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Sökning: WFRF:(Tamenori Yusuke)

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  • Velkov, Yasen, et al. (författare)
  • X-ray-absorption spectroscopy beyond the natural width measured in partial Auger yield mode
  • 2009
  • Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 79:2
  • Tidskriftsartikel (refereegranskat)abstract
    • We report both experimental and theoretical studies on x-ray absorption measured using partial Auger yields of gas phase nitrogen, carbon monoxide, and oxygen molecules near the N 1s ->pi(*), O 1s ->pi(*), and O 1s ->pi(*) regions, respectively. The main tool of our study is a two-dimensional map in which resonant Auger yields are plotted as a function of photon and kinetic energy. The partial yields of the three molecules are analyzed in detail by extracting profiles along various directions in the map. Narrowing of the absorption resonances is observed along the direction of constant kinetic energy. It is shown that such profiles are similar to the conventional x-ray-absorption spectrum for a broad class of molecules whose potential energy surfaces of the final and core-excited states are almost parallel. However, substantial differences with the conventional x-ray-absorption profiles are observed in the general case of nonparallel surfaces due to the lifetime vibrational interference. Here, we suggest a systematic way to eliminate the lifetime vibrational interference.
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3.
  • Yabuta, Hikaru, et al. (författare)
  • Macromolecular organic matter in samples of the asteroid (162173) Ryugu
  • 2023
  • Ingår i: Science. - : American Association for the Advancement of Science. - 0036-8075 .- 1095-9203. ; 379:6634
  • Tidskriftsartikel (refereegranskat)abstract
    • Samples of the carbonaceous asteroid (162173) Ryugu were collected and brought to Earth by the Hayabusa2 spacecraft. We investigated the macromolecular organic matter in Ryugu samples and found that it contains aromatic and aliphatic carbon, ketone, and carboxyl functional groups. The spectroscopic features of the organic matter are consistent with those in chemically primitive carbonaceous chondrite meteorites that experienced parent-body aqueous alteration (reactions with liquid water). The morphology of the organic carbon includes nanoglobules and diffuse carbon associated with phyllosilicate and carbonate minerals. Deuterium and/or nitrogen-15 enrichments indicate that the organic matter formed in a cold molecular cloud or the presolar nebula. The diversity of the organic matter indicates variable levels of aqueous alteration on Ryugus parent body.
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