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- Algaba, Juan-Carlos, et al.
(författare)
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Broadband Multi-wavelength Properties of M87 during the 2017 Event Horizon Telescope Campaign
- 2021
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Ingår i: Astrophysical Journal Letters. - : American Astronomical Society. - 2041-8213 .- 2041-8205. ; 911:1
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Forskningsöversikt (refereegranskat)abstract
- In 2017, the Event Horizon Telescope (EHT) Collaboration succeeded in capturing the first direct image of the center of the M87 galaxy. The asymmetric ring morphology and size are consistent with theoretical expectations for a weakly accreting supermassive black hole of mass ∼6.5 × 109 M o˙. The EHTC also partnered with several international facilities in space and on the ground, to arrange an extensive, quasi-simultaneous multi-wavelength campaign. This Letter presents the results and analysis of this campaign, as well as the multi-wavelength data as a legacy data repository. We captured M87 in a historically low state, and the core flux dominates over HST-1 at high energies, making it possible to combine core flux constraints with the more spatially precise very long baseline interferometry data. We present the most complete simultaneous multi-wavelength spectrum of the active nucleus to date, and discuss the complexity and caveats of combining data from different spatial scales into one broadband spectrum. We apply two heuristic, isotropic leptonic single-zone models to provide insight into the basic source properties, but conclude that a structured jet is necessary to explain M87's spectrum. We can exclude that the simultaneous γ-ray emission is produced via inverse Compton emission in the same region producing the EHT mm-band emission, and further conclude that the γ-rays can only be produced in the inner jets (inward of HST-1) if there are strongly particle-dominated regions. Direct synchrotron emission from accelerated protons and secondaries cannot yet be excluded.
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- Chawla, Amit Kumar, et al.
(författare)
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Study of composition dependent structural, optical, and magnetic properties of Cu-doped Zn1-xCdxS nanoparticles
- 2010
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Ingår i: Journal of Applied Physics. - : AIP Publishing. - 0021-8979 .- 1089-7550. ; 108:12, s. 123519-
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Tidskriftsartikel (refereegranskat)abstract
- Cu-doped Zn1-xCdxS nanoparticles were synthesized by coprecipitation technique in ice bath at 280 K. The band gap energy of Zn1-xCdxS:Cu nanoparticles can be tuned to a lower energy by increasing the Cd content, indicating the formation of the alloyed nanoparticles. The alloy structure is further supported by the systematic shifting of characteristic x-ray diffraction peaks to lower angles with increase in Cd content. Systematic copper doping induces a red shift in the energy band gap of Zn0.9Cd0.1S:Cu nanoparticles with increase in copper concentration. Cu-doped Zn0.9Cd0.1S nanoparticles were found to have ferromagnetic nature at 5 K whereas undoped particles were found to be diamagnetic. Green luminescence further proves proper doping of Cu into the ZnCdS matrix. It is believed that the green luminescence originates from the recombination between the shallow donor level (sulfur vacancy) and the t(2) level of Cu2+. This method provides an inexpensive and simple procedure to produce ternary ZnCdS: Cu nanoparticles with tunable optical properties via changing Cd and/or Cu concentrations.
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- De Adhikari, Amrita, et al.
(författare)
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Polyaniline-Stabilized Intertwined Network-like Ferrocene/Graphene Nanoarchitecture for Supercapacitor Application
- 2017
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Ingår i: Chemistry - An Asian Journal. - : WILEY-V C H VERLAG GMBH. - 1861-4728 .- 1861-471X. ; 12:8, s. 900-909
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Tidskriftsartikel (refereegranskat)abstract
- The present work highlights the effective H-p interaction between metallocenes ( ferrocene; Fc) and graphene and their stabilization in the presence of polyaniline ( PANI) through pi-pi interactions. The PANI-stabilized Fc@ graphene nanocomposite ( FcGA) resembled an intertwined network-like morphology with high surface area and porosity, which could make it a potential candidate for energy-storage applications. The relative interactions between the components were assessed through theoretical ( DFT) calculations. The specific capacitance calculated from galvanostatic charging/discharging indicated that the PANI-stabilized ter-nary nanocomposite exhibited a maximum specific capacitance of 960 Fg(-) at an energy density of 85 WhKg(-1) and a current density of 1 Ag-. Furthermore, electrochemical impedance spectroscopy (EIS) analysis confirmed the low internal resistance of the as-prepared nanocomposites, which showed improved charge-transfer properties of graphene after incorporation of Fc and stabilization with PANI. Additionally, all electrodes were found to be stable up to 5000 cycles with a specific capacitance retention of 86%, thus demonstrating the good reversibility and durability of the electrode material.
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- Konwar, Lakhya Jyoti, et al.
(författare)
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Shape selectivity and acidity effects in glycerol acetylation with acetic anhydride : selective synthesis of triacetin over Y-zeolite and sulfonated mesoporous carbons
- 2015
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Ingår i: Journal of Catalysis. - : Elsevier. - 0021-9517 .- 1090-2694. ; 329, s. 237-247
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Tidskriftsartikel (refereegranskat)abstract
- Abstract 100% triacetin selectivity was achieved in glycerol acetylation with acetic anhydride in 20–50 min in the presence of catalytic amounts of mesoporous sulfonated carbons and zeolite H-Y. Experimental results obtained over a range of solid acids with varying structure and acidic properties indicate that selectivity to triacetin was influenced mainly by the pore structure and catalyst surface acid site density. The shape selectivity effect over microporous zeolites was verified from the molecular dimensions of glycerol, monoacetin, diacetin and triacetin obtained from DFT calculations; on the contrary in mesoporous catalyst surface acid site density was responsible for determining triacetin selectivity.
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- Li, Shujun, et al.
(författare)
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A representative volume element based on translational symmetries for FE analysis of cracked laminates with two arrays of cracks
- 2009
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Ingår i: International Journal of Solids and Structures. - : Elsevier BV. - 0020-7683 .- 1879-2146. ; 46:7-8, s. 1793-1804
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Tidskriftsartikel (refereegranskat)abstract
- A methodology is proposed for the construction of a representative volume element (RVE) for analysis of laminated composites containing two arrays of ply cracks running in different directions. The only requirement is that the cracks in any ply are uniformly spaced, and if more than one ply of a given orientation is cracked, then the crack spacing of individual plies must only be in exact multiples of each other. The spacing of cracks in the two directions can be fully independent. The RVE is constructed through a systematic consideration of translational symmetries present in the cracked laminate. As a result, the boundary conditions on the RVE can be imposed without compromising accuracy. Examples of the application of the RVE methodology are given to illustrate its broad capability and a finite element (FE) stress analysis is performed for these cases to illustrate results such as the crack surface displacements, local stress fields and RVE-averaged elastic properties. For one case, the average properties are compared with experimental results, showing good agreement.
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