| 1. |
- Burger, Paul, 1997, et al.
(författare)
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Atomic Force Manipulation of Single Magnetic Nanoparticles for Spin-Based Electronics
- 2022
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Ingår i: ACS Nano. - : American Chemical Society. - 1936-0851 .- 1936-086X. ; 16:11, s. 19253-19260
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Tidskriftsartikel (refereegranskat)abstract
- Magnetic nanoparticles (MNPs) are instrumental for fabrication of tailored nanomagnetic structures, especially where top-down lithographic patterning is not feasible. Here, we demonstrate precise and controllable manipulation of individual magnetite MNPs using the tip of an atomic force microscope. We verify our approach by placing a single MNP with a diameter of 50 nm on top of a 100 nm Hall bar fabricated in a quasi-two-dimensional electron gas (q2DEG) at the oxide interface between LaAlO3 and SrTiO3 (LAO/STO). A hysteresis loop due to the magnetic hysteresis properties of the magnetite MNPs was observed in the Hall resistance. Further, the effective coercivity of the Hall resistance hysteresis loop could be changed upon field cooling at different angles of the cooling field with respect to the measuring field. The effect is associated with the alignment of the MNP magnetic moment along the easy axis closest to the external field direction across the Verwey transition in magnetite. Our results can facilitate experimental realization of magnetic proximity devices using single MNPs and two-dimensional materials for spin-based nanoelectronics. © 2022 The Authors.
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| 2. |
- Jouan, A., et al.
(författare)
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Multiband Effects in the Superconducting Phase Diagram of Oxide Interfaces
- 2022
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Ingår i: Advanced Materials Interfaces. - : Wiley. - 2196-7350. ; 9:29
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Tidskriftsartikel (refereegranskat)abstract
- A dome-shaped phase diagram of superconducting critical temperature upon doping is often considered as a hallmark of unconventional superconductors. This behavior, observed in SrTiO3-based interfaces, whose electronic density is controlled by field-effect, has not been explained unambiguously yet. Here, a generic scenario for the superconducting phase diagram of these oxide interfaces is elaborated based on transport experiments on a double-gate LaAlO3/SrTiO3 field-effect device and Schrödinger–Poisson numerical simulations of the quantum well. The optimal doping point of maximum Tc is ascribed to the transition between a single-gap and a fragile two-gap s±-wave superconducting state involving bands of different orbital character. Close to this point, a bifurcation in the dependence of Tc on the carrier density, which can be controlled by the details of the doping execution, is observed experimentally and reproduced by numerical simulations. Where doping with a back-gate triggers the filling of a new (Formula presented.) subband and initiates the overdoped regime, doping with a top-gate delays the filling of the subband and maintains the 2D electron gaz in the single-gap state of higher Tc. Such a bifurcation, whose branches can be followed reversibly, provides a generic explanation for the dome-shaped superconducting phase diagram that could be extended to other multiband superconducting materials.
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| 3. |
- Jouan, A., et al.
(författare)
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Quantized conductance in a one-dimensional ballistic oxide nanodevice
- 2020
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Ingår i: Nature Electronics. - : Springer Science and Business Media LLC. - 2520-1131. ; 3:4, s. 201-206
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Tidskriftsartikel (refereegranskat)abstract
- The electric-field effect control of two-dimensional electron gases (2-DEGs) has allowed nanoscale electron quantum transport to be explored in semiconductors. Structures based on transition metal oxides have electronic states that favour the emergence of novel quantum orders that are absent in conventional semiconductors and the 2-DEG formed at a LaAlO3/SrTiO3 interface-a structure in which superconductivity and spin-orbit coupling can coexist-is a promising platform to develop devices for spintronics and topological electronics. However, field-effect control of the properties of this interface at the nanoscale remains challenging. Here we show that a quantum point contact can be formed in a LaAlO3/SrTiO3 interface through electrostatic confinement of the 2-DEG using a split gate. Our device exhibits a quantized conductance due to ballistic transport in a controllable number of one-dimensional conducting channels. Under a magnetic field, the direct observation of the Zeeman splitting between spin-polarized bands allows the determination of the Lande g-factor, whose value differs strongly from that of the free electrons. Through source-drain voltage measurements, we also performed a spectroscopic investigation of the 3d energy levels inside the quantum point contact. The LaAlO3/SrTiO3 quantum point contact could potentially be used as a spectrometer to probe Majorana states in an oxide 2-DEG. A quantum point contact formed in the two-dimensional electron gas of a LaAlO3/SrTiO3 interface exhibits quantized conductance due to ballistic transport in a controllable number of one-dimensional conducting channels.
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| 4. |
- Park, D. S., et al.
(författare)
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The emergence of magnetic ordering at complex oxide interfaces tuned by defects
- 2020
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Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723 .- 2041-1723. ; 11:1
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Tidskriftsartikel (refereegranskat)abstract
- Complex oxides show extreme sensitivity to structural distortions and defects, and the intricate balance of competing interactions which emerge at atomically defined interfaces may give rise to unexpected physics. In the interfaces of non-magnetic complex oxides, one of the most intriguing properties is the emergence of magnetism which is sensitive to chemical defects. Particularly, it is unclear which defects are responsible for the emergent magnetic interfaces. Here, we show direct and clear experimental evidence, supported by theoretical explanation, that the B-site cation stoichiometry is crucial for the creation and control of magnetism at the interface between non-magnetic ABO3-perovskite oxides, LaAlO3 and SrTiO3. We find that consecutive defect formation, driven by atomic charge compensation, establishes the formation of robust perpendicular magnetic moments at the interface. Our observations propose a route to tune these emerging magnetoelectric structures, which are strongly coupled at the polar-nonpolar complex oxide interfaces.
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| 5. |
- Singh, Gyanendra, 1983, et al.
(författare)
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Gate-tunable pairing channels in superconducting non-centrosymmetric oxides nanowires
- 2022
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Ingår i: npj Quantum Materials. - : Springer Science and Business Media LLC. - 2397-4648. ; 7:1
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Tidskriftsartikel (refereegranskat)abstract
- Two-dimensional SrTiO3-based interfaces stand out among non-centrosymmetric superconductors due to their intricate interplay of gate-tunable Rashba spin-orbit coupling and multi-orbital electronic occupations, whose combination theoretically prefigures various forms of non-standard superconductivity. By employing superconducting transport measurements in nano-devices we present strong experimental indications of unconventional superconductivity in the LaAlO3/SrTiO3 interface. The central observations are the substantial anomalous enhancement of the critical current by small magnetic fields applied perpendicularly to the plane of electron motion, and the asymmetric response with respect to the magnetic field direction. These features cannot be accommodated within a scenario of canonical spin-singlet superconductivity. We demonstrate that the experimental observations can be described by a theoretical model based on the coexistence of Josephson channels with intrinsic phase shifts. Our results exclude a time-reversal symmetry breaking scenario and suggest the presence of anomalous pairing components that are compatible with inversion symmetry breaking and multi-orbital physics.
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| 6. |
- Singh, Gyanendra, 1983, et al.
(författare)
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Nanopatterning of weak links in superconducting oxide interfaces
- 2021
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Ingår i: Nanomaterials. - : MDPI AG. - 2079-4991. ; 11:2, s. 1-11
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Tidskriftsartikel (refereegranskat)abstract
- The interface between two wide band-gap insulators, LaAlO3 and SrTiO3 (LAO/STO), hosts a quasi-two-dimensional electron gas (q2DEG), two-dimensional superconductivity, ferromagnetism, and giant Rashba spin-orbit coupling. The co-existence of two-dimensional superconductivity with gate-tunable spin-orbit coupling and multiband occupation is of particular interest for the realization of unconventional superconducting pairing. To investigate the symmetry of the superconducting order parameter, phase sensitive measurements of the Josephson effect are required. We describe an approach for the fabrication of artificial superconducting weak links at the LAO/STO interface using direct high-resolution electron beam lithography and low-energy argon ion beam irradiation. The method does not require lift-off steps or sacrificial layers. Therefore, resolution is only limited by the electron beam lithography and pattern transfer. We have realized superconducting weak links with a barrier thickness of 30–100 nm. The barrier transparency of the weak links can be controlled by the irradiation dose and further tuned by a gate voltage. Our results open up new possibilities for the realization of quantum devices in oxide interfaces.
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| 7. |
- Singh, Gyanendra, 1983, et al.
(författare)
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Two-gap s± -wave superconductivity at an oxide interface
- 2022
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Ingår i: Physical Review B. - 2469-9969 .- 2469-9950. ; 105:6
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Tidskriftsartikel (refereegranskat)abstract
- After half a century of debate, superconductivity in doped SrTiO3 has come to the fore again with the discovery of interfacial superconductivity in the LaAlO3 /SrTiO3 heterostructures. While these interfaces share the interesting properties of bulk SrTiO3, quantum confinement generates a complex band structure involving bands with different orbital symmetries whose occupancy is tunable by electrostating doping. Multigap superconductivity has been predicted to emerge in LaAlO3 /SrTiO3 at large doping, with a Bose-Einstein condensation character at the Lifshtiz transition. In this article, we report on the measurement of the upper critical magnetic field Hc2 of superconducting (110)-oriented LaAlO3 /SrTiO3 heterostructures and evidence a two-gap superconducting regime at high doping. Our results are quantitatively explained by a theoretical model based on the formation of an unconventional s±-wave superconducting state with a repulsive coupling between the two condensates.
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