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Sökning: WFRF:(Åström E)

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1.
  • Lichtenberg, Elinor M., et al. (författare)
  • A global synthesis of the effects of diversified farming systems on arthropod diversity within fields and across agricultural landscapes
  • 2017
  • Ingår i: Global Change Biology. - : Wiley. - 1354-1013 .- 1365-2486. ; 23:11, s. 4946-4957
  • Tidskriftsartikel (refereegranskat)abstract
    • Agricultural intensification is a leading cause of global biodiversity loss, which can reduce the provisioning of ecosystem services in managed ecosystems. Organic farming and plant diversification are farm management schemes that may mitigate potential ecological harm by increasing species richness and boosting related ecosystem services to agroecosystems. What remains unclear is the extent to which farm management schemes affect biodiversity components other than species richness, and whether impacts differ across spatial scales and landscape contexts. Using a global metadataset, we quantified the effects of organic farming and plant diversification on abundance, local diversity (communities within fields), and regional diversity (communities across fields) of arthropod pollinators, predators, herbivores, and detritivores. Both organic farming and higher in-field plant diversity enhanced arthropod abundance, particularly for rare taxa. This resulted in increased richness but decreased evenness. While these responses were stronger at local relative to regional scales, richness and abundance increased at both scales, and richness on farms embedded in complex relative to simple landscapes. Overall, both organic farming and in-field plant diversification exerted the strongest effects on pollinators and predators, suggesting these management schemes can facilitate ecosystem service providers without augmenting herbivore (pest) populations. Our results suggest that organic farming and plant diversification promote diverse arthropod metacommunities that may provide temporal and spatial stability of ecosystem service provisioning. Conserving diverse plant and arthropod communities in farming systems therefore requires sustainable practices that operate both within fields and across landscapes.
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2.
  • Vicedo-Cabrera, A.M., et al. (författare)
  • The burden of heat-related mortality attributable to recent human-induced climate change
  • 2021
  • Ingår i: Nature Climate Change. - : Nature Publishing Group. - 1758-678X .- 1758-6798. ; 11:6, s. 492-500
  • Tidskriftsartikel (refereegranskat)abstract
    • Climate change affects human health; however, there have been no large-scale, systematic efforts to quantify the heat-related human health impacts that have already occurred due to climate change. Here, we use empirical data from 732 locations in 43 countries to estimate the mortality burdens associated with the additional heat exposure that has resulted from recent human-induced warming, during the period 1991–2018. Across all study countries, we find that 37.0% (range 20.5–76.3%) of warm-season heat-related deaths can be attributed to anthropogenic climate change and that increased mortality is evident on every continent. Burdens varied geographically but were of the order of dozens to hundreds of deaths per year in many locations. Our findings support the urgent need for more ambitious mitigation and adaptation strategies to minimize the public health impacts of climate change.
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3.
  • Yu, Changxun, et al. (författare)
  • Iron behavior in a northern estuary: Large pools of non-sulfidized Fe(II) associated with organic matter
  • 2015
  • Ingår i: Chemical Geology. - : Elsevier BV. - 0009-2541 .- 1872-6836. ; 413, s. 73-85
  • Tidskriftsartikel (refereegranskat)abstract
    • The estuaries of the Northern Baltic Sea (Gulf of Bothnia) receive an abundance of diagenetically reactive catchment-derived Fe, which is to a large degree complexed with organicmatter or present as Fe (hydr-) oxides. However, our understanding of sedimentary Fe diagenesis in these estuaries is limited. To address this limitation, the present study examines Fe geochemistry in a 3.5-m-thick estuarine benthic mud layer and three samples of suspended particulate matter of a catchment on the eastern Gulf of Bothnia. The age-depth model of the mud, constructed on the basis of sedimentary features as well as Cs-137 and aquatic plant C-14 determinations, revealed a high average rate of sedimentation (5 cm . yr(-1)) for the upper mud unit (0-182.5 cm, corresponding to 1973-2011), in response to intensive land-use (ditching) in the catchment since the 1960s and 1970s. The intensive land-use has resulted in a strong increase in the Fe accumulation rates, but has not caused a recognizable impact on the diagenetic processes of Fe including features such as degree of sulfidization and solid-phase partitioning. Iron X-ray absorption spectroscopy (XAS) indicated that in the suspended particulate matter, large proportions (47-58%) of Fe occur as Fe(III)-organic complexes and 2-line ferrihydrite. In the mud, the former is completely reduced, and reactive Fe (defined via extraction with 1 MHCl) was high throughout (52-68%, median = 61%) and strongly dominated by Fe(II). This reactive Fe(II) pool was sulfidized to only a limited extent (degree of reactive sulfidization = 11-26%, median = 17%). This phenomenon is attributed to the brackish-water conditions (i.e. low in sulfate) and the abundant input of reactive Fe(III) from the catchment, leading to a surplus of dissolved Fe2+ over dissolved sulfide in the sediment. The low availability of dissolved sulfide, in combination with the high average sedimentation rate, limits the formation of intermediate reduced sulfur compounds at the water-sediment interface, thereby retarding the conversion of FeS into pyrite (ratios of pyrite-S to AVS = 0.17-1.73, median = 0.37; degree of pyritization = 1-17%, median = 3%). Iron XAS, in combination with wavelet transform analysis, of representative sediment segments from the upper and lower mud units suggests that the non-sulfidized Fe(II) pool is dominantly complexed by organic matter, with the remaining Fe(II) occurring as mackinawite. This has implications for the understanding of early Fe diagenesis in settings with a high input of organic matter and relatively low supply of sulfate. (C) 2015 Elsevier B.V. All rights reserved.
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4.
  • Yu, Changxun, et al. (författare)
  • Manganese accumulation and solid-phase speciation in a 3.5 m thick mud sequence from the estuary of an acidic and Mn-rich creek, northern Baltic Sea
  • 2016
  • Ingår i: Chemical Geology. - : Elsevier BV. - 0009-2541 .- 1872-6836. ; 437, s. 56-66
  • Tidskriftsartikel (refereegranskat)abstract
    • In sediments, manganese (Mn) is typically enriched in the form of authigenic Mn hydroxides at the water-sediment interface where intensive redox cycling of Mn occurs. Here we show, based on existing hydrochemical and geochemical (sediment core) data and new detailed chemical and mineralogical characterization of a 3.5 m long sediment core from a Boreal estuary, that the behavior of Mn can be profoundly different and more complex in estuarine settings receiving an abundance of terrestrial Mn. The most notable feature in the 3.5 m long sediment core is two depth intervals (60-155 cm and 181-230 cm) where there are strong fine-scale variations in Mn concentrations with peaks episodically reaching up to 10-25 g kg(-1) and 6.7-12 g kg(-1), respectively. X-ray absorption spectroscopy and sequential chemical extraction show that Mn occurs mainly as authigenic rhodochrosite at these two depth intervals and is mainly surface-sorbed in other sections with relatively low and stable Mn concentrations. The data suggests that the strong fine-scale variations in Mn concentrations are a reflection of the extent of formation and settling of Mn hydroxides, the precursors of the authigenic rhodochrosite (and also of the surface-sorbed Mn), rather than Mn input to the estuary or redox-related Mn translocation within the sediment. There was agreement between the results of linear combination fitting of extended X-ray absorption fine structure data and a 7-step sequential chemical extraction (SCE) in terms of quantification of surface-sorbed Mn species, whereas the SCE experiment failed to fractionate a majority of rhodochrosite into SCE step-2 (1M NH4-acetate at pH 6), which is frequently employed to dissolve carbonate. We ascribe this discrepancy to only partial dissolution of rhodochrosite in the weakly acidic (pH = 6) NH4-acetate leach.
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5.
  • Åström, E., et al. (författare)
  • Precision measurements of linear scattering density using muon tomography
  • 2016
  • Ingår i: Journal of Instrumentation. - : Institute of Physics Publishing. - 1748-0221. ; 11:7
  • Tidskriftsartikel (refereegranskat)abstract
    • We demonstrate that muon tomography can be used to precisely measure the properties of various materials. The materials which have been considered have been extracted from an experimental blast furnace, including carbon (coke) and iron oxides, for which measurements of the linear scattering density relative to the mass density have been performed with an absolute precision of 10%. We report the procedures that are used in order to obtain such precision, and a discussion is presented to address the expected performance of the technique when applied to heavier materials. The results we obtain do not depend on the specific type of material considered and therefore they can be extended to any application.
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6.
  • Åström, Mats E., 1963-, et al. (författare)
  • Extensive accumulation of rare earth elements in estuarine sediments affected by leaching of acid sulfate soils
  • 2020
  • Ingår i: Boreal Environment Research. - : Finnish Environmental Inst. - 1239-6095 .- 1797-2469. ; 25, s. 105-120
  • Tidskriftsartikel (refereegranskat)abstract
    • The concentrations, loads and speciation of rare earth elements (REEs) were studied in a 3.5 m thick mud depositional succession from an estuary in the Gulf of Bothnia. The uppermost 182.5 cm of the mud, estimated to have deposited from the early 1970s to 2011 (sampling year), had very high REE concentrations (596-1456 ppm) and accumulation rates (5.2-28 g m(-2) year(-1)). This was explained by large REE export from acid sulfate soils after they became efficiently drained with modern drainage techniques. Geochemical and synchrotron-based spectroscopic (XANES) analyses showed that the REEs in the mud are relatively firmly bound in non-clastic phases, likely adsorbed by clay minerals and also to some extent by iron oxyhydroxides. Below 182.5 cm, the REE concentrations successively decreased down to background values at the base at 3.5 m, reflecting less efficient drainage and leaching of the acid sulfate soils in previous decades and centuries.
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9.
  • Drake, Henrik, et al. (författare)
  • Variability of sulphur isotope ratios in pyrite and dissolved sulphate in granitoid fractures down to 1km depth - Evidence for widespread activity of sulphur reducing bacteria
  • 2013
  • Ingår i: Geochimica et Cosmochimica Acta. - : Elsevier BV. - 0016-7037 .- 1872-9533. ; 102, s. 143-161
  • Tidskriftsartikel (refereegranskat)abstract
    • Euhedral pyrite crystals in 46 open bedrock (granitoid) fractures at depths down to nearly 1 km were analysed for sulphur isotope ratios (delta S-34) by the in situ secondary ion mass spectrometry (SIMS) technique and by conventional bulk-grain analysis, and were compared with groundwater data. Twenty nine of the fractures sampled for pyrite had corresponding data for groundwater, including chemistry and isotopic ratios of sulphate, which provided a unique opportunity to compare the sulphur-isotopic ratios of pyrite and dissolved sulphate both at site and fracture-specific scales. Assessment of pyrite age and formation conditions were based on the geological evolution of the area (Laxemar, SE Sweden), and on data on co-genetic calcite as follows: (1) the isotopic ratios of the calcite crystals (delta O-18, delta C-13, Sr-87/Sr-86) were compared with previously defined isotopic features of fracture mineral assemblages precipitated during various geological periods, and (2) the delta O-18 of the calcites were compared with the delta O-18 of groundwater in fractures corresponding to those where the calcite/pyrite assemblages were sampled. Taken together, the data show that all the sampled fractures carried pyrite/calcite that are low-temperature and precipitated from the current groundwater or similar pre-existing groundwater, except at depths of -300 to -600 m where water with a glacial component dominates and the crystals are from pre-modern fluids. An age of <10 Ma are anticipated for the pre-modern fluids. The delta S-34(pyr) showed huge variations across individual crystals (such as -32 to +73 parts per thousand) and extreme minimum (-50 parts per thousand) and maximum (+91 parts per thousand) values. For this kind of extreme S-isotopic variation at earth-surface conditions there is no other explanation than activity of sulphur reducing bacteria coupled with sulphate-limited conditions. Indeed, the most common subgrain feature was an increase in delta S-34(pyr) values from interior to rim of the crystal, which we interpret are related to successively higher delta S-34 values of the dissolved source SO42- caused by ongoing bacterial sulphate reduction in fractures with low-flow or stagnant waters. The measured groundwater had delta S-34(SO4) values of +9 parts per thousand to +37 parts per thousand, with the highest values associated with low sulphate concentrations. These values are overall, and especially in the sulphate-poor waters down to -400 m, somewhat higher than the anticipated initial values, and can thus, like for the S-34-enriched pyrites, be explained by a Rayleigh distillation process driven by microbial sulphate reduction. An intriguing feature was that the delta S-34(SO4) values of the groundwater were in no case reaching up to the values required to produce biogenic pyrite with delta S-34 values of +40 parts per thousand to +91 parts per thousand. To explain this feature, we suggest that groundwater in low-flow fractures with near-stagnant water (carrying sulphate and pyrite with high delta S-34) is masked by high-flow parts of the fracture system carrying groundwater that often contains sulphate in abundance and considerably less fractionated with respect to S-34 and S-32. In order to gain detailed knowledge of chemical processes and patterns in groundwater in fractured rock, fracture-mineral investigations are a powerful tool, as we have shown here for the sulphur system. (C) 2012 Elsevier Ltd. All rights reserved.
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