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- Mathieu, Roland, et al.
(författare)
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Bandwidth-disorder phase diagram of half-doped layered manganites
- 2006
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Ingår i: Physical Review B. Condensed Matter and Materials Physics. - 1098-0121 .- 1550-235X. ; 74:2
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Tidskriftsartikel (refereegranskat)abstract
- Phase diagrams in the plane of rA (the average ionic radius, related to the one-electron bandwidth W) and σ2 (the ionic radius variance, measuring the quenched disorder), or bandwidth-disorder phase diagrams, have been established for perovskite manganites, with a three-dimensional (3D) Mn-O network. Here we establish the intrinsic bandwidth-disorder phase diagram of half-doped layered manganites with a two-dimensional (2D) Mn-O network, examining in detail the parent state of the colossal magnetoresistance phenomenon in crystals without ferromagnetic instability. The consequences of the reduced dimensionality, from 3D to 2D, for the order-disorder phenomena in the charge-orbital sectors are also highlighted.
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- Hudl, Mattias, et al.
(författare)
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Complex magnetism and magnetic-field-driven electrical polarization of Co(3)TeO(6)
- 2011
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Ingår i: Physical Review B. Condensed Matter and Materials Physics. - 1098-0121 .- 1550-235X. ; 84:18, s. 180404-
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Tidskriftsartikel (refereegranskat)abstract
- The magnetic and electrical properties of Co(3)TeO(6) single crystals with corundum-related structure reveal a magnetic-field-induced polarization below 21 K. A sharp peak in the specific heat at approximate to 18 K indicates a reconstructive-type first-order phase transition. From second-harmonic generation measurements, breaking of inversion symmetry is evident and the point-group symmetry was determined as m. The temperature and magnetic-field dependences of the magnetic and electrical polarizations are discussed in the light of the SHG results.
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- Ivanov, Sergey A., et al.
(författare)
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Spin and dipole order in geometrically frustrated mixed-valence manganite Pb3Mn7O15
- 2016
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Ingår i: Journal of materials science. Materials in electronics. - : Springer Science and Business Media LLC. - 0957-4522 .- 1573-482X. ; 27:12, s. 12562-12573
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Tidskriftsartikel (refereegranskat)abstract
- The structural, magnetic, and dielectric properties of Pb3Mn7O15 have been investigated using high-quality single crystals. Pb3Mn7O15 adopts a pseudo-hexagonal orthorhombic structure, with partially filled Kagom, layers connected by ribbons of edge-sharing MnO6 octahedra and intercalated Pb cations. There are 9 inequivalent sites in the structure for the Mn ions, which exist both as Mn3+ and Mn4+. Pb3Mn7O15 undergoes an antiferromagnetic transition below T-N similar to 67 K, with significant geometric frustration. Neutron powder diffraction on crushed single crystals allowed us to determine the low-temperature antiferromagnetic magnetic structure. We discuss the magnetic interaction pathways in the structure and possible interplay between the structural distortions imprinted by the lone-electron pair of Pb2+ cations and Mn3+/Mn4+ charge ordering.
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- M. A. Hossain, B. Bohnenbuck, Y. D. Chuang, M. W. Haverkort, I. S. Elfimov, A.Tanaka, A. G. Cruz Gonzalez, Z. Hu, H.-J. Lin, C. T. Chen, R. Mathieu, Y. Tokura, Y. Yoshida, L. H. Tjeng, Z. Hussain, B. Keimer, G. A. Sawatzky and A. Damascelli
(författare)
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Mott versus Slater-type metal-insulator transition in Mn-substituted Sr3Ru2O7
- 2012
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Ingår i: Physical Review B Condensed Matter. - 0163-1829 .- 1095-3795. ; 86, s. 041102(R)-
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Tidskriftsartikel (refereegranskat)
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- Mathieu, Roland, et al.
(författare)
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Coexistence of long-ranged charge and orbital order and spin-glass state in single-layered manganites with weak quenched disorder
- 2007
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Ingår i: Europhysics letters. - : IOP Publishing. - 0295-5075 .- 1286-4854. ; 80:3, s. 37001-
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Tidskriftsartikel (refereegranskat)abstract
- The relationship between orbital and spin degrees of freedom in the single crystals of the hole-doped Pr1-xCa1+xMnO4, 0.3 <= x <= 0.7 has been investigated by means of ac-magnetometry and charge transport. We show that in an intermediate underdoped region, with 0.35 <= x < 0.5, the "orbital-master spin-slave" relationship commonly observed in half-doped manganites does not take place. The long-ranged charge-orbital order is not accompanied by an antiferromagnetic transition at low temperatures, but by a frustrated short-ranged magnetic state bringing forth a spin-glass phase. We discuss in detail the nature and origin of this true spin-glass state, which, as in the half-doped manganites with large quenched disorder, is not related to the macroscopic phase separation observed in crystals with minor defects or impurities.
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