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1.
  • Barnasas, A., et al. (författare)
  • Quantum confinement effects of thin ZnO films by experiment and theory
  • 2020
  • Ingår i: Physica. E, Low-Dimensional systems and nanostructures. - : ELSEVIER. - 1386-9477 .- 1873-1759. ; 120
  • Tidskriftsartikel (refereegranskat)abstract
    • Thin ZnO films with thickness ranging between 2 and 300 nm have been grown on quartz, Corning glass and Si (100) substrates by radio frequency magnetron sputtering. The film thickness was determined by pre-calibrated quartz balance with the help of x-ray reflectivity measurements. X-ray diffraction experiments revealed the formation of highly-textured hexagonal ZnO. Ultraviolet-visible light absorption spectroscopy has shown a "blue shift" of the direct band gap of ZnO. The experimental results are interpreted as evidences of quantum confinement effects. This is supported by theoretical predictions of the optical gap, which was calculated in the framework of effective mass approximation by solving the two particle (electron and hole) Hartree-Fock equations. The observed fair agreement between theoretical and experimental results corroborates the quantum confinement interpretation.
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2.
  • Poulopoulos, Panagiotis, et al. (författare)
  • Intense Quantum Confinement Effects in Cu(2)O Thin Films
  • 2011
  • Ingår i: The Journal of Physical Chemistry C. - : American Chemical Society (ACS). - 1932-7447 .- 1932-7455. ; 115:30, s. 14839-14843
  • Tidskriftsartikel (refereegranskat)abstract
    • Thin Cu(2)O films in the thickness range 0.75-230 nm have been prepared on high-quality corning glass, quartz, and Si(100) substrates by radio frequency magnetron sputtering of Cu targets and subsequent oxidation in a furnace under air. Ultraviolet-visible light absorption spectroscopy experiments reveal a blue shift of the energy between the top valence and the first excited conduction sub-bands. The shift increases smoothly as the film thickness decreases. The maximum value observed for the thinnest film is very large, reaching a value of 1.2 eV. Such a shift was not easy to be observed in the past due to the very small Bohr radius of Cu(2)O. The experimental results, which indicate the presence of intense quantum confinement effects, are well-described by theoretical calculations based on the potential morphing method in the Hartree-Fock approximation.
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