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Sökning: WFRF:(Rappe A. M.)

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1.
  • Chen, F., et al. (författare)
  • Reply to "comment on 'Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO3 ' "
  • 2018
  • Ingår i: Physical Review B. - 2469-9950. ; 97:22
  • Tidskriftsartikel (refereegranskat)abstract
    • In this reply to S. Durbin's comment on our original paper "Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO3," we concur that his final equations 8 and 9 more accurately describe the change in diffracted intensity as a function of Ti displacement. We also provide an alternative derivation based on an ensemble average over unit cells. The conclusions of the paper are unaffected by this correction.
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2.
  • Chen, F., et al. (författare)
  • Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO3
  • 2016
  • Ingår i: Physical Review B. - 1098-0121. ; 94:18
  • Tidskriftsartikel (refereegranskat)abstract
    • The dynamical processes associated with electric field manipulation of the polarization in a ferroelectric remain largely unknown but fundamentally determine the speed and functionality of ferroelectric materials and devices. Here we apply subpicosecond duration, single-cycle terahertz pulses as an ultrafast electric field bias to prototypical BaTiO3 ferroelectric thin films with the atomic-scale response probed by femtosecond x-ray-scattering techniques. We show that electric fields applied perpendicular to the ferroelectric polarization drive large-amplitude displacements of the titanium atoms along the ferroelectric polarization axis, comparable to that of the built-in displacements associated with the intrinsic polarization and incoherent across unit cells. This effect is associated with a dynamic rotation of the ferroelectric polarization switching on and then off on picosecond time scales. These transient polarization modulations are followed by long-lived vibrational heating effects driven by resonant excitation of the ferroelectric soft mode, as reflected in changes in the c-axis tetragonality. The ultrafast structural characterization described here enables a direct comparison with first-principles-based molecular-dynamics simulations, with good agreement obtained.
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3.
  • Daranciang, Dan, et al. (författare)
  • Ultrafast Photovoltaic Response in Ferroelectric Nanolayers
  • 2012
  • Ingår i: Physical Review Letters. - 1079-7114. ; 108:8
  • Tidskriftsartikel (refereegranskat)abstract
    • We show that light drives large-amplitude structural changes in thin films of the prototypical ferroelectric PbTiO3 via direct coupling to its intrinsic photovoltaic response. Using time-resolved x-ray scattering to visualize atomic displacements on femtosecond time scales, photoinduced changes in the unit-cell tetragonality are observed. These are driven by the motion of photogenerated free charges within the ferroelectric and can be simply explained by a model including both shift and screening currents, associated with the displacement of electrons first antiparallel to and then parallel to the ferroelectric polarization direction.
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4.
  • Duffy, J. Emmett, et al. (författare)
  • Toward a Coordinated Global Observing System for Seagrasses and Marine Macroalgae
  • 2019
  • Ingår i: Frontiers in Marine Science. - : Frontiers Media S.A.. - 2296-7745. ; 6
  • Forskningsöversikt (refereegranskat)abstract
    • In coastal waters around the world, the dominant primary producers are benthic macrophytes, including seagrasses and macroalgae, that provide habitat structure and food for diverse and abundant biological communities and drive ecosystem processes. Seagrass meadows and macroalgal forests play key roles for coastal societies, contributing to fishery yields, storm protection, biogeochemical cycling and storage, and important cultural values. These socio-economically valuable services are threatened worldwide by human activities, with substantial areas of seagrass and macroalgal forests lost over the last half-century. Tracking the status and trends in marine macrophyte cover and quality is an emerging priority for ocean and coastal management, but doing so has been challenged by limited coordination across the numerous efforts to monitor macrophytes, which vary widely in goals, methodologies, scales, capacity, governance approaches, and data availability. Here, we present a consensus assessment and recommendations on the current state of and opportunities for advancing global marine macrophyte observations, integrating contributions from a community of researchers with broad geographic and disciplinary expertise. With the increasing scale of human impacts, the time is ripe to harmonize marine macrophyte observations by building on existing networks and identifying a core set of common metrics and approaches in sampling design, field measurements, governance, capacity building, and data management. We recommend a tiered observation system, with improvement of remote sensing and remote underwater imaging to expand capacity to capture broad-scale extent at intervals of several years, coordinated with strati fied in situ sampling annually to characterize the key variables of cover and taxonomic or functional group composition, and to provide ground-truth. A robust networked system of macrophyte observations will be facilitated by establishing best practices, including standard protocols, documentation, and sharing of resources at all stages of work flow, and secure archiving of open-access data. Because such a network is necessarily distributed, sustaining it depends on close engagement of local stakeholders and focusing on building and long-term maintenance of local capacity, particularly in the developing world. Realizing these recommendations will producemore effective, efficient, and responsive observing, a more accurate global picture of change in vegetated coastal systems, and stronger international capacity for sustaining observations.
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5.
  • Jones, Benjamin L. H., et al. (författare)
  • Dependence on seagrass fisheries governed by household income and adaptive capacity
  • 2022
  • Ingår i: Ocean and Coastal Management. - : Elsevier BV. - 0964-5691 .- 1873-524X. ; 225
  • Tidskriftsartikel (refereegranskat)abstract
    • Seagrass meadows, like other tropical coastal ecosystems, are highly productive and sustain millions of people worldwide. However, the factors that govern the use of seagrass as a fishing habitat over other habitats are largely unknown, especially at the household scale. Using socioeconomic factors from 147 villages across four countries within the Indo-Pacific, we examined the drivers of household dependence on seagrass. We revealed that seagrass was the most common habitat used for fishing across villages in all the countries studied, being preferred over other habitats for reliability. Using structural equation modelling, we exposed how household income and adaptive capacity appears to govern dependence on seagrass. Poorer households were less likely to own motorboats and dependent on seagrass as they were unable to fish elsewhere, whereas wealthier households were more likely to invest in certain fishing gears that incentivised them to use seagrass habitats due to high rewards and low effort requirements. Our findings accentuate the complexity of seagrass social-ecological systems and the need for empirical household scale data for effective management. Safeguarding seagrass is vital to ensure that vulnerable households have equitable and equal access to the resource, addressing ocean recovery and ensuring sustainable coastal communities.
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6.
  • Jones, Benjamin L., et al. (författare)
  • Local Ecological Knowledge Reveals Change in Seagrass Social–Ecological Systems
  • 2022
  • Ingår i: Oceans. - : MDPI AG. - 2673-1924. ; 3:3, s. 419-430
  • Tidskriftsartikel (refereegranskat)abstract
    • It is widely recognized that humanity is currently facing multiple planetary crises, including the widespread loss of biodiversity and a rapidly changing climate. The impacts of these crises are often far reaching and threaten food security (SDG goal two: zero hunger). Small-scale fisheries are estimated to provide livelihoods for over one hundred million people and sustenance for approximately one billion people but face a plethora of threats and challenges linked to planetary crises. In this multi-country assessment (150 coastal villages across five countries within the Indo-Pacific), household interviews revealed how seagrass meadows are important to small-scale fisheries, particularly as a place to find and collect a reliable source of food. Interviews also revealed that habitat loss and the over-exploitation of these resources are placing people and their food security at risk. This study exposed how dynamic local ecological knowledge can be, uncovering personal opinions and responsibilities that result in the hybridization of knowledge. Here, we demonstrate the importance of using local ecological knowledge to incorporate shared values into management but also highlight that an integrated approach, pairing local and conventional scientific knowledge, is needed urgently if we are to meet the needs of people while simultaneously conserving biodiversity.
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  • Resultat 1-6 av 6

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