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Sökning: WFRF:(Wen Yuanfan)

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1.
  • Han, Jianhua, et al. (författare)
  • In situ formation of thermoset matrices for improved stability in organic photovoltaics
  • 2024
  • Ingår i: Joule. - 2542-4351. ; In Press
  • Tidskriftsartikel (refereegranskat)abstract
    • The performance of organic photovoltaics (OPVs) has rapidly increased. Yet, achieving long-term stability in the nano-morphology and thereby sustaining device performance remains challenging. Herein, we show that incorporating in-situ-forming cross-linked thermoset (CLT) matrices into the bulk heterojunction blends is a simple, general, and efficient strategy for high-performing and resilient OPVs. Our simulations and experimental data prove that these high-modulus CLT matrices featuring hydrogen-bonding interactions can freeze the nano-morphology, resulting in long-term thermal and photostable OPV devices. We demonstrate that this approach works efficiently with eight different blends and show that OPV devices can withstand 85°C for 1,000 h without losing performance. Blends with CLT matrices double the energy generated from OPV devices, showing an energy density output of 4,054 mW⋅h cm−2 over an 11-week operating period under outdoor conditions. This methodology opens avenues for both developing new thermoset networks for OPV and their use in other optoelectronic applications.
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2.
  • Paleti, Sri Harish Kumar, et al. (författare)
  • Hexanary blends : a strategy towards thermally stable organic photovoltaics
  • 2023
  • Ingår i: Nature Communications. - : Nature Publishing Group. - 2041-1723. ; 14:1
  • Tidskriftsartikel (refereegranskat)abstract
    • Non-fullerene based organic solar cells display a high initial power conversion efficiency but continue to suffer from poor thermal stability, especially in case of devices with thick active layers. Mixing of five structurally similar acceptors with similar electron affinities, and blending with a donor polymer is explored, yielding devices with a power conversion efficiency of up to 17.6%. The hexanary device performance is unaffected by thermal annealing of the bulk-heterojunction active layer for at least 23 days at 130 °C in the dark and an inert atmosphere. Moreover, hexanary blends offer a high degree of thermal stability for an active layer thickness of up to 390 nm, which is advantageous for high-throughput processing of organic solar cells. Here, a generic strategy based on multi-component acceptor mixtures is presented that permits to considerably improve the thermal stability of non-fullerene based devices and thus paves the way for large-area organic solar cells. 
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