| 1. |
- Morozov, Konstantin M., et al.
(författare)
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Efficient UV Luminescence from Organic-Based Tamm Plasmon Structures Emitting in the Strong-Coupling Regime
- 2020
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Ingår i: The Journal of Physical Chemistry C. - : AMER CHEMICAL SOC. - 1932-7447 .- 1932-7455. ; 124:39, s. 21656-21663
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Tidskriftsartikel (refereegranskat)abstract
- Excitons in organic semiconductors possessing a large oscillator strength demonstrate strong coupling with cavity modes at room temperature. A large Stokes shift in some organic semiconductors enriches and complicates the picture of the emission in strongly coupled systems of organic excitons and light. Here, we demonstrate strong coupling of excitons in 4,4-bis(N-carbazolyl)-1,1-biphenyl (CBP) and Tamm plasmons in the ultraviolet (UV) band, accompanied by a bright emission from the structure. Reflection measurements demonstrate the pronounced formation of the lower and upper polariton modes with Rabi splitting of the magnitude of 0.3 eV, and the emission peak experiences a substantial red shift with respect to the lower polariton mode. Both radiative and nonradiative decay rates in the Tamm plasmon CBP structure are increased with respect to a bare CBP. Such peculiar behavior is attributed to the simultaneous manifestation of strong coupling and weak coupling of the CBP molecule emitters to the Tamm plasmons.
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| 2. |
- Morozov, Konstantin M., et al.
(författare)
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Opposite Sign of Polarization Splitting in Ultrastrongly Coupled Organic Tamm Plasmon Structures
- 2021
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Ingår i: The Journal of Physical Chemistry C. - : AMER CHEMICAL SOC. - 1932-7447 .- 1932-7455. ; 125:15, s. 8376-8381
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Tidskriftsartikel (refereegranskat)abstract
- The properties of the ultrastrongly coupled Tamm plasmon cavity filled with a high-oscillator-strength organic material DPAVBi (4,4-bis[4-(di-p-tolylamino)styryl]biphenyl) are studied using theoretical and experimental methods. An analytical model predicts the opposite sign of polarization splitting for the lower and upper polariton cases and a giant absolute value of the splitting. A set of organic Tamm plasmon cavities with different detuning parameters are fabricated. We demonstrate that all structures are operating in the ultrastrong coupling regime: the values of the Rabi splitting are close to a 20% fraction of the exciton energy. The measured angle-dependent reflectivity spectra structure for both transverse electric (TE) and transverse magnetic (TM) polarizations confirm the predicted theoretical model. We obtained a giant value of the polarization splitting of up to 180 meV for both polariton branches. We believe that it is the first demonstration of such peculiar polarization splitting behavior of polaritons in the ultrastrong coupling regime.
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| 3. |
- Pozina, Galia, et al.
(författare)
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Nonlinear behavior of the emission in the periodic structure of InAs monolayers embedded in a GaAs matrix
- 2017
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Ingår i: Physica status solidi. B, Basic research. - : WILEY-V C H VERLAG GMBH. - 0370-1972 .- 1521-3951. ; 254:4
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Tidskriftsartikel (refereegranskat)abstract
- We report time-resolved photoluminescence (TRPL) measurements performed at different temperatures for the Bragg structure containing 60 InAs monolayer-based quantum wells (QWs) periodically arranged in a GaAs matrix. TRPL data reveal an appearance of the additional superradiant (SR) mode originated from coherent collective interaction of QWs. The SR mode is not manifested in the case if a small number of QWs is excited, then only an exciton emission related to the InAs QWs dominates the PL spectrum. The SR mode demonstrates a superlinear dependence of the intensity and radiative decay rate on the excitation power and its intensity increases at elevated temperatures compared to the excitonic emission. The photoluminescence delay time is much shorter for the SR mode indicating that the relaxation of hot excitons can occur via stimulated scattering processes. The specific behavior of the SR emission can have a strong potential for different applications such as optical logic devices, superluminescent diodes, optical switches, and low-threshold lasers. Time-resolved photoluminescence image at low temperature for the Bragg structure consisting of InAs monolayer-based quantum wells (inset).
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| 4. |
- Girshova, Elizaveta I, et al.
(författare)
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Proposal for a photoacoustic ultrasonic generator based on Tamm plasmon structures
- 2020
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Ingår i: Optics Express. - : OPTICAL SOC AMER. - 1094-4087. ; 28:18, s. 26161-26169
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Tidskriftsartikel (refereegranskat)abstract
- The scheme of a generation of ultrasound waves based on optically excited Tamm plasmon structures is proposed. It is shown that Tamm plasmon structures can provide total absorption of a laser pulse with arbitrary wavelength in a metallic layer providing the possibility of the use of an infrared semiconductor laser for the excitation of ultrasound waves. Laser pulse absorption, heat transfer and dynamical properties of the structure are modeled, and the optimal design of the structure is found. It is demonstrated that the Tamm plasmon-based photoacoustic generator can emit ultrasound waves in the frequency band up to 100 MHz with predefined frequency spectrum. (C) 2020 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
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| 5. |
- Ivanov, Konstantin A., et al.
(författare)
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Control of the surface plasmon dispersion and Purcell effect at the metamaterial-dielectric interface
- 2020
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Ingår i: Scientific Reports. - : NATURE RESEARCH. - 2045-2322. ; 10:1
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Tidskriftsartikel (refereegranskat)abstract
- The use of metamaterial as a way to mitigate the negative effects of absorption in metals on the Purcell effect in metal-dielectric structures is investigated. A layered metal-dielectric structure is considered as an anisotropic medium in the long-wavelength limit. The dispersion of the surface plasmon appearing at the boundary between such a structure and a different dielectric material, as well as the position of the peak in the local density of states are studied for various combinations of materials and filling factors of the periodic structure. The calculated frequency dependence of the Purcell factor demonstrates an increase in peak value compared to the conventional plasmonic structure. The results obtained using effective media approach are compared to the results of numerical modelling.
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| 6. |
- Morozov, Konstantin M., et al.
(författare)
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Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
- 2019
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Ingår i: Scientific Reports. - : NATURE PUBLISHING GROUP. - 2045-2322. ; 9
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Tidskriftsartikel (refereegranskat)abstract
- Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 105. However, the role of absorption in real metals has not been thoroughly considered. We provide a theoretical analysis showing that absorption leads to diminishing values of Purcell factor. We also suggest that using emitting organic compounds such as CBP (4,4-Bis(N-carbazolyl)-1,1-biphenyl) can lead to a moderate increase of about an order of magnitude in the Purcell factor. Defining the experimentally measured Purcell factor as a ratio between the excited state lifetimes in bare CBP and in periodic structure, this increase in the fabricated periodic structure is demonstrated through a 4-8 times decrease in excited state radiative lifetime compared to a bare organic material in a wide emission spectrum.
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| 7. |
- Pozina, Galia, et al.
(författare)
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Emission Properties of GaN Planar Hexagonal Microcavities
- 2020
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Ingår i: Physica Status Solidi (a) applications and materials science. - : WILEY-V C H VERLAG GMBH. - 1862-6300 .- 1862-6319. ; 217:14
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Tidskriftsartikel (refereegranskat)abstract
- Fabrication of microcavities based on III-nitrides is challenging due to difficulties with the coherent growth of heterostructures having a large number of periods, at the same time keeping a good precision in terms of thickness and composition of the alloy. A planar design for GaN microresonators supporting whispering gallery modes is suggested. GaN hexagonal microstructures are fabricated by selective-area metalorganic vapor phase epitaxy using focused ion beam for mask patterning. Low-temperature cathodoluminescence spectra measured with a high spatial resolution demonstrate two dominant emission lines in the near bandgap region. These lines merge at room temperature into a broad emission band peaking at approximate to 3.3 eV, which is shifted toward lower energies compared with the reference excitonic spectrum measured for the GaN layer. A numerical analysis of exciton-polariton modes shows that some strongly localized cavity modes can have high Purcell coefficients and can strongly interact with the GaN exciton.
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| 8. |
- Pozina, Galia, et al.
(författare)
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Enhancement of light emission in Bragg monolayer-thick quantum well structures
- 2019
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Ingår i: Scientific Reports. - : NATURE PUBLISHING GROUP. - 2045-2322. ; 9
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Tidskriftsartikel (refereegranskat)abstract
- Control over spontaneous emission rate is important for improving efficiency in different semiconductor applications including lasers, LEDs and photovoltaics. Usually, an emitter should be placed inside the cavity to increase the spontaneous emission rate, although it is technologically challenging. Here we experimentally demonstrate a phenomenon of super-radiance observed in a cavity-less periodic Bragg structure based on InAs monolayer-thick multiple quantum wells (MQW). The collective super-radiant mode shows enhanced emission rate for specific angles and frequencies. This behaviour correlates with the calculations demonstrating individual spots of the enhanced Purcell coefficient near the Bragg condition curve. This study provides a perspective for realization of surface emitting cavity-less lasers with distributed feedback.
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| 9. |
- Pozina, Galia, et al.
(författare)
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Optical Cavity Based on GaN Planar Nanowires Grown by Selective Area Metal-Organic Vapor Phase Epitaxy
- 2019
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Ingår i: Physica status solidi. B, Basic research. - : WILEY-V C H VERLAG GMBH. - 0370-1972 .- 1521-3951. ; 256:6
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Tidskriftsartikel (refereegranskat)abstract
- GaN planar nanowires (NWs) are fabricated by selective area metal-organic vapor phase epitaxy using focused ion beam etching of trench pattern in the Si3N4 mask. Two crystallographic orientations of NWs along [1120] and [1010] directions are investigated. The coherent growth is confirmed for both directions; however, the best morphology, crystalline and optical properties are found in the GaN planar NWs fabricated along the [1010] axis. Cathodoluminescence (CL) at 5K reveals a presence of Fabry-Perot modes in the region of 1.8-2.5 eV for the NWs fabricated in the [1010] direction. The position and intensity of the Fabry-Perot peaks vary depending on measured point within the NW, which is explained by the model based on the Purcell coefficient calculations. It is shown that small fluctuations in the NW thickness cause a noticeable shift of the Fabry-Perot modes energies, while the enhancement or reduction of the emission intensity for the Fabry-Perot peaks depend on the position of the emitter inside the planar NW.
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| 10. |
- Pozina, Galia, et al.
(författare)
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Purcell Effect and Nonlinear Behavior of the Emission in a Periodic Structure Composed of InAs Monolayers Embedded in a GaAs Matrix
- 2019
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Ingår i: Annalen der Physik. - : WILEY-V C H VERLAG GMBH. - 0003-3804 .- 1521-3889. ; 531:6
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Tidskriftsartikel (refereegranskat)abstract
- Enhancement of spontaneous emission in a resonant Bragg quantum well (QW) structure with 60 periods of triple InAs monolayers embedded in a GaAs matrix is studied experimentally and theoretically. From measurements of the time-resolved photoluminescence, besides the QW exciton at 1.47 eV, a specific super-radiant (SR) emission demonstrating nonlinear properties is found. The SR mode shows a near-quadratic dependence of intensity on excitation power, while its energy position follows the Bragg condition. It is revealed that the SR mode shows a peculiar non-monotonic dependence of intensity on direction, with a maximum observed at approximately 40 degrees. The enhancement in the SR emission at a specific direction is correlated well with suggested theoretical consideration of the modal Purcell factor for periodic quantum well structures.
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