| 1. |
- Klintenberg, Mattias, et al.
(författare)
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The use of molecular dynamics to simulate the temperature dependence of the calculated absorption spectrum for Nd3+:YAG
- 1999
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Ingår i: Materials Science Forum. - 0255-5476. ; 315-317, s. 42-50
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Tidskriftsartikel (refereegranskat)abstract
- The use of molecular dynamics (MD) and the inclusion of configuration interaction (CI) effects have been shown to be important in the simulation of polarized absorption spectra for rare-earth doped compounds. This work, focuses on how well the MD approach can account for the temperature dependence of the calculated absorption spectrum for Nd3+:YAG, using the standard MD pair-potential of the Born-Mayer-Huggins form. All simulated spectra are compared to the corresponding experimental spectra. The results indicate that the simple pair-potential must be replaced by a many-body potential to describe the motion of the ions with sufficient accuracy. They also suggest that an “effective temperature” (T') should be used in the MD simulation of the form T'=aT+b
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| 2. |
- Goldner, Ph., et al.
(författare)
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Long coherence lifetime and electromagnetically induced transparency in a highly-spin-concentrated solid
- 2009
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Ingår i: Physical Review A (Atomic, Molecular and Optical Physics). - 1050-2947. ; 79:3
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Tidskriftsartikel (refereegranskat)abstract
- We have studied a rare-earth-doped crystal, Pr3+:La-2(WO4)(3), which exhibits a high magnetic-moment density. Although the latter favors rare-earth dephasing, a nuclear-spin coherence lifetime of 250 mu s has been observed, as well as electromagnetically induced transparency (EIT). This suggests that a broad range of materials could be considered for quantum information applications such as quantum memories for light, where solids are especially attractive. Absorption and dispersion curves are independently in very good agreement with EIT theory. Fano-like profiles have also been observed.
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| 3. |
- Guillot-Noel, O., et al.
(författare)
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Hyperfine structure and hyperfine coherent properties of praseodymium in single-crystalline La-2(WO4)(3) by hole-burning and photon-echo techniques
- 2009
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Ingår i: Physical Review B (Condensed Matter and Materials Physics). - 1098-0121. ; 79:15
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Tidskriftsartikel (refereegranskat)abstract
- We studied the hyperfine structure and hyperfine coherent properties of the H-3(4)(0)-> D-1(2)(0) transition of Pr3+ ions in a tungstate single crystal La-2(WO4)(3) by hole-burning and photon-echo techniques. This work is motivated by the search of an efficient three level Lambda system in this new compound with which we could build up a quantum memory. By nonconventional hole-burning experiments, the ordering of the hyperfine splittings in the H-3(4)(0) ground state and in the D-1(2)(0) excited state is obtained. The hyperfine splittings are thus ordered: 24.6 and 14.9 MHz for the H-3(4)(0) level and 5.0 and 7.3 MHz for the D-1(2)(0) level. The relative and absolute transition strengths of individual hyperfine transitions are determined by comparing absorption strengths and by measuring the Rabi flopping frequency as the transition is coherently driven. Free induction and Raman echo decays give inhomogeneous and homogeneous hyperfine linewidths of 57 +/- 2 and 1.25 +/- 0.1 kHz, respectively.
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| 4. |
- Guillot-Noel, O., et al.
(författare)
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Hyperfine structure, optical dephasing, and spectral-hole lifetime of single-crystalline Pr3+: La-2(WO4)(3)
- 2007
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Ingår i: Physical Review B (Condensed Matter and Materials Physics). - 1098-0121. ; 75:20
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Tidskriftsartikel (refereegranskat)abstract
- Most of the experiments related to quantum information applications, involving rare-earth doped inorganic crystals, are performed on yttrium orthosilicate single crystals. The work presented here is motivated by the search of new compounds which can be used in the field of quantum computing and/or quantum storage. Relaxation times and hyperfine structure of the H-3(4)(0)-> D-1(2)(0) transition in 1.4% Pr3+:La-2(WO4)(3) at 4 K have been measured by photon-echo and spectral-hole-burning techniques. The hyperfine splittings of the ground H-3(4)(0) and the excited D-1(2)(0) states are 14.9 +/- 0.1 MHz, 24.6 +/- 0.1 MHz and 5.0 +/- 0.1 MHz, 7.3 +/- 0.1 MHz, respectively. An inhomogeneous linewidth of 18.8 +/- 0.1 GHz was measured. A homogeneous linewidth of 25.3 +/- 2.0 kHz was obtained with or without an external magnetic field of about 14 mT. The fluorescence dynamics of the D-1(2) level obtained by a direct excitation in the H-3(4)-> D-1(2) transition gives a nonexponential decay which indicates energy-transfer processes. This decay can be accurately fitted by the Inokuti-Hirayama model [J. Chem. Phys. 43, 1978 (1965)] with a radiative lifetime of 61 +/- 1 mu s giving a minimal homogeneous linewidth of 2.6 kHz. The spectral-hole lifetime due to population redistribution within the ground hyperfine levels is 16 +/- 2 s. The results obtained for the La-2(WO4)(3) compound make this crystal an interesting host for quantum applications.
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| 5. |
- Moncorge, R, et al.
(författare)
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Linear and non-linear spectroscopy of Ho3+-doped YVO4 and LuVO4
- 2005
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Ingår i: Journal of Physics: Condensed Matter. - : IOP Publishing. - 1361-648X .- 0953-8984. ; 17:42, s. 6751-6762
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Tidskriftsartikel (refereegranskat)abstract
- Rare-earth-doped crystals can be attractive materials for quantum information processing, because of the long coherence times that can be expected, in particular, from non-Kramers ions. In this paper, Ho3+-doped yttrium and lutetium vanadate single crystals have been investigated using linear and coherent optical spectroscopy. For Ho3+:YVO4, the crystal-field levels of the I-5(8), F-5, F-5(4) and S-5(2) multiplets have been determined and compared with crystal-field level calculations. This allowed us to unambiguously assign most of the observed transitions, although some results suggest that the site symmetry of the Ho3+ ion could deviate from D-2d. Similar conclusions were reached for Ho3+:LuVO4. Hole burning measurements indicate that the coherence time of the I-5(8)-F-5(5) optical transitions is rather short in both compounds (around 40 ns). Assuming that the coherence is limited by spin interactions, this is accounted for by the high nuclear moment of the nearby vanadium ions, since the large crystal-field level splittings of the I-5(8) and F-5(5) multiplets do not favour a large enhanced nuclear Zeeman effect.
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