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1.
  • Monti, Damien, et al. (författare)
  • Multivalent Batteries-Prospects for High Energy Density: Ca Batteries
  • 2019
  • Ingår i: Frontiers in Chemistry. - : Frontiers Media SA. - 2296-2646. ; 7:FEB
  • Tidskriftsartikel (refereegranskat)abstract
    • Batteries based on Ca hold the promise to leapfrog ahead regarding increases in energy densities and are especially attractive as Ca is the 5th most abundant element in the Earth's crust. The viability of Ca metal anodes has recently been shown by approaches that either use wide potential window electrolytes at moderately elevated temperatures or THE-based electrolytes at room temperature. This paper provides realistic estimates of the practical energy densities for Ca-based rechargeable batteries at the cell level, calculated using open source models for several concepts. The results from the Ca metal anode batteries indicate that doubled or even tripled energy density as compared to the state-of-the-art Li-ion batteries is viable if a practical proof-of-concept can be achieved.
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2.
  • Younesi, Reza, et al. (författare)
  • Electrochemical performance and interfacial properties of Li-metal in lithium bis(fluorosulfonyl)imide based electrolytes
  • 2017
  • Ingår i: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322. ; 7
  • Tidskriftsartikel (refereegranskat)abstract
    • Successful usage of lithium metal as the negative electrode or anode in rechargeable batteries can be an important step to increase the energy density of lithium batteries. Performance of lithium metal in a relatively promising electrolyte solution composed of lithium bis( uorosulfonyl)imide (LiN(SO2F)2; LiFSI) salt dissolved in 1,2-dimethoxyethane (DME) is here studied. The in uence of the concentration of the electrolyte salt −1 M or 4 M LiFSI- is investigated by varying important electrochemical parameters such as applied current density and plating capacity. X-ray photoelectron spectroscopy analysis as a surface sensitive technique is here used to analyze that how the composition of the solid electrolyte interphase varies with the salt concentration and with the number of cycles.
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