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Sökning: WFRF:(Knorr W.)

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  • Allison, David B, et al. (författare)
  • Goals in Nutrition Science 2015-2020.
  • 2015
  • Ingår i: Frontiers in nutrition. - : Frontiers Media SA. - 2296-861X. ; 2
  • Tidskriftsartikel (refereegranskat)
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4.
  • Dong, Shuo, et al. (författare)
  • Direct measurement of key exciton properties: Energy, dynamics, and spatial distribution of the wave function
  • 2021
  • Ingår i: Natural Sciences. - : Wiley. - 2698-6248. ; 1:1
  • Tidskriftsartikel (refereegranskat)abstract
    • Excitons, Coulomb-bound electron–hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. Although optical signatures of excitons have been studied extensively, experimental access to the excitonic wave function itself has been elusive. Using multidimensional photoemission spectroscopy, we present a momentum-, energy-, and time-resolved perspective on excitons in the layered semiconductor WSe2. By tuning the excitation wavelength, we determine the energy–momentum signature of bright exciton formation and its difference from conventional single-particle excited states. The multidimensional data allow to retrieve fundamental exciton properties like the binding energy and the exciton–lattice coupling and to reconstruct the real-space excitonic distribution function via Fourier transform. All quantities are in excellent agreement with microscopic calculations. Our approach provides a full characterization of the exciton properties and is applicable to bright and dark excitons in semiconducting materials, heterostructures, and devices. Key points: The full life cycle of excitons is recorded with time- and angle-resolved photoemission spectroscopy. The real-space distribution of the excitonic wave function is visualized. Direct measurement of the exciton-phonon interaction.
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5.
  • Kaminski, T., et al. (författare)
  • An interactive tool to analyse the benefit of space missions sensing the terrestrial vegetation
  • 2012
  • Ingår i: ; , s. 4883-4886
  • Konferensbidrag (refereegranskat)abstract
    • The study has developed an interactive mission benefit analysis (MBA) tool that allows instantaneous evaluation of a range of potential mission designs. The designs are evaluated in terms of their constraint on carbon and water fluxes through calibration of a terrestrial bisphere model. The constraint is quantified by methematically rigorous uncertainty propagation in CCDAS. Applying the MBA tool, the study showed that the benefit of FAPAR data is most pronounced for hydrological quantities and moderate for quantities related to carbon fluxes from ecosystems. In semi-arid regions, where vegetation is strongly water limited, the constraint delivered by FAPAR for hydrological quantities was especially large, as documented by the results for Africa and Australia. Sensor resolution is less critical for successful data assimilation, and with even relatively short time series of only a few years, significant uncertainty reduction can be achieved.
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6.
  • Kaminski, T., et al. (författare)
  • Constraining a terrestrial biosphere model with remotely sensed atmospheric carbon dioxide
  • 2017
  • Ingår i: Remote Sensing of Environment. - : Elsevier BV. - 0034-4257. ; 203, s. 109-124
  • Tidskriftsartikel (refereegranskat)abstract
    • We present two novel earth observation products derived from the BESD and EMMA XCO2 products which were respectively retrieved from SCIAMACHY and GOSAT observations within the GreenHouse Gas project of ESA's Climate Change Initiative (GHG-CCI). These products are inferred by a Carbon Cycle Data Assimilation System (CCDAS) and consist of net and gross biosphere-atmosphere fluxes of carbon dioxide on a global 0.5° grid. As a further dataset provided by the CCI, the burnt area product developed by its Fire忌i project was used in the CCDAS to prescribe the emission component from biomass burning. The new flux products are provided with per-pixel uncertainty ranges. Fluxes with uncertainty ranges can also be provided aggregated in space and time, e.g. over given regions or as annual means. For both, posterior flux fields inferred from BESD and EMMA products, transport model simulations show reasonable agreement with the atmospheric carbon dioxide concentration observed at flask sampling stations. This means that the information provided by the terrestrial and transport models, the respective GHG ECV product, the burnt area ECV product, a product of the Fraction of Absorbed Photosynthetically Active Radiation used to drive the model, and the atmospheric flask samples is largely consistent. The most prominent feature in the posterior net flux is the tropical source of CO2 inferred from both products. But for the EMMA product this release, especially over South America, is with 300 gC/m2/year much more pronounced than for BESD. This confirms findings by a recent intercomparison of transport inversions using GOSAT data by Houweling et al. (2015). The reason for the larger net flux is increased heterotrophic respiration. For both products the posterior 2010 sink over Europe (without Russia) is in the range of a recent compilation of European flux estimates by Reuter et al. (2016b). The posterior 2010 uptake of Australia (including Oceania) inferred from the EMMA product is 1.3 ± 0.2 PgC/year and appears to confirm the high sink also derived from GOSAT by Detmers et al. (2015) over a slightly different period and area. While for some regions (USA, Canada, Europe, Russia, Asia) the one standard deviation uncertainty ranges derived from BESD and EMMA do overlap, for some other regions (Brazil, Africa, Australia) this is not the case. It is not clear yet whether this is due to the uncertainty specifications in the respective products or the handling of uncertainty in the assimilation chain. Assumptions on correlation of observational uncertainty in space and time have a considerable impact on the inferred flux fields (≈ 60 gC/m2/year). The effect of adding an uncertainty that approximates the error in the retrieval system is of similar size.
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7.
  • Kaminski, T., et al. (författare)
  • Constraining terrestrial carbon fluxes through assimilation of SMOS products
  • 2018
  • Ingår i: 2018 IEEE International Geoscience and Remote Sensing Symposium, IGARSS 2018 - Proceedings. - 9781538671504 ; 2018-July, s. 1455-1458
  • Konferensbidrag (refereegranskat)abstract
    • The ongoing ESA funded'SMOS + Vegetation' project combines a retrieval component that aims at further improving the SMOS VOD product with an assimilation component that aims at demonstrating the added value of this product in constraining simulated land surface fluxes of carbon dioxide. This contribution focuses on the project's modelling and assimilation component. We describe the construction of dedicated observation operators that link the state of the terrestrial biosphere model to simulated VOD and surface layer soil moisture. We present our carbon assimilation system around a terrestrial biosphere model and demonstrate its operation through simultaneous assimilation of the SMOS VOD product over seven sites covering a range of plant functional types.
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8.
  • Kaminski, T., et al. (författare)
  • The BETHY/JSBACH Carbon Cycle Data Assimilation System: experiences and challenges
  • 2013
  • Ingår i: Journal of Geophysical Research - Biogeosciences. - : American Geophysical Union (AGU). - 2169-8953. ; 118:4, s. 1414-1426
  • Forskningsöversikt (refereegranskat)abstract
    • We present the concept of the Carbon Cycle Data Assimilation System and describe its evolution over the last two decades from an assimilation system around a simple diagnostic model of the terrestrial biosphere to a system for the calibration and initialization of the land component of a comprehensive Earth system model. We critically review the capability of this modeling framework to integrate multiple data streams, to assess their mutual consistency and with the model, to reduce uncertainties in the simulation of the terrestrial carbon cycle, to provide, in a traceable manner, reanalysis products with documented uncertainty, and to assist the design of the observational network. We highlight some of the challenges we met and experience we gained, give recommendations for operating the system, and suggest directions for future development.
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9.
  • Knorr, W., et al. (författare)
  • Climate, CO2 and human population impacts on global wildfire emissions
  • 2016
  • Ingår i: Biogeosciences. - : Copernicus GmbH. - 1726-4170 .- 1726-4189. ; 13:1, s. 267-282
  • Tidskriftsartikel (refereegranskat)abstract
    • Wildfires are by far the largest contributor to global biomass burning and constitute a large global source of atmospheric traces gases and aerosols. Such emissions have a considerable impact on air quality and constitute a major health hazard. Biomass burning also influences the radiative balance of the atmosphere and is thus not only of societal, but also of significant scientific interest. There is a common perception that climate change will lead to an increase in emissions as hot and dry weather events that promote wildfire will become more common. However, even though a few studies have found that the inclusion of CO2 fertilisation of photosynthesis and changes in human population patterns will tend to somewhat lower predictions of future wildfire emissions, no such study has included full ensemble ranges of both climate predictions and population projections, including the effect of different degrees of urbanisation. Here, we present a series of 124 simulations with the LPJ-GUESS-SIMFIRE global dynamic vegetation-wildfire model, including a semi-empirical formulation for the prediction of burned area based on fire weather, fuel continuity and human population density. The simulations use Climate Model Intercomparison Project 5 (CMIP5) climate predictions from eight Earth system models. These were combined with two Representative Concentration Pathways (RCPs) and five scenarios of future human population density based on the series of Shared Socioeconomic Pathways (SSPs) to assess the sensitivity of emissions to the effect of climate, CO2 and humans. In addition, two alternative parameterisations of the semi-empirical burned-area model were applied. Contrary to previous work, we find no clear future trend of global wildfire emissions for the moderate emissions and climate change scenario based on the RCP 4.5. Only historical population change introduces a decline by around 15% since 1900. Future emissions could either increase for low population growth and fast urbanisation, or continue to decline for high population growth and slow urbanisation. Only for high future climate change (RCP8.5), wildfire emissions start to rise again after ca. 2020 but are unlikely to reach the levels of 1900 by the end of the 21st century. We find that climate warming will generally increase the risk of fire, but that this is only one of several equally important factors driving future levels of wildfire emissions, which include population change, CO2 fertilisation causing woody thickening, increased productivity and fuel load and faster litter turnover in a warmer climate.
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