| 1. |
- Bergues, B., et al.
(författare)
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Nonlinear interaction of 100-eV attosecond XUV-pulses with core electrons in Xenon
- 2018
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Ingår i: Optics InfoBase Conference Papers. - : Optica Publishing Group. - 9781557528209
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Konferensbidrag (refereegranskat)abstract
- We demonstrate multiphoton ionization of inner-shell electrons in Xenon with 100-eV attosecond pulses. This was achieved with a novel XUV source based on high-harmonic generation in the gas phase driven with multi-TW few-cycle laser pulses.
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| 2. |
- Bergues, B., et al.
(författare)
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Tabletop nonlinear optics in the 100-eV spectral region
- 2018
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Ingår i: Optica. - : Optical Society of America. - 2334-2536. ; 5:3, s. 237-242
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Tidskriftsartikel (refereegranskat)abstract
- Nonlinear light-matter interactions in the extreme ultraviolet (XUV) are a prerequisite to perform XUV-pump/XUV-probe spectroscopy of core electrons. Such interactions are now routinely investigated at free-electron laser (FEL) facilities. Yet, electron dynamics are often too fast to be captured with the femtosecond resolution of state-of-the-art FELs. Attosecond pulses from laser-driven XUV-sources offer the necessary temporal resolution. However, intense attosecond pulses supporting nonlinear processes have only been available for photon energy below 50 eV, precluding XUV-pump/XUV-probe investigation of typical inner-shell processes. Here, we surpass this limitation by demonstrating two-photon absorption from inner electronic shells of xenon at photon energies around 93 eV and 115 eV. This advance opens the door for attosecond real-time observation of nonlinear electron dynamics deep inside atoms.
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| 3. |
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| 4. |
- Hartmann, G., et al.
(författare)
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Circular dichroism measurements at an x-ray free-electron laser with polarization control
- 2016
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Ingår i: Review of Scientific Instruments. - : AIP Publishing. - 0034-6748 .- 1089-7623. ; 87:8
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Tidskriftsartikel (refereegranskat)abstract
- A non-destructive diagnostic method for the characterization of circularly polarized, ultraintense, short wavelength free-electron laser (FEL) light is presented. The recently installed Delta undulator at the LCLS (Linac Coherent Light Source) at SLAC National Accelerator Laboratory (USA) was used as showcase for this diagnostic scheme. By applying a combined two-color, multi-photon experiment with polarization control, the degree of circular polarization of the Delta undulator has been determined. Towards this goal, an oriented electronic state in the continuum was created by non-resonant ionization of the O2 1s core shell with circularly polarized FEL pulses at hν 700 eV. An also circularly polarized, highly intense UV laser pulse with hν 3.1 eV was temporally and spatially overlapped, causing the photoelectrons to redistribute into so-called sidebands that are energetically separated by the photon energy of the UV laser. By determining the circular dichroism of these redistributed electrons using angle resolving electron spectroscopy and modeling the results with the strong-field approximation, this scheme allows to unambiguously determine the absolute degree of circular polarization of any pulsed, ultraintense XUV or X-ray laser source. © 2016 Author(s).
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| 5. |
- Hartmann, N., et al.
(författare)
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Attosecond time-energy structure of X-ray free-electron laser pulses
- 2018
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Ingår i: Nature Photonics. - : Springer Science and Business Media LLC. - 1749-4885 .- 1749-4893. ; 12:4, s. 215-220
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Tidskriftsartikel (refereegranskat)abstract
- The time-energy information of ultrashort X-ray free-electron laser pulses generated by the Linac Coherent Light Source is measured with attosecond resolution via angular streaking of neon 1s photoelectrons. The X-ray pulses promote electrons from the neon core level into an ionization continuum, where they are dressed with the electric field of a circularly polarized infrared laser. This induces characteristic modulations of the resulting photoelectron energy and angular distribution. From these modulations we recover the single-shot attosecond intensity structure and chirp of arbitrary X-ray pulses based on self-amplified spontaneous emission, which have eluded direct measurement so far. We characterize individual attosecond pulses, including their instantaneous frequency, and identify double pulses with well-defined delays and spectral properties, thus paving the way for X-ray pump/X-ray probe attosecond free-electron laser science. © 2018 The Author(s).
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| 6. |
- Heider, R., et al.
(författare)
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Megahertz-compatible angular streaking with few-femtosecond resolution at x-ray free-electron lasers
- 2019
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Ingår i: Physical Review A. - 2469-9926. ; 100:5
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Tidskriftsartikel (refereegranskat)abstract
- Highly brilliant, coherent, femtosecond x-ray pulses delivered by free-electron lasers (FELs) constitute one of the pillars of modern ultrafast science. Next generation FEL facilities provide up to megahertz repetition rates and pulse durations down to the attosecond regime utilizing self-amplification of spontaneous emission. However, the stochastic nature of this generation mechanism demands single-shot pulse characterization to perform meaningful experiments. Here we demonstrate a fast yet robust online analysis technique capable of megahertz-rate mapping of the temporal intensity structure and arrival time of x-ray FEL pulses with few-femtosecond resolution. We performed angular streaking measurements of both neon photo- and Auger electrons and show their applicability for a direct time-domain feedback system during ongoing experiments. The fidelity of the real-time pulse characterization algorithm is corroborated by resolving isolated x-ray pulses and double pulse trains with few-femtosecond substructure, thus paving the way for x-ray-pump-x-ray-probe FEL science at repetition rates compatible with the demands of LCLS-II and European XFEL.
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| 7. |
- Sanchez-Gonzalez, A., et al.
(författare)
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Accurate prediction of X-ray pulse properties from a free-electron laser using machine learning
- 2017
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Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723. ; 8
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Tidskriftsartikel (refereegranskat)abstract
- Free-electron lasers providing ultra-short high-brightness pulses of X-ray radiation have great potential for a wide impact on science, and are a critical element for unravelling the structural dynamics of matter. To fully harness this potential, we must accurately know the X-ray properties: intensity, spectrum and temporal profile. Owing to the inherent fluctuations in free-electron lasers, this mandates a full characterization of the properties for each and every pulse. While diagnostics of these properties exist, they are often invasive and many cannot operate at a high-repetition rate. Here, we present a technique for circumventing this limitation. Employing a machine learning strategy, we can accurately predict X-ray properties for every shot using only parameters that are easily recorded at high-repetition rate, by training a model on a small set of fully diagnosed pulses. This opens the door to fully realizing the promise of next-generation high-repetition rate X-ray lasers.
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| 8. |
- Wenz, J., et al.
(författare)
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Dual-energy electron beams from a compact laser-driven accelerator
- 2019
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Ingår i: Nature Photonics. - : Nature Publishing Group. - 1749-4885 .- 1749-4893. ; 13, s. 263-269
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Tidskriftsartikel (refereegranskat)abstract
- Ultrafast pump–probe experiments open the possibility to track fundamental material behaviour, such as changes in electronic configuration, in real time. To date, most of these experiments are performed using an electron or a high-energy photon beam that is synchronized to an infrared laser pulse. Entirely new opportunities can be explored if not only a single, but multiple synchronized, ultrashort, high-energy beams are used. However, this requires advanced radiation sources that are capable of producing dual-energy electron beams, for example. Here, we demonstrate simultaneous generation of twin-electron beams from a single compact laser wakefield accelerator. The energy of each beam can be individually adjusted over a wide range and our analysis shows that the bunch lengths and their delay inherently amount to femtoseconds. Our proof-of-concept results demonstrate an elegant way to perform multi-beam experiments in the future on a laboratory scale.
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