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- Ciancio, Regina, 1978, et al.
(författare)
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Atomic structure of functional interfaces in Sr2RuO4/Sr3Ru2O7 eutectic crystals
- 2009
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Ingår i: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 95:14, s. 142507 (artno)-
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Tidskriftsartikel (refereegranskat)abstract
- Sr2RuO4/Sr3Ru2O7 eutectic system is investigated by transmission electron microscopy (TEM) and high angle annular dark field scanning TEM (STEM). The Sr2RuO4/Sr3Ru2O7 lamellar structure allows studying tunneling and proximity effects between spin-triplet superconductor Sr2RuO4 and metamagnetic normal metal Sr3Ru2O7. Our analyses reveal two typologies of interfaces within the eutectic: interfaces parallel to the growth direction are sharp and defect-free whereas interfaces perpendicular to the growth direction appear wavy and decorated with Ru precipitates. These results indicate that interfaces parallel to the growth direction are the best candidates for Sr2RuO4/Sr3Ru2O7 natural junctions to study the unusual superconductivity of Sr2RuO4. (C) 2009 American Institute of Physics. [doi: 10.1063/1.3243691]
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| 3. |
- Ciancio, Regina, 1978, et al.
(författare)
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Toward intrinsic functionalities of bilayered ruthenate Sr3Ru2O7
- 2009
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Ingår i: Physical Review B - Condensed Matter and Materials Physics. - 2469-9950 .- 2469-9969. ; 80:5, s. 054110 (artno)-
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Tidskriftsartikel (refereegranskat)abstract
- Polymorphic materials are known for being prone to intergrowth. Remarkable examples are strontium ruthenates whose properties are dramatically tuned by impurities and disorder. In particular, Sr3Ru2O7 shows a strong variation in transport and magnetic properties depending on synthesis process. It is therefore crucial to correlate atomic structure and properties to identify the functionalities of individual nanostructural constituents. We report a comparative study between Sr3Ru2O7 crystals grown as single phase and in Sr3Ru2O7-Sr2RuO4 eutectics. Our analysis by transmission electron microscopy reveals that Sr3Ru2O7 domains of the eutectic have a significantly lower level of impurities compared to Sr3Ru2O7 single-phase crystals, where intergrowths of Sr4Ru3O10 and SrRuO3 phase are seen. This is confirmed by magnetic measurements. These results identify the eutectic solidification as a fruitful way to grow highly pure crystals of polymorphic materials which, in combination with recent technological developments allowing the extraction of embedded features of crystals, opens a pathway for understanding of their physical properties and applications.
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| 4. |
- Fittipaldi, R., et al.
(författare)
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Superconductivity in Sr2RuO4-Sr3Ru2O7 eutectic crystals
- 2008
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Ingår i: Europhysics Letters. - : IOP Publishing. - 0295-5075 .- 1286-4854. ; 83:2, s. Art. no. 27007-
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Tidskriftsartikel (refereegranskat)abstract
- Superconducting behavior has been observed in the Sr2RuO4-Sr3Ru2O7 eutectic system as grown by the flux-feeding floating-zone technique. A supercurrent flows across a single interface between Sr2RuO4 and Sr3Ru2O7 areas at distances that are far beyond those expected in a conventional proximity effect. The current-voltage characteristics within the Sr3Ru2O7 macrodomain, as extracted from the eutectic, exhibit signatures of superconductivity in the bilayered Sr3Ru2O7 region. Detailed microstructural, morphological and compositional analyses address issues on the concentration and the size of Sr2RuO4 inclusions within the Sr3Ru2O7 matrix. We speculate on the possibility of inhomogeneous superconductivity in the eutectic Sr3Ru2O7 and exotic pairing induced by the Sr2RuO4 inclusions. Copyright (C) EPLA, 2008.
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