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Sökning: WFRF:(Dentener Frank)

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1.
  • Emberson, Lisa D., et al. (författare)
  • Ozone effects on crops and consideration in crop models
  • 2018
  • Ingår i: European Journal of Agronomy. - : Elsevier BV. - 1161-0301. ; 100:Special Issue: SI, s. 19-34
  • Tidskriftsartikel (refereegranskat)abstract
    • © 2018 The Authors We review current knowledge of the processes by which ozone will cause injury and damage to crop plants. We do this both through an understanding of the limitations to ozone uptake (i.e. ozone being transferred from some height in the atmosphere to the leaf boundary layer and subsequent uptake via the stomata) as well as through the internal plant processes that will result in the absorbed ozone dose causing damage and/or injury. We consider these processes across a range of scales by which ozone impacts plants, from cellular metabolism influencing leaf level physiology up to whole canopy and root system processes and feedbacks. We explore how these impacts affect leaf level photosynthesis and senescence (and associated carbon assimilation) as well as whole canopy resource acquisition (e.g. water and nutrients) and ultimately crop growth and yield. We consider these processes from the viewpoint of developing crop growth models capable of incorporating key ozone impact processes within modelling structures that assess crop growth under a variety of different abiotic stresses. These models would provide a dynamic assessment of the impact of ozone within the context of other key variables considered important in determining crop growth and yield. We consider the ability to achieve such modelling through an assessment of the different types of crop model currently available (e.g. empirical, radiation use efficiency, and photosynthesis based crop growth models). Finally, we show how international activities such as the AgMIP (Agricultural Modelling and Improvement Intercomparison Project) could see crop growth modellers collaborate to assess the capabilities of different crop models to simulate the effects of ozone and other stresses. The development of robust crop growth models capable of including ozone effects would substantially improve future national, regional and global risk assessments that aim to assess the role that ozone might play under future climatic conditions in limiting food supply.
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2.
  • Hicks, Kevin, et al. (författare)
  • Soil sensitivity to acidification in Asia : Status and prospects
  • 2008
  • Ingår i: Ambio. ; 37:4, s. 295-303
  • Tidskriftsartikel (refereegranskat)abstract
    • Exceedance of steady-state critical loads for soil acidification is consistently found in southern China and parts of SE Asia, but there is no evidence of impacts outside of China. This study describes a methodology for calculating the time to effects for soils sensitive to acidic deposition in Asia under potential future sulfur (S), nitrogen (N), and calcium (Ca) emission scenarios. The calculations are matched to data availability in Asia to produce regional-scale maps that provide estimates of the time (y) it will take for soil base saturation to reach a critical limit of 20% in response to acidic inputs. The results show that sensitive soil types in areas of South, Southeast, and East Asia, including parts of southern China, Burma, Hainan, Laos, Thailand, Vietnam, and the Western Ghats of India, may acidify to a significant degree on a 0–50 y timescale, depending on individual site management and abiotic and biotic characteristics. To make a clearer assessment of risk, site-specific data are required for soil chemistry and deposition (especially base cation deposition); S and N retention in soils and ecosystems; and biomass harvesting and weathering rates from sites across Asia representative of different soil and vegetation types and management regimes. National and regional assessments of soils using the simple methods described in this paper can provide an appreciation of the time dimension of soil acidification–related impacts and should be useful in planning further studies and, possibly, implementing measures to reduce risks of acidification
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3.
  • Knorr, Wolfgang, et al. (författare)
  • Air quality impacts of European wildfire emissions in a changing climate
  • 2016
  • Ingår i: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 16:9, s. 5685-5703
  • Tidskriftsartikel (refereegranskat)abstract
    • Wildfires are not only a threat to human property and a vital element of many ecosystems, but also an important source of air pollution. In this study, we first review the available evidence for a past or possible future climate-driven increase in wildfire emissions in Europe. We then introduce an ensemble of model simulations with a coupled wildfire-dynamic-ecosystem model, which we combine with published spatial maps of both wildfire and anthropogenic emissions of several major air pollutants to arrive at air pollutant emission projections for several time slices during the 21st century. The results indicate moderate wildfire-driven emission increases until 2050, but there is a possibility of large increases until the last decades of this century at high levels of climate change. We identify southern and north-eastern Europe as potential areas where wildfires may surpass anthropogenic pollution sources during the summer months. Under a scenario of high levels of climate change (Representative Concentration Pathway, RCP, 8.5), emissions from wildfires in central and northern Portugal and possibly southern Italy and along the west coast of the Balkan peninsula are projected to reach levels that could affect annual mean particulate matter concentrations enough to be relevant for meeting WHO air quality targets.
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4.
  • Knorr, Wolfgang, et al. (författare)
  • Wildfire air pollution hazard during the 21st century
  • 2017
  • Ingår i: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 17:14, s. 9223-9236
  • Tidskriftsartikel (refereegranskat)abstract
    • Wildfires pose a significant risk to human livelihoods and are a substantial health hazard due to emissions of toxic smoke. Previous studies have shown that climate change, increasing atmospheric CO2, and human demographic dynamics can lead to substantially altered wildfire risk in the future, with fire activity increasing in some regions and decreasing in others. The present study re-examines these results from the perspective of air pollution risk, focussing on emissions of airborne particulate matter (PM2. 5), combining an existing ensemble of simulations using a coupled fire-dynamic vegetation model with current observation-based estimates of wildfire emissions and simulations with a chemical transport model. Currently, wildfire PM2. 5 emissions exceed those from anthropogenic sources in large parts of the world. We further analyse two extreme sets of future wildfire emissions in a socio-economic, demographic climate change context and compare them to anthropogenic emission scenarios reflecting current and ambitious air pollution legislation. In most regions of the world, ambitious reductions of anthropogenic air pollutant emissions have the potential to limit mean annual pollutant PM2. 5 levels to comply with World Health Organization (WHO) air quality guidelines for PM2. 5. Worst-case future wildfire emissions are not likely to interfere with these annual goals, largely due to fire seasonality, as well as a tendency of wildfire sources to be situated in areas of intermediate population density, as opposed to anthropogenic sources that tend to be highest at the highest population densities. However, during the high-fire season, we find many regions where future PM2. 5 pollution levels can reach dangerous levels even for a scenario of aggressive reduction of anthropogenic emissions.
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6.
  • McGrath, Matthew J., et al. (författare)
  • The consolidated European synthesis of CO2 emissions and removals for the European Union and United Kingdom : 1990-2020
  • 2023
  • Ingår i: Earth System Science Data. - 1866-3508. ; 15:10, s. 4295-4370
  • Tidskriftsartikel (refereegranskat)abstract
    • Quantification of land surface-atmosphere fluxes of carbon dioxide (CO2) and their trends and uncertainties is essential for monitoring progress of the EU27+UK bloc as it strives to meet ambitious targets determined by both international agreements and internal regulation. This study provides a consolidated synthesis of fossil sources (CO2 fossil) and natural (including formally managed ecosystems) sources and sinks over land (CO2 land) using bottom-up (BU) and top-down (TD) approaches for the European Union and United Kingdom (EU27+UK), updating earlier syntheses (Petrescu et al., 2020, 2021). Given the wide scope of the work and the variety of approaches involved, this study aims to answer essential questions identified in the previous syntheses and understand the differences between datasets, particularly for poorly characterized fluxes from managed and unmanaged ecosystems. The work integrates updated emission inventory data, process-based model results, data-driven categorical model results, and inverse modeling estimates, extending the previous period 1990-2018 to the year 2020 to the extent possible. BU and TD products are compared with the European national greenhouse gas inventory (NGHGI) reported by parties including the year 2019 under the United Nations Framework Convention on Climate Change (UNFCCC). The uncertainties of the EU27+UK NGHGI were evaluated using the standard deviation reported by the EU member states following the guidelines of the Intergovernmental Panel on Climate Change (IPCC) and harmonized by gap-filling procedures. Variation in estimates produced with other methods, such as atmospheric inversion models (TD) or spatially disaggregated inventory datasets (BU), originate from within-model uncertainty related to parameterization as well as structural differences between models. By comparing the NGHGI with other approaches, key sources of differences between estimates arise primarily in activities. System boundaries and emission categories create differences in CO2 fossil datasets, while different land use definitions for reporting emissions from land use, land use change, and forestry (LULUCF) activities result in differences for CO2 land. The latter has important consequences for atmospheric inversions, leading to inversions reporting stronger sinks in vegetation and soils than are reported by the NGHGI. For CO2 fossil emissions, after harmonizing estimates based on common activities and selecting the most recent year available for all datasets, the UNFCCC NGHGI for the EU27+UK accounts for 926g±g13gTggCgyr-1, while eight other BU sources report a mean value of 948 [937,961]gTggCgyr-1 (25th, 75th percentiles). The sole top-down inversion of fossil emissions currently available accounts for 875gTggC in this same year, a value outside the uncertainty of both the NGHGI and bottom-up ensemble estimates and for which uncertainty estimates are not currently available. For the net CO2 land fluxes, during the most recent 5-year period including the NGHGI estimates, the NGHGI accounted for -91g±g32gTggCgyr-1, while six other BU approaches reported a mean sink of -62 [-117,-49]gTggCgyr-1, and a 15-member ensemble of dynamic global vegetation models (DGVMs) reported -69 [-152,-5]gTggCgyr-1. The 5-year mean of three TD regional ensembles combined with one non-ensemble inversion of -73gTggCgyr-1 has a slightly smaller spread (0th-100th percentiles of [-135,+45]gTggCgyr-1), and it was calculated after removing net land-atmosphere CO2 fluxes caused by lateral transport of carbon (crop trade, wood trade, river transport, and net uptake from inland water bodies), resulting in increased agreement with the NGHGI and bottom-up approaches. Results at the category level (Forest Land, Cropland, Grassland) generally show good agreement between the NGHGI and category-specific models, but results for DGVMs are mixed. Overall, for both CO2 fossil and net CO2 land fluxes, we find that current independent approaches are consistent with the NGHGI at the scale of the EU27+UK. We conclude that CO2 emissions from fossil sources have decreased over the past 30 years in the EU27+UK, while land fluxes are relatively stable: positive or negative trends larger (smaller) than 0.07 (-0.61)gTggCgyr-2 can be ruled out for the NGHGI. In addition, a gap on the order of 1000gTggCgyr-1 between CO2 fossil emissions and net CO2 uptake by the land exists regardless of the type of approach (NGHGI, TD, BU), falling well outside all available estimates of uncertainties. However, uncertainties in top-down approaches to estimate CO2 fossil emissions remain uncharacterized and are likely substantial, in addition to known uncertainties in top-down estimates of the land fluxes. The data used to plot the figures are available at 10.5281/zenodo.8148461 (McGrath et al., 2023).
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7.
  • Messori, Gabriele, et al. (författare)
  • The impact of future atmospheric circulation changes over the Euro-Atlantic sector on urban PM2.5 concentrations
  • 2018
  • Ingår i: Tellus. Series B, Chemical and physical meteorology. - : Stockholm University Press. - 0280-6509 .- 1600-0889. ; 70:1
  • Tidskriftsartikel (refereegranskat)abstract
    • Air quality management is strongly driven by legislative aspects related to the exceedance of air quality limit values. Here, we use the Norwegian Climate Centre's Earth System Model to assess the impact of a future scenario of maximum feasible aerosol emission abatement and increasing greenhouse gases (RCP4.5) on urban PM2.5 concentrations in Europe. Daily PM2.5 concentrations are assessed using a novel downscaling method which allows us to compute exceedances of current and planned air quality thresholds. For the latter, we assume that future ambitious emission reductions are likely to be accompanied by stricter air quality thresholds. The changes in PM2.5 concentrations are discussed in the context of the large-scale atmospheric changes observed relative to the present-day climate.Our results show a more positive North Atlantic Oscillation mean state in the future, combined with a large eastward shift of both North Atlantic sea-level pressure centres of action. This is associated with more frequent mid-latitude blocking and a northward shift of the jet stream. These changes favour higher than expected anthropogenic urban PM2.5 concentrations in Southern Europe, while they have the opposite effect on the northern half of the continent. In the future scenario, PM concentrations in substantial parts of Southern Europe are found to exceed the World Health Organisation Air Quality Guideline daily limit of 25g/m(3) on 25 to over 50days per year, and annual guidelines of 10 mu g/m(3) on more than 80% of the 30years analysed in our study. We conclude that alterations in atmospheric circulation in the future, induced by stringent maximum feasible air pollution mitigation as well as GHG emissions, will negatively influence the effectiveness of these emission abatements over large parts of Europe. This has important implications for future air quality policies.
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8.
  • Petrescu, Ana Maria Roxana, et al. (författare)
  • The consolidated European synthesis of CH4 and N2O emissions for the European Union and United Kingdom: 1990-2019
  • 2023
  • Ingår i: Earth System Science Data. - : COPERNICUS GESELLSCHAFT MBH. - 1866-3508 .- 1866-3516. ; 15:3, s. 1197-1268
  • Tidskriftsartikel (refereegranskat)abstract
    • Knowledge of the spatial distribution of the fluxes of greenhouse gases (GHGs) and their temporal variability as well as flux attribution to natural and anthropogenic processes is essential to monitoring the progress in mitigating anthropogenic emissions under the Paris Agreement and to inform its global stocktake. This study provides a consolidated synthesis of CH4 and N2O emissions using bottom-up (BU) and top-down (TD) approaches for the European Union and UK (EU27 + UK) and updates earlier syntheses (Petrescu et al., 2020, 2021). The work integrates updated emission inventory data, process-based model results, data-driven sector model results and inverse modeling estimates, and it extends the previous period of 1990-2017 to 2019. BU and TD products are compared with European national greenhouse gas inventories (NGHGIs) reported by parties under the United Nations Framework Convention on Climate Change (UNFCCC) in 2021. Uncertainties in NGHGIs, as reported to the UNFCCC by the EU and its member states, are also included in the synthesis. Variations in estimates produced with other methods, such as atmospheric inversion models (TD) or spatially disaggregated inventory datasets (BU), arise from diverse sources including within-model uncertainty related to parameterization as well as structural differences between models. By comparing NGHGIs with other approaches, the activities included are a key source of bias between estimates, e.g., anthropogenic and natural fluxes, which in atmospheric inversions are sensitive to the prior geospatial distribution of emissions. For CH4 emissions, over the updated 2015-2019 period, which covers a sufficiently robust number of overlapping estimates, and most importantly the NGHGIs, the anthropogenic BU approaches are directly comparable, accounting for mean emissions of 20.5 TgCH(4) yr(-1) (EDGARv6.0, last year 2018) and 18.4 TgCH(4) yr(-1) (GAINS, last year 2015), close to the NGHGI estimates of 17 :5 +/- 2 :1 TgCH(4) yr(-1). TD inversion estimates give higher emission estimates, as they also detect natural emissions. Over the same period, high-resolution regional TD inversions report a mean emission of 34 TgCH(4) yr(-1). Coarser-resolution global-scale TD inversions result in emission estimates of 23 and 24 TgCH(4) yr(-1) inferred from GOSAT and surface (SURF) network atmospheric measurements, respectively. The magnitude of natural peatland and mineral soil emissions from the JSBACH-HIMMELI model, natural rivers, lake and reservoir emissions, geological sources, and biomass burning together could account for the gap between NGHGI and inversions and account for 8 TgCH(4) yr(-1). For N2O emissions, over the 2015-2019 period, both BU products (EDGARv6.0 and GAINS) report a mean value of anthropogenic emissions of 0.9 TgN(2)Oyr(-1), close to the NGHGI data (0 :8 +/- 55% TgN(2)Oyr(-1)). Over the same period, the mean of TD global and regional inversions was 1.4 TgN(2)Oyr(-1) (excluding TOMCAT, which reported no data). The TD and BU comparison method defined in this study can be operationalized for future annual updates for the calculation of CH4 and N2O budgets at the national and EU27 C UK scales. Future comparability will be enhanced with further steps involving analysis at finer temporal resolutions and estimation of emissions over intra-annual timescales, which is of great importance for CH4 and N2O, and may help identify sector contributions to divergence between prior and posterior estimates at the annual and/or inter-annual scale. Even if currently comparison between CH4 and N2O inversion estimates and NGHGIs is highly uncertain because of the large spread in the inversion results, TD inversions inferred from atmospheric observations represent the most independent data against which inventory totals can be compared. With anticipated improvements in atmospheric modeling and observations, as well as modeling of natural fluxes, TD inversions may arguably emerge as the most powerful tool for verifying emission inventories for CH4, N2O and other GHGs. The referenced dataset srelated to figures are visualized at https://doi.org/10.5281/zenodo.7553800 (Petrescu et al., 2023).
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9.
  • Toreti, Andrea, et al. (författare)
  • The exceptional 2018 European water seesaw calls for action on adaptation
  • 2019
  • Ingår i: Earth's Future. - : American Geophysical Union (AGU). - 2328-4277. ; 7:6, s. 652-663
  • Tidskriftsartikel (refereegranskat)abstract
    • Temperature and precipitation are the most important factors responsible for agricultural productivity variations. In 2018 spring/summer growing season, Europe experienced concurrent anomalies of both. Drought conditions in central and northern Europe caused yield reductions up to 50% for the main crops, yet wet conditions in southern Europe saw yield gains up to 34%, both with respect to the previous 5‐years' mean. Based on the analysis of documentary and natural proxy based seasonal paleoclimate reconstructions for the past half millennium, we show that the 2018 combination of climatic anomalies in Europe was unique. The water seesaw, a marked dipole of negative water anomalies in central Europe and positive ones in southern Europe, distinguished 2018 from the five previous similar droughts since 1976. Model simulations reproduce the 2018 European water seesaw in only four years out of 875 years in historical runs and projections. Future projections under the RCP8.5 scenario show that 2018‐like temperature and rainfall conditions, favourable to crop growth, will occur less frequent in southern Europe. In contrast, in central Europe high‐end emission scenario climate projections show that droughts as intense as 2018 could become a common occurrence as early as 2043. Whilst integrated European and global agricultural markets limited agro‐economic shocks caused by 2018's extremes, there is an urgent need for adaptation strategies for European agriculture to consider futures without the benefits of any water seesaw.
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