| 1. |
- Aldahan, Ala, et al.
(författare)
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Distribution of I-127 and I-129 in preciptitation at high European latitudes
- 2009
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Ingår i: Geophysical Research Letters. - 0094-8276 .- 1944-8007. ; 36, s. L11805-
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Tidskriftsartikel (refereegranskat)abstract
- We here present the most extensive data set on the distribution of I-127 and I-129 in precipitation (rain and snow) covering the period 2000-2006 and European latitudes 55 degrees N-68 degrees N. Our results indicate a wide variation in the concentrations and fluxes of the two isotopes associated with generally higher values at near coastal sites compared to the inland ones. Total wet-related annual deposition of I-127 and I-129 on Sweden and Denmark is estimated at about 1.2 x 10(9) g and 60 g respectively. The average annual I-129 wet deposition accounts for <1% and <0.05% of the total annual gaseous and liquid, respectively, discharges from the Sellafiled and La Hague Facilities. The I-127 annual wet deposition represents < 1% of the estimated global oceanic iodine flux. Air mass trajectories suggest that events of enhanced I-129 in precipitation are closely related to southwesterly weather fronts from regions of elevated concentrations.
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| 2. |
- Aldahan, Ala, et al.
(författare)
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Iodine-129 enrichment in sediment of the Baltic Sea
- 2007
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Ingår i: Applied Geochemistry. - : Elsevier BV. - 0883-2927 .- 1872-9134. ; 22:3, s. 637-647
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Tidskriftsartikel (refereegranskat)abstract
- Sediments are an excellent archive for evaluation of time-series environmental contamination of water systems. Measurements of ultra-trace radioactive species, such as 129I, provide information for both chronologic calibration and anthropogenic emissions during the nuclear era. Here data are presented on 129I and other chemical parameters from two sediment cores collected in the Baltic Sea during 1997. The sediment sections have a relatively uniform grain size (clay–mud) and cover a period of about 50 a. Distribution of 129I in the sediment strongly relates to the liquid release records from the nuclear reprocessing facilities at Sellafield and La Hague. However, syn- and post-depositional alteration of organic matter at the sediment–water interface and within the sediment column may have contributed to slightly obliterating the anthropogenic 129I signals. Indication of Chernobyl-derived 129I occurs in the sediment profile, but is apparently overridden by the overwhelming flux from the nuclear reprocessing facilities. Although the record did not cover the pre-nuclear era (before 1945) sections, the ultra sensitive 129I profile provides a potential tool for relative dating and monitoring sources of water and sediment to the region.
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| 3. |
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| 4. |
- Alshamsi, Dalal M., et al.
(författare)
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Uranium isotopes in carbonate aquifers of arid region setting
- 2013
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Ingår i: Journal of Radioanalytical and Nuclear Chemistry. - : Springer Science and Business Media LLC. - 0236-5731 .- 1588-2780. ; 298:3, s. 1899-1905
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Tidskriftsartikel (refereegranskat)abstract
- Groundwater in arid and semiarid regions is vital resource for many uses and therefore information about concentrations of uranium isotopes among other chemical parameters are necessary. In the study presented here, distribution of U-238 and U-235 in groundwater of four selected locations in the southern Arabian peninsula, namely at two locations within the United Arab Emirates (UAE) and two locations in Oman are discussed. The analyses of the uranium isotopes were performed using ICP-MS and the results indicated a range of concentrations for U-235 and (238) U at 3-39 ng L-1 (average: 18 ng L-1) and 429-5,293 ng L-1 (average: 2,508 ng L-1) respectively. These uranium concentrations are below the higher permissible WHO limit for drinking water and also comparable to averages found in groundwater from similar aquifers in Florida and Tunisia. Negative correlation between rainfall and uranium concentrations suggests that in lithologically comparable aquifers, climate may influence the concentration of uranium in subtropical to arid regions.
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| 5. |
- An, Junghwa, et al.
(författare)
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Permanent Genetic Resources added to Molecular Ecology Resources Database 1 October 2009-30 November 2009
- 2010
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Ingår i: Molecular Ecology Resources. - : Wiley. - 1755-098X .- 1755-0998. ; 10:2, s. 404-408
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Tidskriftsartikel (refereegranskat)abstract
- This article documents the addition of 411 microsatellite marker loci and 15 pairs of Single Nucleotide Polymorphism (SNP) sequencing primers to the Molecular Ecology Resources Database. Loci were developed for the following species: Acanthopagrus schlegeli, Anopheles lesteri, Aspergillus clavatus, Aspergillus flavus, Aspergillus fumigatus, Aspergillus oryzae, Aspergillus terreus, Branchiostoma japonicum, Branchiostoma belcheri, Colias behrii, Coryphopterus personatus, Cynogolssus semilaevis, Cynoglossus semilaevis, Dendrobium officinale, Dendrobium officinale, Dysoxylum malabaricum, Metrioptera roeselii, Myrmeciza exsul, Ochotona thibetana, Neosartorya fischeri, Nothofagus pumilio, Onychodactylus fischeri, Phoenicopterus roseus, Salvia officinalis L., Scylla paramamosain, Silene latifo, Sula sula, and Vulpes vulpes. These loci were cross-tested on the following species: Aspergillus giganteus, Colias pelidne, Colias interior, Colias meadii, Colias eurytheme, Coryphopterus lipernes, Coryphopterus glaucofrenum, Coryphopterus eidolon, Gnatholepis thompsoni, Elacatinus evelynae, Dendrobium loddigesii Dendrobium devonianum, Dysoxylum binectariferum, Nothofagus antarctica, Nothofagus dombeyii, Nothofagus nervosa, Nothofagus obliqua, Sula nebouxii, and Sula variegata. This article also documents the addition of 39 sequencing primer pairs and 15 allele specific primers or probes for Paralithodes camtschaticus.
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| 6. |
- Chen, Peng, et al.
(författare)
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Relationship between precipitation and Be-10 and impacts on soil dynamics
- 2020
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Ingår i: Catena (Cremlingen. Print). - : Elsevier BV. - 0341-8162 .- 1872-6887. ; 195
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Tidskriftsartikel (refereegranskat)abstract
- Meteoric beryllium-10 (Be-10) is commonly used as a proxy of landscape dynamics (erosion and sedimentation rates) and soil development. Soil represents the first-stage reservoir of meteoric Be-10, and variability in the concentration of the isotope in soils may be affected by soil properties and atmospheric deposition. Although many investigations have targeted this issue, there are still problems in estimating the atmospheric input of the isotope in different soil environments. Here, we used Be-10 data measured in soils distributed across China to explore the potential influence of meteorological and pedological conditions on the isotope concentration and related applications. In addition, to determine the mechanisms controlling Be-10 concentrations in topsoil on a regional scale, the soil samples were sub-divided into 18 different catchments according to fluvial systems. The results indicated that there were significant negative correlations between precipitation and the soil Be-10 concentration in high-precipitation regions (> 1200 mm.y(-1)) and significant positive correlations for soils in low precipitation regions (< 1200 mm.y(-1)). The data also revealed that precipitation is the most important variable controlling the Be-10 concentration in soils of China when compared with the effects of soil properties such as grain size, mineralogy, pH, and cation exchange capacity. Land use and soil erosion may have limited impacts on the distribution of Be-10 in soils.
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| 7. |
- Chen, Peng, et al.
(författare)
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Tendency of soil erosion dynamics by coupling radioisotopes and RUSLE model on the Southeastern Tibetan Plateau in response to climate warming and human activity
- 2023
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Ingår i: Catena. - : Elsevier BV. - 0341-8162. ; 223
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Tidskriftsartikel (refereegranskat)abstract
- Soil erosion has created landscape problems in many parts of the world and in particular in cold regions where the sensitive permafrost conditions have changed due to climate warming. Such a case occurred in the Tibetan Plateau (TP), which has been strongly affected by global warming and human activities. Monitoring technologies, like remote sensing and field surveys were used to explore soil erosion rates in the TP, but they were limited by the resolution and meteorological disturbance factors or the spatial and time scales. Here, we present for the first time 210Pbex (excess lead-210) and 137Cs (caesium-137) data of soils from the southeastern TP (SETP) covering an area of 640,000 km2. In the permafrost-dominant areas, the results show mean soil-erosion rates in the last 56–100 years that were relatively higher (1891 t·km−2·a-1) based on 210Pbex than those based on 137Cs (1623 t·km−2·a-1). Modelling results from the Revised Universal Soil Loss Equation (RUSLE) indicate relatively high mean soil erosion rates of 4363 and 4394 t·km−2·a-1 using a period covering the last 40 or 10 years respectively. Our data suggest accelerating erosion rates on the SETP that are linked to permafrost degradation, and glacier and snow melting due to accelerating global climate warming. The increase in ground surface temperature of ∼2 °C in the last four decades has further shifted the regional hydrology, affecting the degeneration of vegetation cover and a further increase in soil-erosion rates. However, our radionuclides data also expose low erosion rates in the seasonally frozen ground at some sampling sites which indicates the complex nature of erosion trends in cold regions that require careful adaptation of soil management.
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| 8. |
- Englund, Edvard, et al.
(författare)
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Modeling fallout of anthropogenic I-129
- 2008
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Ingår i: Environmental Science and Technology. - : American Chemical Society (ACS). - 0013-936X .- 1520-5851. ; 42:24, s. 9225-9230
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Tidskriftsartikel (refereegranskat)abstract
- Despite the relatively well-recognized emission rates of the anthropogenic 128I, there is little knowledge about the temporal fallout patterns and magnitude of fluxes since the start of the atomic era at the early 1940s.We here present measurements of annual 129I concentrations in sediment archives from Sweden and Finland covering the period 1942-2006. The results revealed impression of 129I emissions from the nuclear reprocessing facility at Sellafield and La Hague and a clear Chernobyl fallout enhancement during 1986. In order to estimate relative contributions from the different sources, a numerical model approach was used taking into accountthe emission rates/ estimated fallout, transport pathways, and the sediment system. The model outcomes suggest a relatively dominating marine source of 129I to north Europe compared to direct gaseous releases. A transfer rate of 129I from sea to atmosphere is derived for pertinent sea areas (English Channel, Irish Sea, and North Sea), which is estimated at 0.04 to 0.21 y-1.
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| 9. |
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| 10. |
- Hansen, Violeta, et al.
(författare)
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Iodide and iodate ((129)I and (127)I) in surface water of the Baltic Sea, Kattegat and Skagerrak
- 2011
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Ingår i: Science of the Total Environment. - : Elsevier BV. - 0048-9697 .- 1879-1026. ; 412, s. 296-303
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Tidskriftsartikel (refereegranskat)abstract
- Despite the common incorporation of iodine in the biological cycle and occurrence of huge contamination of the radioactive isotope (129)I in the Baltic Proper, Skagerrak and Kattegat, there is no data on chemical speciation of iodine in these waters. We here present first time data on iodine isotopes (129)I and (127)I species as iodide and iodate in surface seawater samples collected from 16 locations in August 2006 and 19 locations in April 2007 in the Baltic Proper, Skagerrak and Kattegat. After extensive separation methods, the isotopes concentrations were determined using accelerator mass spectrometry (AMS) technique for the (129)I and inductively coupled plasma mass spectroscopy (ICP-MS) for (127)I. High concentrations of both isotopes species were found in the Skagerrak-Kattegat basins, whereas the values in the Baltic Proper are low for both species. The ratios of (129)I(-)/(129)IO(3)(-) and (127)I-/(127)IO(3)(-) significantly increase from south to central Baltic Sea, and iodide (both isotopes) appears as the predominant inorganic iodine species along the Baltic Sea. The results show insignificant change in (129)I and (127)I speciation and suggest that reduction of iodate and oxidation of iodide in Skagerrak and Kattegat may be a slow process. Additionally, the positive correlation between salinity and iodide and iodate (both isotopes) may reflect effective control of Skagerrak water mass on iodine distribution in surface water of the Baltic Sea.
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