| 1. |
- Lan, Changxing, et al.
(författare)
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Intercomparison of eddy-covariance software for urban tall-tower sites
- 2024
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Ingår i: Atmospheric Measurement Techniques. - 1867-1381. ; 17:9, s. 2649-2669
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Tidskriftsartikel (refereegranskat)abstract
- Long-term tall-tower eddy-covariance (EC) measurements have been recently established in three European pilot cities as part of the ICOS-Cities project. We conducted a comparison of EC software to ensure a reliable generation of interoperable flux estimates, which is the prerequisite for avoiding methodological biases and improving the comparability of the results. We analyzed datasets covering 5 months collected from EC tall-tower installations located in urbanized areas of Munich, Zurich, and Paris. Fluxes of sensible heat, latent heat, and CO2 were calculated using three software packages (i.e., TK3, EddyPro, and eddy4R) to assess the uncertainty of flux estimations attributed to differences in implemented postprocessing schemes. A very good agreement on the mean values and standard deviations was found across all three sites, which can probably be attributed to a uniform instrumentation, data acquisition, and preprocessing. The overall comparison of final flux time series products showed a good but not yet perfect agreement among the three software packages. TK3 and EddyPro both calculated fluxes with low-frequency spectral correction, resulting in better agreement than between TK3 and the eddy4R workflow with disabled low-frequency spectral treatment. These observed flux discrepancies indicate the crucial role of treating low-frequency spectral loss in flux estimation for tall-tower EC systems.
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| 2. |
- Personne, Erwan, et al.
(författare)
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SURFATM-NH3 : a model combining the surface energy balance and bi-directional exchanges of ammonia applied at the field scale
- 2009
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Ingår i: Biogeosciences. - Göttingen, Germany : Copernicus Publications. - 1726-4170 .- 1726-4189. ; 6:8, s. 1371-1388
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Tidskriftsartikel (refereegranskat)abstract
- A new biophysical model SURFATM-NH3, simulating the ammonia (NH3) exchange between terrestrial ecosystems and the atmosphere is presented. SURFATM-NH3 consists of two coupled models: (i) an energy budget model and (ii) a pollutant exchange model, which distinguish the soil and plant exchange processes. The model describes the exchanges in terms of adsorption to leaf cuticles and bi-directional transport through leaf stomata and soil. The results of the model are compared with the flux measurements over grassland during the GRAMINAE Integrated Experiment at Braunschweig, Germany. The dataset of GRAMINAE allows the model to be tested in various meteorological and agronomic conditions: prior to cutting, after cutting and then after the application of mineral fertilizer. The whole comparison shows close agreement between model and measurements for energy budget and ammonia fluxes. The major controls on the ground and plant emission potential are the physicochemical parameters for liquid-gas exchanges which are integrated in the compensation points for live leaves, litter and the soil surface. Modelled fluxes are highly sensitive to soil and plant surface temperatures, highlighting the importance of accurate estimates of these terms. The model suggests that the net flux depends not only on the foliar (stomatal) compensation point but also that of leaf litter. SURFATM-NH3 represents a comprehensive approach to studying pollutant exchanges and its link with plant and soil functioning. It also provides a simplified generalised approach (SVAT model) applicable for atmospheric transport models.
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| 3. |
- Schallhart, Simon, et al.
(författare)
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Characterization of total ecosystem-scale biogenic VOC exchange at a Mediterranean oak–hornbeam forest
- 2016
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Ingår i: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7324. ; 16:11, s. 7171-7194
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Tidskriftsartikel (refereegranskat)abstract
- Recently, the number and amount of biogenically emitted volatile organic compounds (VOCs) has been discussed in great detail. Depending on the ecosystem, the published number varies between a dozen and several hundred compounds. We present ecosystem exchange fluxes from a mixed oak–hornbeam forest in the Po Valley, Italy. The fluxes were measured by a proton transfer reaction-time-of-flight (PTR-ToF) mass spectrometer and calculated using the eddy covariance (EC) method. Detectable fluxes were observed for up to 29 compounds, dominated by isoprene, which comprised over 60 % of the total upward flux (on a molar basis). The daily average of the total VOC upward flux was 10.4 nmol m−2 s−1. Methanol had the highest concentration and accounted for the largest downward flux. Methanol seemed to be deposited to dew, as the downward flux happened in the early morning, right after the calculated surface temperature came closest to the calculated dew point temperature.We estimated that up to 30 % of the upward flux of methyl vinyl ketone (MVK) and methacrolein (MACR) originated from atmospheric oxidation of isoprene. A comparison between two methods for the flux detection (manual and automated) was made. Their respective advantages and disadvantages were discussed and the differences in their results shown. Both provide comparable results.
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| 4. |
- Sutton, Mark A., et al.
(författare)
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Dynamics of ammonia exchange with cut grassland : Synthesis of results and conclusions of the GRAMINAE Integrated Experiment
- 2009
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Ingår i: Biogeosciences. - Goettingen : Nicolaus Copernicus University Press. - 1726-4170 .- 1726-4189. ; 6:12, s. 2907-2934
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Tidskriftsartikel (refereegranskat)abstract
- Improved data on biosphere-atmosphere exchange are fundamental to understanding the production and fate of ammonia (NH3) in the atmosphere. The GRAMINAE Integrated Experiment combined novel measurement and modelling approaches to provide the most comprehensive analysis of the interactions to date. Major intercomparisons of micrometeorological parameters and NH3 flux measurements using the aerodynamic gradient method and relaxed eddy accumulation (REA) were conducted. These showed close agreement, though the REA systems proved insufficiently precise to investigate vertical flux divergence. Grassland management had a large effect on fluxes: emissions increased after grass cutting (−50 to 700 ng m-2 s-1 NH3) and after N-fertilization (0 to 3800 ng m-2 s -1) compared with before the cut (−60 to 40 ng m-2 s -1). © Author(s) 2009.
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| 5. |
- Tang, Angela Che Ing, et al.
(författare)
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Detection and attribution of an anomaly in terrestrial photosynthesis in Europe during the COVID-19 lockdown
- 2023
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Ingår i: Science of the Total Environment. - 0048-9697 .- 1879-1026. ; 903
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Tidskriftsartikel (refereegranskat)abstract
- Carbon dioxide (CO2) uptake by plant photosynthesis, referred to as gross primary production (GPP) at the ecosystem level, is sensitive to environmental factors, including pollutant exposure, pollutant uptake, and changes in the scattering of solar shortwave irradiance (SWin) − the energy source for photosynthesis. The 2020 spring lockdown due to COVID-19 resulted in improved air quality and atmospheric transparency, providing a unique opportunity to assess the impact of air pollutants on terrestrial ecosystem functioning. However, detecting these effects can be challenging as GPP is influenced by other meteorological drivers and management practices. Based on data collected from 44 European ecosystem-scale CO2 flux monitoring stations, we observed significant changes in spring GPP at 34 sites during 2020 compared to 2015–2019. Among these, 14 sites showed an increase in GPP associated with higher SWin, 10 sites had lower GPP linked to atmospheric and soil dryness, and seven sites were subjected to management practices. The remaining three sites exhibited varying dynamics, with one experiencing colder and rainier weather resulting in lower GPP, and two showing higher GPP associated with earlier spring melts. Analysis using the regional atmospheric chemical transport model (LOTOS-EUROS) indicated that the ozone (O3) concentration remained relatively unchanged at the research sites, making it unlikely that O3 exposure was the dominant factor driving the primary production anomaly. In contrast, SWin increased by 9.4 % at 36 sites, suggesting enhanced GPP possibly due to reduced aerosol optical depth and cloudiness. Our findings indicate that air pollution and cloudiness may weaken the terrestrial carbon sink by up to 16 %. Accurate and continuous ground-based observations are crucial for detecting and attributing subtle changes in terrestrial ecosystem functioning in response to environmental and anthropogenic drivers.
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| 6. |
- Yi, Chuixiang, et al.
(författare)
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Climate control of terrestrial carbon exchange across biomes and continents
- 2010
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Ingår i: Environmental Research Letters. - : IOP Publishing. - 1748-9326. ; 5:3
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Tidskriftsartikel (refereegranskat)abstract
- Understanding the relationships between climate and carbon exchange by terrestrial ecosystems is critical to predict future levels of atmospheric carbon dioxide because of the potential accelerating effects of positive climate-carbon cycle feedbacks. However, directly observed relationships between climate and terrestrial CO2 exchange with the atmosphere across biomes and continents are lacking. Here we present data describing the relationships between net ecosystem exchange of carbon (NEE) and climate factors as measured using the eddy covariance method at 125 unique sites in various ecosystems over six continents with a total of 559 site-years. We find that NEE observed at eddy covariance sites is (1) a strong function of mean annual temperature at mid-and high-latitudes, (2) a strong function of dryness at mid-and low-latitudes, and (3) a function of both temperature and dryness around the mid-latitudinal belt (45 degrees N). The sensitivity of NEE to mean annual temperature breaks down at similar to 16 degrees C (a threshold value of mean annual temperature), above which no further increase of CO2 uptake with temperature was observed and dryness influence overrules temperature influence.
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