| 1. |
- Saunois, M., et al.
(författare)
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The global methane budget 2000–2012
- 2016
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Ingår i: Earth System Science Data. - : Copernicus GmbH. - 1866-3508 .- 1866-3516. ; 8:2, s. 697-751
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Tidskriftsartikel (refereegranskat)abstract
- The global methane (CH4) budget is becoming an increasingly important component for managing realistic pathways to mitigate climate change. This relevance, due to a shorter atmospheric lifetime and a stronger warming potential than carbon dioxide, is challenged by the still unexplained changes of atmospheric CH4 over the past decade. Emissions and concentrations of CH4 are continuing to increase, making CH4 the second most important human-induced greenhouse gas after carbon dioxide. Two major difficulties in reducing uncertainties come from the large variety of diffusive CH4 sources that overlap geographically, and from the destruction of CH4 by the very short-lived hydroxyl radical (OH). To address these difficulties, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate research on the methane cycle, and producing regular (∼ biennial) updates of the global methane budget. This consortium includes atmospheric physicists and chemists, biogeochemists of surface and marine emissions, and socio-economists who study anthropogenic emissions. Following Kirschke et al. (2013), we propose here the first version of a living review paper that integrates results of top-down studies (exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models, inventories and data-driven approaches (including process-based models for estimating land surface emissions and atmospheric chemistry, and inventories for anthropogenic emissions, data-driven extrapolations). For the 2003–2012 decade, global methane emissions are estimated by top-down inversions at 558 Tg CH4 yr−1, range 540–568. About 60 % of global emissions are anthropogenic (range 50–65 %). Since 2010, the bottom-up global emission inventories have been closer to methane emissions in the most carbon-intensive Representative Concentrations Pathway (RCP8.5) and higher than all other RCP scenarios. Bottom-up approaches suggest larger global emissions (736 Tg CH4 yr−1, range 596–884) mostly because of larger natural emissions from individual sources such as inland waters, natural wetlands and geological sources. Considering the atmospheric constraints on the top-down budget, it is likely that some of the individual emissions reported by the bottom-up approaches are overestimated, leading to too large global emissions. Latitudinal data from top-down emissions indicate a predominance of tropical emissions (∼ 64 % of the global budget, < 30° N) as compared to mid (∼ 32 %, 30–60° N) and high northern latitudes (∼ 4 %, 60–90° N). Top-down inversions consistently infer lower emissions in China (∼ 58 Tg CH4 yr−1, range 51–72, −14 %) and higher emissions in Africa (86 Tg CH4 yr−1, range 73–108, +19 %) than bottom-up values used as prior estimates. Overall, uncertainties for anthropogenic emissions appear smaller than those from natural sources, and the uncertainties on source categories appear larger for top-down inversions than for bottom-up inventories and models. The most important source of uncertainty on the methane budget is attributable to emissions from wetland and other inland waters. We show that the wetland extent could contribute 30–40 % on the estimated range for wetland emissions. Other priorities for improving the methane budget include the following: (i) the development of process-based models for inland-water emissions, (ii) the intensification of methane observations at local scale (flux measurements) to constrain bottom-up land surface models, and at regional scale (surface networks and satellites) to constrain top-down inversions, (iii) improvements in the estimation of atmospheric loss by OH, and (iv) improvements of the transport models integrated in top-down inversions. The data presented here can be downloaded from the Carbon Dioxide Information Analysis Center (http://doi.org/10.3334/CDIAC/GLOBAL_METHANE_BUDGET_2016_V1.1) and the Global Carbon Project.
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| 2. |
- Aires, F., et al.
(författare)
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Microwave hyperspectral measurements for temperature and humidity atmospheric profiling from satellite: The clear-sky case
- 2015
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Ingår i: Journal of Geophysical Research. - 0148-0227 .- 2156-2202 .- 2169-897X .- 2169-8996. ; 120:21, s. 11334-11351
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Tidskriftsartikel (refereegranskat)abstract
- This study investigates the benefits of a satellite HYperspectral Microwave Sensor (HYMS) for the retrieval of atmospheric temperature and humidity profiles, in the context of numerical weather prediction (NWP). In the infrared, hyperspectral instruments have already improved the accuracy of NWP forecasts. Microwave instruments so far only provide observations for a limited number of carefully selected channels. An information content analysis is conducted here to assess the impact of hyperspectral microwave measurements on the retrieval of temperature and water vapor profiles under clear-sky conditions. It uses radiative transfer simulations over a large variety of atmospheric situations. It accounts for realistic observation (instrument and radiative transfer) noise and for a priori information assumptions compatible with NWP practices. The estimated retrieval performance of the HYMS instrument is compared to those of the microwave instruments to be deployed on board the future generation of European operational meteorological satellites (MetOp-SG). The results confirm the positive impact of a HYMS instrument on the atmospheric profiling capabilities compared to MetOp-SG. Temperature retrieval uncertainty, compared to a priori information, is reduced by 2 to 10%, depending on the atmospheric height, and improvement rates are much higher than what will be obtained with MetOp-SG. For humidity sounding these improvements can reach 30%, a significant benefit as compared to MetOp-SG results especially below 250 hPa. The results are not very sensitive to the instrument noise, under our assumptions. The main impact provided by the hyperspectral information originates from the higher resolution in the O2 band around 60 GHz. The results are presented over ocean at nadir, but similar conclusions are obtained for other incidence angles and over land. Key Points A hyperspectral MW instrument could improve temperature & humidity retrieval compared to MetOp-SG The main impact from HYMS comes from higher resolution in the O2 band around 60 GHz Hyperspectral information is not really sensitive to instrument noise.
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| 3. |
- Buehler, Stefan, et al.
(författare)
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Observing ice clouds in the submillimeter spectral range: the CloudIce mission proposal for ESA's Earth Explorer 8
- 2012
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 5:7, s. 1529-1549
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Tidskriftsartikel (refereegranskat)abstract
- Passive submillimeter-wave sensors are a way to obtain urgently needed global data on ice clouds, particularly on the so far poorly characterized 'essential climate variable' ice water path (IWP) and on ice particle size. CloudIce was a mission proposal to the European Space Agency ESA in response to the call for Earth Explorer 8 (EE8), which ran in 2009/2010. It proposed a passive submillimeter-wave sensor with channels ranging from 183 GHz to 664 GHz. The article describes the CloudIce mission proposal, with particular emphasis on describing the algorithms for the data-analysis of submillimeter-wave cloud ice data (retrieval algorithms) and demonstrating their maturity. It is shown that we have a robust understanding of the radiative properties of cloud ice in the millimeter/submillimeter spectral range, and that we have a proven toolbox of retrieval algorithms to work with these data. Although the mission was not selected for EE8, the concept will be useful as a reference for other future mission proposals.
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| 4. |
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| 5. |
- Charlton, J. E., et al.
(författare)
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A sub-millimetre wave airborne demonstrator for the observation of precipitation and ice clouds
- 2010
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Ingår i: International Geoscience and Remote Sensing Symposium (IGARSS). - Piscataway, NJ : IEEE Communications Society. - 9781424433940 ; , s. 1023-1026
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Konferensbidrag (refereegranskat)abstract
- Sub-millimetre remote sensing instruments can provide critical information on cirrus clouds and an alternative way of measuring precipitation with a much smaller antenna than those which microwave sensors currently use. Two satellite concepts CIWSIR and GOMAS were proposed as ESA Earth Explorer missions; these were not funded, however they were recommended for an aircraft demonstrator. ESA studies have been performed to identify the optimum instrument and platform to demonstrate these satellite concepts. This paper reports on one of these preparatory activities; the design of a sub-millimetre wave airborne demonstrator for both ice cloud and precipitation observations which will be able to prove the feasibility of the scientific principles of both satellite missions. The paper will describe the derivation of the demonstrator requirements, consideration of the available platform and instrument options, the design of the selected concept, performance prediction and the outline of a proof of concept flight campaign. It will present the outcome of the study which describes a demonstrator design based upon the new Met Office International Sub-Millimetre Airborne Radiometer (ISMAR).
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| 6. |
- Galligani, V. S., et al.
(författare)
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Meso-scale modelling and radiative transfer simulations of a snowfall event over France at microwaves for passive and active modes and evaluation with satellite observations
- 2015
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 8:3, s. 1605-1616
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Tidskriftsartikel (refereegranskat)abstract
- Microwave passive and active radiative transfer simulations are performed with the Atmospheric Radiative Transfer Simulator (ARTS) for a mid-latitude snowfall event, using outputs from the Meso-NH mesoscale cloud model. The results are compared to the corresponding microwave observations available from MHS and CloudSat. The spatial structures of the simulated and observed brightness temperatures show an overall agreement since the large-scale dynamical structure of the cloud system is reasonably well captured by Meso-NH. However, with the initial assumptions on the single-scattering properties of snow, there is an obvious underestimation of the strong scattering observed in regions with large frozen hydrometeor quantities. A sensitivity analysis of both active and passive simulations to the microphysical parametrizations is conducted. Simultaneous analysis of passive and active calculations provides strong constraints on the assumptions made to simulate the observations. Good agreements are obtained with both MHS and CloudSat observations when the single-scattering properties are calculated using the 'soft sphere' parametrization from Liu (2004), along with the Meso-NH outputs. This is an important step toward building a robust data set of simulated measurements to train a statistically based retrieval scheme.
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| 7. |
- Galligani, V. S., et al.
(författare)
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The impact of the melting layer on the passive microwave cloud scattering signal observed from satellites: A study using TRMM microwave passive and active measurements
- 2013
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Ingår i: Journal of Geophysical Research. - : American Geophysical Union (AGU). - 0148-0227 .- 2156-2202 .- 2169-897X. ; 118:11, s. 5667-5678
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Tidskriftsartikel (refereegranskat)abstract
- Concurrent passive and active microwave measurements onboard the Tropical Rainfall Measurement Mission (TRMM) show that under cloudy conditions, when a melting layer is detected by the precipitation radar, a polarized scattering signal at 85GHz in passive mode is often observed. Radiative transfer simulations confirm the role of large horizontally oriented non-spherical particles on the polarized scattering signal and assess the effect of changes in particle phase, from solid ice to dry snow to melting snow, on the radiative properties. We conclude on the necessity to account for this polarization generated by the clouds in passive microwave rain retrievals and to use this specific signature to help diagnose the precipitation type and derive more accurate algorithms. In addition, analysis of the passive microwave polarized scattering is a unique way to get insight into microphysical properties of clouds at global scale, and this potential should be explored at millimeter and submillimeter frequencies that are more sensitive to the scattering generated by smaller particles.
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| 8. |
- Mahfouf, J.-F., et al.
(författare)
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Information content on temperature and water vapour from a hyper-spectral microwave sensor
- 2015
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Ingår i: Quarterly Journal of the Royal Meteorological Society. - : Wiley. - 0035-9009 .- 1477-870X. ; 141:693, s. 3268-3284
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Tidskriftsartikel (refereegranskat)abstract
- This study examines the information content on atmospheric temperature and humidity profiles that could be provided by a future spaceborne microwave sensor with a few hundred radiances in the millimetre and submillimetre spectral domains (ranging from 7–800 GHz). A channel selection method based on optimal estimation theory is undertaken, using a database of profiles with associated errors from the European Centre for Medium-Range Weather Forecasts (ECMWF) numerical weather prediction model and the radiative transfer model Atmospheric Radiative Transfer Simulator (ARTS) under clear-sky conditions. The main results indicate that, by increasing the number of channels within the oxygen absorption band around 60 GHz and within the water-vapour absorption band at 183 GHz, the accuracy of temperature and humidity retrievals in the troposphere and stratosphere (for temperature) would be noticeably improved compared with present and planned microwave radiometers. The channels located in the absorption lines at 118 GHz and above 200 GHz do not bring significant additional information regarding atmospheric profiles under clear-sky conditions, partly due to greater radiometric noise. With a set of 137 selected channels that contribute to 90% of the total information content (measured by the degree of freedom for signal), it is possible to achieve almost the same performance in terms of variance error reduction as with 276 candidate channels. Sensitivity studies of various prescribed quantities defining the channel selection have been undertaken, in order to check the robustness of the conclusions. They show that none of the choices modifies the above findings.
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| 9. |
- Fluet-Chouinard, Etienne, et al.
(författare)
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Extensive global wetland loss over the past three centuries
- 2023
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Ingår i: Nature. - : Springer Science and Business Media LLC. - 0028-0836 .- 1476-4687. ; 614:7947, s. 281-286
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Tidskriftsartikel (refereegranskat)abstract
- Wetlands have long been drained for human use, thereby strongly affecting greenhouse gas fluxes, flood control, nutrient cycling and biodiversity1,2. Nevertheless, the global extent of natural wetland loss remains remarkably uncertain3. Here, we reconstruct the spatial distribution and timing of wetland loss through conversion to seven human land uses between 1700 and 2020, by combining national and subnational records of drainage and conversion with land-use maps and simulated wetland extents. We estimate that 3.4 million km2 (confidence interval 2.9–3.8) of inland wetlands have been lost since 1700, primarily for conversion to croplands. This net loss of 21% (confidence interval 16–23%) of global wetland area is lower than that suggested previously by extrapolations of data disproportionately from high-loss regions. Wetland loss has been concentrated in Europe, the United States and China, and rapidly expanded during the mid-twentieth century. Our reconstruction elucidates the timing and land-use drivers of global wetland losses, providing an improved historical baseline to guide assessment of wetland loss impact on Earth system processes, conservation planning to protect remaining wetlands and prioritization of sites for wetland restoration4.
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| 10. |
- Froslev Nielsen, Jens Christian, 1987, et al.
(författare)
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Global analysis of biosynthetic gene clusters reveals vast potential of secondary metabolite production in Penicillium species
- 2017
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Ingår i: Nature Microbiology. - : Springer Science and Business Media LLC. - 2058-5276. ; 2:6
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Tidskriftsartikel (refereegranskat)abstract
- Filamentous fungi produce a wide range of bioactive compounds with important pharmaceutical applications, such as antibiotic penicillins and cholesterol-lowering statins. However, less attention has been paid to fungal secondary metabolites compared to those from bacteria. In this study, we sequenced the genomes of 9 Penicillium species and, together with 15 published genomes, we investigated the secondary metabolism of Penicillium and identified an immense, unexploited potential for producing secondary metabolites by this genus. A total of 1,317 putative biosynthetic gene clusters (BGCs) were identified, and polyketide synthase and non-ribosomal peptide synthetase based BGCs were grouped into gene cluster families and mapped to known pathways. The grouping of BGCs allowed us to study the evolutionary trajectory of pathways based on 6-methylsalicylic acid (6-MSA) synthases. Finally, we cross-referenced the predicted pathways with published data on the production of secondary metabolites and experimentally validated the production of antibiotic yanuthones in Penicillia and identified a previously undescribed compound from the yanuthone pathway. This study is the first genus-wide analysis of the genomic diversity of Penicillia and highlights the potential of these species as a source of new antibiotics and other pharmaceuticals.
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