| 1. |
- Bossioli, Elissavet, et al.
(författare)
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Modeling Extreme Warm-Air Advection in the Arctic During Summer : The Effect of Mid-Latitude Pollution Inflow on Cloud Properties
- 2021
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Ingår i: Journal of Geophysical Research - Atmospheres. - 2169-897X .- 2169-8996. ; 126:7
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Tidskriftsartikel (refereegranskat)abstract
- Usually the Arctic is relatively free of anthropogenic influence in summer, which means that particles from natural sources can be the most significant nuclei for cloud droplets. However, this is not the case during anomalously warm-air intrusions when the air origin comes from lower latitudes. In this modeling study, we investigate the effect of mid-latitude pollution inflow (anthropogenic and biomass burning [BB]) on the aerosol-cloud-radiation interactions during an episode of extreme warm-air advection. This particular episode resulted in anomalously high air temperatures over the East Siberian Sea and has accelerated sea-ice melting. The impact of different emission sources on aerosol vertical distribution, chemical composition, cloud formation, and radiation budget is examined using the Weather Research and Forecasting model, fully coupled with chemistry. Elevated turbulent clouds that occurred at the beginning of the episode are found to be more sensitive to aerosol variations and their negative feedback on supersaturation, compared to stably stratified fog layers that were dominant during the core period. Omission of either anthropogenic or BB source results in decreased cloud liquid water and cloud droplet concentrations; however, these changes are not substantially large to significantly modify the net surface radiation budget. Significant reduction of the net surface radiation is only observed if both anthropogenic and BB transported pollution reaches the area of interest.
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| 2. |
- Karalis, Michail, et al.
(författare)
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Effects of secondary ice processes on a stratocumulus to cumulus transition during a cold-air outbreak
- 2022
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Ingår i: Atmospheric research. - : Elsevier Ltd. - 0169-8095 .- 1873-2895. ; 277
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Tidskriftsartikel (refereegranskat)abstract
- The representation of boundary layer clouds during marine Cold-Air Outbreaks (CAO) remains a great challenge for weather prediction models. Recent studies have shown that the representation of the transition from closed stratocumulus clouds to convective cumulus open cells largely depends on microphysical and precipitation processes, which secondary ice production (SIP) may strongly modulate. In this study we use the Weather Research and Forecasting model to investigate the impact of the most well-known SIP mechanisms (Hallett-Mossop, mechanical break-up upon collisions between ice particles and drop-shattering) on a CAO case observed north of the United Kingdom in 2013. While Hallett-Mossop is the only SIP process extensively implemented in atmospheric models, our results indicate that the other two SIP mechanisms are also favored in the examined conditions. Activation of drop-shattering and especially collisional break-up can result in enhanced riming, ice depositional growth and/or ice aggregation. The first two processes quicken liquid depletion in the stratocumulus cloud, while along with aggregation, they enhance precipitation. The increased precipitation results in enhanced evaporation/sublimation in the sub-cloud layer, promoting boundary-layer decoupling, which further accelerates the onset of the stratocumulus break-up. However, the strong sensitivity to the expression of terminal velocity of the precipitating particles and the rimed fraction of cloud ice/snow suggests that the robust implementation of SIP to improve CAO predictions requires data from a large number of CAO events.
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| 3. |
- Achtert, Peggy, et al.
(författare)
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Properties of Arctic liquid and mixed-phase clouds from shipborne Cloudnet observations during ACSE 2014
- 2020
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 20:23, s. 14983-15002
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Tidskriftsartikel (refereegranskat)abstract
- This study presents Cloudnet retrievals of Arctic clouds from measurements conducted during a 3-month research expedition along the Siberian shelf during summer and autumn 2014. During autumn, we find a strong reduction in the occurrence of liquid clouds and an increase for both mixed-phase and ice clouds at low levels compared to summer. About 80 % of all liquid clouds observed during the research cruise show a liquid water path below the infrared black body limit of approximately 50 g m(-2). The majority of mixed-phase and ice clouds had an ice water path below 20 g m(-2). Cloud properties are analysed with respect to cloud-top temperature and boundary layer structure. Changes in these parameters have little effect on the geometric thickness of liquid clouds while mixed-phase clouds during warm-air advection events are generally thinner than when such events were absent. Cloud-top temperatures are very similar for all mixed-phase clouds. However, more cases of lower cloudtop temperature were observed in the absence of warm-air advection. Profiles of liquid and ice water content are normalized with respect to cloud base and height. For liquid water clouds, the liquid water content profile reveals a strong increase with height with a maximum within the upper quarter of the clouds followed by a sharp decrease towards cloud top. Liquid water content is lowest for clouds observed below an inversion during warm-air advection events. Most mixedphase clouds show a liquid water content profile with a very similar shape to that of liquid clouds but with lower maximum values during events with warm air above the planetary boundary layer. The normalized ice water content profiles in mixed-phase clouds look different from those of liquid water content. They show a wider range in maximum values with the lowest ice water content for clouds below an inversion and the highest values for clouds above or extending through an inversion. The ice water content profile generally peaks at a height below the peak in the liquid water content profile - usually in the centre of the cloud, sometimes closer to cloud base, likely due to particle sublimation as the crystals fall through the cloud.
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| 4. |
- Georgakaki, Paraskevi, et al.
(författare)
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Secondary ice production processes in wintertime alpine mixed-phase clouds
- 2022
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Ingår i: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 22:3, s. 1965-1988
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Tidskriftsartikel (refereegranskat)abstract
- Observations of orographic mixed-phase clouds (MPCs) have long shown that measured ice crystal number concentrations (ICNCs) can exceed the concentration of ice nucleating particles by orders of magnitude. Additionally, model simulations of alpine clouds are frequently found to underestimate the amount of ice compared with observations. Surface-based blowing snow, hoar frost, and secondary ice production processes have been suggested as potential causes, but their relative importance and persistence remains highly uncertain. Here we study ice production mechanisms in wintertime orographic MPCs observed during the Cloud and Aerosol Characterization Experiment (CLACE) 2014 campaign at the Jungfraujoch site in the Swiss Alps with the Weather Research and Forecasting model (WRF). Simulations suggest that droplet shattering is not a significant source of ice crystals at this specific location, but breakups upon collisions between ice particles are quite active, elevating the predicted ICNCs by up to 3 orders of magnitude, which is consistent with observations. The initiation of the ice–ice collisional breakup mechanism is primarily associated with the occurrence of seeder–feeder events from higher precipitating cloud layers. The enhanced aggregation of snowflakes is found to drive secondary ice formation in the simulated clouds, the role of which is strengthened when the large hydrometeors interact with the primary ice crystals formed in the feeder cloud. Including a constant source of cloud ice crystals from blowing snow, through the action of the breakup mechanism, can episodically enhance ICNCs. Increases in secondary ice fragment generation can be counterbalanced by enhanced orographic precipitation, which seems to prevent explosive multiplication and cloud dissipation. These findings highlight the importance of secondary ice and seeding mechanisms – primarily falling ice from above and, to a lesser degree, blowing ice from the surface – which frequently enhance primary ice and determine the phase state and properties of MPCs.
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| 5. |
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| 6. |
- Sotiropoulou, Georgia, et al.
(författare)
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Atmospheric conditions during the Arctic Clouds in Summer Experiment (ACSE) : Contrasting open-water and sea-ice surfaces during melt and freeze-up seasons
- 2016
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Ingår i: Journal of Climate. - 0894-8755 .- 1520-0442. ; 29:24, s. 8721-8744
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Tidskriftsartikel (refereegranskat)abstract
- The Arctic Clouds in Summer Experiment (ACSE) was conducted during summer and early autumn 2014, providing a detailed view of the seasonal transition from ice melt into freeze-up. Measurements were taken over both ice-free and ice-covered surfaces, near the ice edge, offering insight to the role of the surface state in shaping the atmospheric conditions. The initiation of the autumn freeze-up was related to a change in air mass, rather than to changes in solar radiation alone; the lower atmosphere cooled abruptly leading to a surface heat loss. During melt season, strong surface inversions persisted over the ice, while elevated inversions were more frequent over open water. These differences disappeared during autumn freeze-up, when elevated inversions persisted over both ice-free and ice-covered conditions. These results are in contrast to previous studies that found a well-mixed boundary layer persisting in summer and an increased frequency of surface-based inversions in autumn, suggesting that our knowledge derived from measurements taken within the pan-Arctic area and on the central ice-pack does not necessarily apply closer to the ice-edge. This study offers an insight to the atmospheric processes that occur during a crucial period of the year; understanding and accurately modeling these processes is essential for the improvement of ice-extent predictions and future Arctic climate projections.
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| 7. |
- Sotiropoulou, Georgia, et al.
(författare)
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Ice multiplication from ice-ice collisions in the high Arctic: Sensitivity to ice habit, rimed fraction, ice type and uncertainties in the numerical description of the process
- 2021
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Ingår i: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 21:12, s. 9741-9760
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Tidskriftsartikel (refereegranskat)abstract
- Atmospheric models often fail to correctly reproduce the microphysical structure of Arctic mixed-phase clouds and underpredict ice water content even when the simulations are constrained by observed levels of ice nucleating particles. In this study we investigate whether ice multiplication from breakup upon ice-ice collisions, a process missing in most models, can account for the observed cloud ice in a stratocumulus cloud observed during the Arctic Summer Cloud Ocean Study (ASCOS) campaign. Our results indicate that the efficiency of this process in these conditions is weak; increases in fragment generation are compensated for by subsequent enhancement of precipitation and subcloud sublimation. Activation of collisional breakup improves the representation of cloud ice content, but cloud liquid remains overestimated. In most sensitivity simulations, variations in ice habit and prescribed rimed fraction have little effect on the results. A few simulations result in explosive multiplication and cloud dissipation; however, in most setups, the overall multiplication effects become substantially weaker if the precipitation sink is enhanced through cloud-ice-to-snow autoconversion. The largest uncertainty stems from the correction factor for ice enhancement due to sublimation included in the breakup parameterization; excluding this correction results in rapid glaciation, especially in simulations with plates. Our results indicate that the lack of a detailed treatment of ice habit and rimed fraction in most bulk microphysics schemes is not detrimental for the description of the collisional breakup process in the examined conditions as long as cloud-ice-to-snow autoconversion is considered.
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| 8. |
- Sotiropoulou, Georgia, et al.
(författare)
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Large-eddy simulation of a warm-air advection episode in the summer Arctic
- 2018
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Ingår i: Quarterly Journal of the Royal Meteorological Society. - : Wiley. - 0035-9009 .- 1477-870X. ; 144:717, s. 2449-2462
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Tidskriftsartikel (refereegranskat)abstract
- While there is an increasing scientific interest in the role of advection of warm and moist air into the Arctic, there is little understanding of the interactive processes between the advected air, boundary-layer clouds and turbulence during such events and almost all studies refer to winter conditions. We use large-eddy simulation (LES) to investigate these processes for an extreme warm-air advection episode observed during summer 2014. The results indicate that moisture advection is the critical factor for cloud formation; shutting off this supply resulted in cloud dissipation, regardless of heat advection being present or not. The dissipation of the cloud reduced the surface energy budget by up to 37W/m(2). Advection of heat suppresses cloud-driven mixing through enhancement of the atmospheric stability. Turning off the large-scale heat transport therefore resulted in a somewhat optically thicker cloud, on average increasing the liquid water path by approximate to 10g/m(2). The results showed little sensitivity to a number of assumptions and simplifications in the LES set-up, such as the prescribed cloud condensation nuclei concentration, friction velocity, surface albedo and the available moisture above the cloud layer.
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| 9. |
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| 10. |
- Sotiropoulou, Georgia, et al.
(författare)
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Late Summer Arctic clouds in the ECMWF forecast model : an evaluation of cloud parameterization scheme
- 2016
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Ingår i: Quarterly Journal of the Royal Meteorological Society. - : Wiley. - 0035-9009 .- 1477-870X. ; 142:694, s. 387-400
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Tidskriftsartikel (refereegranskat)abstract
- Mixed-phase clouds are an integral part of the Arctic climate system, for precipitation and for their interactions with radiation and thermodynamics. Mixed-phase processes are often poorly represented in global models and many use an empirically based diagnostic partition between the liquid and ice phases that is dependent solely on temperature. However, increasingly more complex microphysical parametrizations are being implemented allowing a more physical representation of mixed-phase clouds.This study uses in situ observations from the Arctic Summer Cloud Ocean Study (ASCOS) field campaign in the central Arctic to assess the impact of a change from a diagnostic to a prognostic parametrization of mixed-phase clouds and increased vertical resolution in the European Centre for Medium-Range Weather Forecasts (ECMWF) Integrated Forecast System (IFS). The newer cloud scheme improves the representation of the vertical structure of mixed-phase clouds, with supercooled liquid water at cloud top and ice precipitating below, improved further with higher vertical resolution. Increased supercooled liquid water and decreased ice content are both in closer agreement with observations. However, these changes do not result in any substantial improvement in surface radiation, and a warm and moist bias in the lowest part of the atmosphere remains. Both schemes also fail to capture the transitions from overcast to cloud-free conditions. Moreover, whereas the observed cloud layer is frequently decoupled from the surface, the modelled clouds remain coupled to the surface most of the time. The changes implemented to the cloud scheme are an important step forward in improving the representation of Arctic clouds, but improvements in other aspects such as boundary-layer turbulence, cloud radiative properties, sensitivity to low aerosol concentrations and representation of the sea-ice surface may also need to be addressed.
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