha...
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https://doi.org/10.1...
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https://research.cha...
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Abstract
Ämnesord
Stäng
- Herein, a novel small molecule donor is first developed, FSM6, which is a cognate molecule to BTR possessing similar molecular structure with comparable optical absorption but different crystallinity. The efficient fullerene-type ternary small molecular solar cells (SMSCs) based on an alloy donor of BTR and FSM6 in a thick film of 250 nm reveal the improved hierarchical phase separation morphology and molecular structural order of ternary active layers with improved crystallinity of the key donor component BTR. Furthermore, FSM6 as the key third component also plays a role of charge transfer accelerator in ternary SMSCs. As a result, the optimal ternary SMSCs based on BTR:FSM6:PC71BM achieve a high power conversion efficiency (PCE) up to 10.21% with the synergistically improved open-circuit voltage of 0.950 V, short-circuit current density of 13.85 mA cm(-2), and fill factor of 77.6%, in comparison with either the binary SMSCs of BTR:PC71BM (PCE = 9.37%) or FSM6:PC71BM (PCE = 8.00%). This work provides a promising methodology to optimize device morphology for high-performance ternary SMSCs by combining two cognate small molecules with similar absorption spectra but different crystallinity as an alloy donor.
Ämnesord
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
- NATURVETENSKAP -- Kemi -- Annan kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Other Chemistry Topics (hsv//eng)
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
Nyckelord
- morphology optimization
- ternary small molecule solar cells
- thick films
- alloy donors
Publikations- och innehållstyp
- art (ämneskategori)
- ref (ämneskategori)
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Till lärosätets databas
- Av författaren/redakt...
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Fan, Qunping, 19 ...
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Liu, Tao
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Zhang, Ming
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Su, Wenyan
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Mendez Romero, U ...
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Yang, Tao
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visa fler...
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Geng, Xinjian
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Hou, Lintao
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Yu, Donghong
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Liu, Feng
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Yan, He
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Wang, Ergang, 19 ...
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visa färre...
- Om ämnet
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- NATURVETENSKAP
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NATURVETENSKAP
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och Kemi
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och Materialkemi
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- NATURVETENSKAP
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NATURVETENSKAP
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och Kemi
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och Annan kemi
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- NATURVETENSKAP
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NATURVETENSKAP
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och Fysik
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och Den kondenserade ...
- Artiklar i publikationen
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Small Methods
- Av lärosätet
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Chalmers tekniska högskola