| 1. |
- Martinelli, L., et al.
(författare)
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Collective Nature of Orbital Excitations in Layered Cuprates in the Absence of Apical Oxygens
- 2024
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Ingår i: Physical Review Letters. - 1079-7114 .- 0031-9007. ; 132:6
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Tidskriftsartikel (refereegranskat)abstract
- We have investigated the 3d orbital excitations in CaCuO2 (CCO), Nd2CuO4 (NCO), and La2CuO4 (LCO) using high-resolution resonant inelastic x-ray scattering. In LCO they behave as well-localized excitations, similarly to several other cuprates. On the contrary, in CCO and NCO the dxy orbital clearly disperses, pointing to a collective character of this excitation (orbiton) in compounds without apical oxygen. We ascribe the origin of the dispersion as stemming from a substantial next-nearest-neighbor (NNN) orbital superexchange. Such an exchange leads to the liberation of the orbiton from its coupling to magnons, which is associated with the orbiton hopping between nearest neighbor copper sites. Finally, we show that the exceptionally large NNN orbital superexchange can be traced back to the absence of apical oxygens suppressing the charge transfer energy.
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| 2. |
- Pelliciari, Jonathan, et al.
(författare)
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Evolution of spin excitations from bulk to monolayer FeSe
- 2021
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Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723 .- 2041-1723. ; 12:1
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Tidskriftsartikel (refereegranskat)abstract
- In ultrathin films of FeSe grown on SrTiO (FeSe/STO), the superconducting transition temperature T is increased by almost an order of magnitude, raising questions on the pairing mechanism. As in other superconductors, antiferromagnetic spin fluctuations have been proposed to mediate SC making it essential to study the evolution of the spin dynamics of FeSe from the bulk to the ultrathin limit. Here, we investigate the spin excitations in bulk and monolayer FeSe/STO using resonant inelastic x-ray scattering (RIXS) and quantum Monte Carlo (QMC) calculations. Despite the absence of long-range magnetic order, bulk FeSe displays dispersive magnetic excitations reminiscent of other Fe-pnictides. Conversely, the spin excitations in FeSe/STO are gapped, dispersionless, and significantly hardened relative to its bulk counterpart. By comparing our RIXS results with simulations of a bilayer Hubbard model, we connect the evolution of the spin excitations to the Fermiology of the two systems revealing a remarkable reconfiguration of spin excitations in FeSe/STO, essential to understand the role of spin fluctuations in the pairing mechanism.
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| 3. |
- Andersson, Eric, 1992, et al.
(författare)
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Fabrication and electrical transport characterization of high quality underdoped YBa2Cu3O7-δ nanowires
- 2020
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Ingår i: Superconductor Science and Technology. - : IOP Publishing. - 0953-2048 .- 1361-6668. ; 33:6
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Tidskriftsartikel (refereegranskat)abstract
- We present the fabrication and electrical transport characterization of underdoped YBa2Cu3O7-δnanowires. The nanowires have been realized without any protective capping layer and theyshow transport properties similar to those of the parent thin film, demonstrating that they havenot been damaged by the nanopatterning. The current-voltage characteristics of the underdopednanowires show large hysteretic voltage switching at the critical current, in contrast to theflux-flow like characteristics of optimally doped nanostructures, indicating the formation of aself-stabilizing hot spot. These results open up new possibilities for using the underdopednanowires as single photon detectors and for exploring the underdoped side of the YBa2Cu3O7-δphase diagram at the nanoscale.
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| 4. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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Charge order at high temperature in cuprate superconductors
- 2021
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Ingår i: Journal of the Physical Society of Japan. - 1347-4073 .- 0031-9015. ; 90:11
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Forskningsöversikt (refereegranskat)abstract
- The presence of different electronic orders other than superconductivity populating the phase diagram of cuprates suggests that they might be the key to disclose the mysteries of this class of materials. In particular charge order in the form of charge density waves (CDW), i.e., the incommensurate modulation of electron density in the CuO2 planes, is ubiquitous across different families and presents a clear interplay with superconductivity. Until recently, CDW had been found to be confined inside a rather small region of the phase diagram, below the pseudogap temperature and the optimal doping. This occurrence might shed doubts on the possibility that such “low temperature phenomenon” actually rules the properties of cuprates either in the normal or in the superconducting states. However, recent resonant X-ray scattering (RXS) experiments are overturning this paradigm. It results that very short-ranged charge modulations permeate a much wider region of the phase diagram, coexisting with CDW at lower temperatures and persisting up to temperatures well above the pseudogap opening. Here we review the characteristics of these high temperature charge modulations, which are present in several cuprate families, with similarities and differences. A particular emphasis is put on their dynamical character and on their coupling to lattice and magnetic excitations, properties that can be determined with high resolution resonant inelastic x-ray scattering (RIXS).
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| 5. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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Dynamical charge density fluctuations pervading the phase diagram of a Cu-based high-Tc superconductor
- 2019
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Ingår i: Science. - : American Association for the Advancement of Science (AAAS). - 0036-8075 .- 1095-9203. ; 365:6456, s. 906-910
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Tidskriftsartikel (refereegranskat)abstract
- Charge density modulations have been observed in all families of high–critical temperature (Tc) superconducting cuprates. Although they are consistently found in the underdoped region of the phase diagram and at relatively low temperatures, it is still unclear to what extent they influence the unusual properties of these systems. Using resonant x-ray scattering, we carefully determined the temperature dependence of charge density modulations in YBa2Cu3O7–d and Nd1+xBa2–xCu3O7–d for several doping levels. We isolated short-range dynamical charge density fluctuations in addition to the previously known quasi-critical charge density waves. They persist up to well above the pseudogap temperature T*, are characterized by energies of a few milli–electron volts, and pervade a large area of the phase diagram.
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| 6. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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Engineering underdoped CuO2 nanoribbons in nm-thick a -axis YBa2Cu3 O7-δ films
- 2024
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Ingår i: Physical Review Materials. - 2475-9953. ; 8:4
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Tidskriftsartikel (refereegranskat)abstract
- In underdoped cuprate high-Tc superconductors, various local orders and symmetry-breaking states, in addition to superconductivity, reside in the CuO2 planes. The confinement of the CuO2 planes can therefore play a fundamental role in modifying the hierarchy between the various orders and their intertwining with superconductivity. Here we present the growth of a-axis oriented YBa2Cu3O7-δ films, spanning the whole underdoped side of the phase diagram. In these samples, the CuO2 planes are confined by the film thickness, effectively forming unit-cell-thick nanoribbons. The unidirectional confinement at the nanoscale enhances the in-plane anisotropy of the films. By x-ray diffraction and resistance vs temperature measurements, we have discovered the suppression of the orthorhombic-to-tetragonal transition at low dopings, and a very high anisotropy of the normal state resistance in the b-c plane, the latter being connected to a weak coupling between adjacent CuO2 nanoribbons. These findings show that the samples we have grown represent a novel system, different from the bulk, where future experiments can possibly shed light on the rich and mysterious physics occurring within the CuO2 planes.
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| 7. |
- Arpaia, Riccardo, 1985, et al.
(författare)
-
Engineering underdoped CuO2 nanoribbons in nm-thick a -axis YBa2Cu3 O7-δ films
- 2024
-
Ingår i: Physical Review Materials. - : American Physical Society. - 2475-9953. ; 8:4
-
Tidskriftsartikel (refereegranskat)abstract
- In underdoped cuprate high-Tc superconductors, various local orders and symmetry-breaking states, in addition to superconductivity, reside in the CuO2 planes. The confinement of the CuO2 planes can therefore play a fundamental role in modifying the hierarchy between the various orders and their intertwining with superconductivity. Here we present the growth of a-axis oriented YBa2Cu3O7-δ films, spanning the whole underdoped side of the phase diagram. In these samples, the CuO2 planes are confined by the film thickness, effectively forming unit-cell-thick nanoribbons. The unidirectional confinement at the nanoscale enhances the in-plane anisotropy of the films. By x-ray diffraction and resistance vs temperature measurements, we have discovered the suppression of the orthorhombic-to-tetragonal transition at low dopings, and a very high anisotropy of the normal state resistance in the b-c plane, the latter being connected to a weak coupling between adjacent CuO2 nanoribbons. These findings show that the samples we have grown represent a novel system, different from the bulk, where future experiments can possibly shed light on the rich and mysterious physics occurring within the CuO2 planes.
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| 8. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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High-temperature superconducting nanowires for photon detection
- 2015
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Ingår i: Physica C: Superconductivity and its Applications. - : Elsevier BV. - 0921-4534. ; 509, s. 16-21
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Tidskriftsartikel (refereegranskat)abstract
- The possible use of high-temperature superconductors (HTS) for realizing superconducting nanowire single-photon detectors is a challenging, but also promising, aim because of their ultrafast electron relaxation times and high operating temperatures. The state-of-the-art HTS nanowires with a 50-nm thickness and widths down to 130 nm have been fabricated and tested under a 1550-nm wavelength laser irradiation. Experimental results presenting both the amplitude and rise times of the photoresponse signals as a function of the normalized detector bias current, measured in a wide temperature range, are discussed. The presence of two distinct regimes in the photoresponse temperature dependence is clearly evidenced, indicating that there are two different response mechanisms responsible for the HTS photoresponse mechanisms.
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| 9. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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Highly homogeneous YBCO/LSMO nanowires for photoresponse experiments
- 2014
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Ingår i: Superconductor Science and Technology. - : IOP Publishing. - 0953-2048 .- 1361-6668. ; 27:4
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Tidskriftsartikel (refereegranskat)abstract
- By using nanolithography and a soft etching procedure, we have realized YBa2Cu3O7-x/La0.7Sr0.3MnO3 (YBCO/LSMO) nanowires, with cross sections down to 100 x 50 nm(2) that ensure the cover age of areas up to 10 x 30 mu m(2). The LSMO layer acts as a capping for YBCO, minimizing the degradation of the superconducting properties taking place during the patterning; moreover, as a ferromagnetic manganite, it is expected to accelerate the relaxation dynamics of quasiparticles in YBCO, making such a system potentially attractive for applications in superconducting ultrafast optoelectronics. The reproducibility of the values of the critical current densities measured in different devices with the same geometry makes our nanowires ideal candidates for photoresponse experiments. First measurements have shown a satisfactory photoresponse from YBCO/LSMO devices.
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| 10. |
- Arpaia, Riccardo, 1985, et al.
(författare)
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Improved Nanopatterning for YBCO Nanowires Approaching the Depairing Current
- 2013
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Ingår i: IEEE Transactions on Applied Superconductivity. - : Institute of Electrical and Electronics Engineers (IEEE). - 1558-2515 .- 1051-8223. ; 23:3
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Tidskriftsartikel (refereegranskat)abstract
- An improved nanopatterning procedure has been developed to obtain YBa2Cu3O7-x nanowires with cross-sections as small as 50 x 50 nm(2), protected by an Au capping layer. To probe the effective role of the Au protecting layer, we have measured the current-voltage characteristics and the resistive transition in temperature of the nanowires. Critical current densities up to 108 A/cm(2) have been achieved at T = 4.2 K, approaching the theoretical depairing current limit. The resistance, measured as a function of temperature close to T-c, has been fitted with a thermal activated phase slip model, including the effect of the gold layer. The extracted values of the superconducting coherence length and of the London penetration depth give current densities consistent with the measured ones. These results cannot be achieved with nanowires without the Au capping layer.
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