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Sökning: WFRF:(Putkonen Jaakko)

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1.
  • Niinisto, Jaakko, et al. (författare)
  • Advanced cyclopentadienyl precursors for atomic layer deposition of ZrO2 thin films
  • 2008
  • Ingår i: Journal of Materials Chemistry. - : Royal Society of Chemistry (RSC). - 0959-9428 .- 1364-5501. ; 18:28, s. 3385-3390
  • Tidskriftsartikel (refereegranskat)abstract
    • ZrO2 thin films were grown onto silicon (100) substrates by atomic layer deposition (ALD) using novel cyclopentadienyl-type precursors, namely (CpMe)(2)ZrMe2 and (CpMe)(2)Zr(OMe) Me (Cp = cyclopentadienyl, C5H5) together with ozone as the oxygen source. Growth characteristics were studied in the temperature range of 250 to 500 degrees C. An ALD-type self-limiting growth mode was verified for both processes at 350 degrees C where highly conformal films were deposited onto high aspect ratio trenches. Signs of thermal decomposition were not observed at or below 400 degrees C, a temperature considerably exceeding the thermal decomposition temperature of the Zr-alkylamides. Processing parameters were optimised at 350 degrees C, where deposition rates of 0.55 and 0.65 angstrom cycle(-1) were obtained for (CpMe)(2)ZrMe2/O-3 and (CpMe)(2)Zr(OMe)Me/O-3, respectively. The films grown from both precursors were stoichiometric and polycrystalline with an increasing contribution from the metastable cubic phase with decreasing film thickness. In the films grown from (CpMe)(2)ZrMe2, the breakdown field did not essentially depend on the film thickness, whereas in the films grown from (CpMe)(2)Zr(OMe)Me the structural homogeneity and breakdown field increased with decreasing film thickness. The films exhibited good capacitive properties that were characteristic of insulating oxides and did not essentially depend on the precursor chemistry.
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2.
  • Oehri, Jacqueline, et al. (författare)
  • Vegetation type is an important predictor of the arctic summer land surface energy budget
  • 2022
  • Ingår i: Nature Communications. - : Springer Nature. - 2041-1723. ; 13
  • Tidskriftsartikel (refereegranskat)abstract
    • Despite the importance of high-latitude surface energy budgets (SEBs) for land-climate interactions in the rapidly changing Arctic, uncertainties in their prediction persist. Here, we harmonize SEB observations across a network of vegetated and glaciated sites at circumpolar scale (1994–2021). Our variance-partitioning analysis identifies vegetation type as an important predictor for SEB-components during Arctic summer (June-August), compared to other SEB-drivers including climate, latitude and permafrost characteristics. Differences among vegetation types can be of similar magnitude as between vegetation and glacier surfaces and are especially high for summer sensible and latent heat fluxes. The timing of SEB-flux summer-regimes (when daily mean values exceed 0 Wm−2) relative to snow-free and -onset dates varies substantially depending on vegetation type, implying vegetation controls on snow-cover and SEB-flux seasonality. Our results indicate complex shifts in surface energy fluxes with land-cover transitions and a lengthening summer season, and highlight the potential for improving future Earth system models via a refined representation of Arctic vegetation types.
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