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Sökning: WFRF:(Nordblad F.)

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  • Garg, K. B., et al. (författare)
  • Study of Sb substitution for Pr in the Pr0.67Ba0.33MnO3 system
  • 2009
  • Ingår i: Journal of Magnetism and Magnetic Materials. - : Elsevier BV. - 0304-8853 .- 1873-4766. ; 321:4, s. 305-311
  • Tidskriftsartikel (refereegranskat)abstract
    • We study the effect of Sb substitution for Pr in the hole-doped system Pr0.67Ba0.33MnO3 (PBMO) for different doping levels of Sb. The two electrical resistivity transitions observed in the pristine sample PBMO shift to low temperatures on Sb doping with an overall increase in the electrical resistivity. The significant local lattice distortion and the grain boundary effects caused by the large cation size mismatch between Pr3+ and Sb3+ suppresses the double-exchange (DE) interaction and enhances the super-exchange (SE) interaction. The compounds show a significant and increasing value of magnetoresistance at temperatures below the Curie temperature, not expected from the DE model. The Curie temperature decreases with increase in Sb content but the saturation magnetization is little affected by the substitution. The spins, however, stay well aligned in the low-temperature regime. Our X-ray near-edge absorption spectra (XANES) and core level photoemission (XPS) data clearly show the Sb cation to be in +3 state and rule out any possibility of e-doping in our compounds.
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3.
  • Andersson, P.S., et al. (författare)
  • The importance of river water inflow and shelf sediment-sea water exchange in the East Siberian Sea for the Nd isotopic composition of Arctic Ocean water
  • 2009
  • Ingår i: Geochimica et Cosmochimica Acta. - 0016-7037 .- 1872-9533. ; 73:13, Suppl. 1, s. A41-
  • Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
    • With data generated from cruises to the Canada Basin in 2000, to the Eurasian and Central Arctic Ocean basins in 2001, to the Fram Strait in 2002 and to the Chuckchi Sea in 2005 we now have a good general view of the distribution and isotopic composition of Nd (εNd) in the Arctic Ocean [1, 2]. The restricted Arctic Ocean basin is surrounded by large continental shelves, covering more than 50% of its total area.Distinct from other oceans, with surface water Nd depletion, there is throughout the Arctic a pattern of high Nd concentrations, up to 58pM, at the surface that gradually diminish with depth to 15-18pM in the deep waters. A range of isotopic variations across the Arctic and within individual depth profiles reflects the different sources of waters. The dominant source of water and Nd is the Atlantic (εNd= -10.7). Radiogenic isotope Nd signatures can be traced in Pacific water flowing into the Canada Basin and further into the Eurasian Basin (up to εNd= -6.5). The variation of εNd and concentration in the Arctic Ocean suggest that Nd input from rivers and shelf sediments is also of great importance.Improving our understanding of the vast Siberian Shelves influence on Nd and trace element behaviour in the Arctic Ocean was one of the main objectives of the International Siberian Shelf Study 2008 (ISSS-08). The ISSS-08 cruise recovered filtered water (<0.2µm), particles and sediments from the Laptev and East Siberian Seas as well as estuarine and river water from Lena, Indigirka and Kolyma. Crucial processes, including loss of river water Nd in the estuarine region and shelf sediment-sea water exchange will be discussed in terms of controlling the Nd concentration and isotopic composition of sea water.[1] Andersson et al. (2008) GCA 72, 2854-2867. [2] Porcelli et al. (2009, in press) GCA. (2009, in press)
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  • De Toro, J. A., et al. (författare)
  • A nanoparticle replica of the spin-glass state
  • 2013
  • Ingår i: Applied Physics Letters. - : AIP Publishing. - 0003-6951 .- 1077-3118. ; 102:18, s. 183104-
  • Tidskriftsartikel (refereegranskat)abstract
    • A simple single-phase material, a random close-packed (volume fraction 67%) ensemble of highly monodisperse bare maghemite (gamma-Fe2O3) nanoparticles, is shown to exhibit ideal superspin-glass behavior (mimicking that of model spin-glasses), namely, an unprecedentedly sharp onset of the absorption component of the ac susceptibility, narrow memory dips in the zero-field-cooled magnetization and a spin-glass characteristic field-dependence of the magnetic susceptibility. This ideal behavior is attributed to the remarkably narrow dispersion in particle size and to the highly dense and spatially homogeneous configuration ensured by the random close-packed arrangement. This material is argued to constitute the closest nanoparticle analogue to a conventional (atomic) magnetic state found to date. 
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  • Hansen, M. F., et al. (författare)
  • Critical dynamics of an interacting magnetic nanoparticle system
  • 2002
  • Ingår i: Journal of Physics. - : IOP Publishing. - 0953-8984 .- 1361-648X. ; 14:19, s. 4901-
  • Tidskriftsartikel (refereegranskat)abstract
    • Effects of dipole-dipole interactions on the magnetic relaxation have been investigated for three Fe-C nanoparticle samples with volume concentrations of 0.06, 5 and 17 vol%. While both the 5 and 17 vol% samples exhibit collective behaviour due to dipolar interactions, only the 17 vol% sample displays critical behaviour close to its transition temperature. The behaviour of the 5 vol% sample can be attributed to a mixture of collective and single-particle dynamics.
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  • HUDNER, J, et al. (författare)
  • PREPARATION OF YBA2CU3O7-X FILMS AND YBA2CU3O7-X/Y2O3 MULTILAYERS USING COEVAPORATION AND ATOMIC OXYGEN
  • 1993
  • Ingår i: Journal of Applied Physics. - : AIP Publishing. - 0021-8979 .- 1089-7550. ; 73, s. 3096-3098
  • Tidskriftsartikel (refereegranskat)abstract
    • Thin layers of YBa2Cu3O7-x (YBCO) deposited on LaAlO3 substrates have been prepared in situ by coevaporation of Y, Ba, and Cu. Incorporation of oxygen was accomplished by an atomic oxygen beam source with high cracking efficiency. The total oxygen flow at the substrate could be kept low enough to permit the use of a quadrupole mass spectrometer for evaporation rate monitoring. Films were strongly c-axis oriented with rocking curve full width at half-maximum values of 0.6-degrees. Transport measurements on patterned films yielded critical current densities of 6 x 10(6) A/cm2 at 77 K. The deposition method was demonstrated to be feasible for preparation of Y2O3/YBCO heterostructures.
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