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1.
  • Carlström, Stefanos, et al. (författare)
  • Spatially and spectrally resolved quantum path interference with chirped driving pulses
  • 2016
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 18:12
  • Tidskriftsartikel (refereegranskat)abstract
    • We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. The structures are of two kinds; off-axis interference from the long trajectory only and on-axis interference including the short and long trajectories. The former is readily visible in the far-field spectrum, modulating both the spectral and spatial profile. To access the latter, we vary the chirp of the fundamental, imparting different phases on the different trajectories, thereby changing their relative phase. Using this method together with an analytical model, we are able to explain the on-axis behaviour and access the dipole phase parameters for the short (${\alpha }_{{\rm{s}}}$) and long (${\alpha }_{{\rm{l}}}$) trajectories. The extracted results compare very well with phase parameters calculated by solving the time-dependent Schrödinger equation. Going beyond the analytical model, we are also able to successfully reproduce the off-axis interference structure.
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2.
  • Kanski, Janusz, 1946, et al. (författare)
  • Electronic structure of (Ga,Mn)As revisited
  • 2017
  • Ingår i: New Journal of Physics. - : Institute of Physics (IOP). - 1367-2630. ; 19:2, s. 1-8
  • Tidskriftsartikel (refereegranskat)abstract
    • The detailed nature of electronic states mediating ferromagnetic coupling in dilute magnetic semiconductors, specifically (Ga,Mn)As, has been an issue of long debate. Two confronting models have been discussed emphasizing host band vs. impurity band carriers. Using angle resolved photoemission we show that the electronic structure of the (Ga,Mn)As system is significantly modified from that of GaAs throughout the valence band. Close to the Fermi energy, the presence of Mn induces a strong mixing of the bulk bands of GaAs, which results in the appearance of a highly dispersive band in the gap region of GaAs.For Mn concentrations above 1% the band reaches the Fermi level, and can thus host the delocalized holes needed for ferromagnetic coupling. Overall, our data provide a firm evidence of delocalized carriers belonging to the modified host valence band.
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3.
  • Konopik, Michael, et al. (författare)
  • Solving the subset sum problem with a nonideal biological computer
  • 2021
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:9
  • Tidskriftsartikel (refereegranskat)abstract
    • We consider the solution of the subset sum problem based on a parallel computer consisting of self-propelled biological agents moving in a nanostructured network that encodes the computing task in its geometry. We develop an approximate analytical method to analyze the effects of small errors in the nonideal junctions composing the computing network by using a Gaussian confidence interval approximation of the multinomial distribution. We concretely evaluate the probability distribution for error-induced paths and determine the minimal number of agents required to obtain a proper solution. We finally validate our theoretical results with exact numerical simulations of the subset sum problem for different set sizes and error probabilities, and discuss the scalability of the nonideal problem using realistic experimental error probabilities.
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4.
  • Small, Lara S.R., et al. (författare)
  • The bar-hinge motor : A synthetic protein design exploiting conformational switching to achieve directional motility
  • 2019
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 21:1
  • Tidskriftsartikel (refereegranskat)abstract
    • One challenge to synthetic biology is to design functional machines from natural building blocks, from individual amino acids up to larger motifs such as the coiled coil. Here we investigate a novel bipedal motor concept, the Bar-Hinge Motor (BHM), a peptide-based motor capable of executing directed motion via externally controlled conformational switching between a straight bar and a V-shaped hinged form. Incorporating ligand-regulated binding to a DNA track and periodic control of ligand supply makes the BHM an example of a 'clocked walker'. Here, we employ a coarse-grained computational model for the BHM to assess the feasibility of a proposed experimental realization, with conformational switching regulated through the photoisomerization of peptide-bound azobenzene molecules. The results of numerical simulations using the model show that the incorporation of this conformational switch is necessary for the BHM to execute directional, rather than random, motion on a one-dimensional track. The power-stroke-driven directed motion is seen in the model even under conditions that underestimate the level of control we expect to be able to produce in the experimental realisation, demonstrating that this type of design should be an excellent vehicle for exploring the physics behind protein motion. By investigating its force-dependent dynamics, we show that the BHM is capable of directional motion against an applied load, even in the more relaxed conformational switching regimes. Thus, BHM appears to be an excellent candidate for a motor design incorporating a power stroke, enabling us to explore the ability of switchable coiled-coil designs to deliver power strokes within synthetic biology.
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5.
  • Morrison, S, et al. (författare)
  • Physical replicas and the Bose glass in cold atomic gases
  • 2008
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 10:7
  • Tidskriftsartikel (refereegranskat)abstract
    • We study cold atomic gases in a disorder potential and analyse the correlations between different systems subjected to the same disorder landscape. Such independent copies with the same disorder landscape are known as replicas. While, in general, these are not accessible experimentally in condensed matter systems, they can be realized using standard tools for controlling cold atomic gases in an optical lattice. Of special interest is the overlap function which represents a natural order parameter for disordered systems and is a correlation function between the atoms of two independent replicas with the same disorder. We demonstrate an efficient measurement scheme for the determination of this disorder-induced correlation function. As an application, we focus on the disordered Bose–Hubbard model and determine the overlap function within the perturbation theory and a numerical analysis. We find that the measurement of the overlap function allows for the identification of the Bose-glass phase in certain parameter regimes.
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6.
  • Alegret, Joan, 1977, et al. (författare)
  • Green's tensor calculations of plasmon resonances of single holes and hole pairs in thin gold films
  • 2008
  • Ingår i: New Journal of Physics. - Bristol, UK : IOP Publishing. - 1367-2630. ; 10, s. 13-
  • Tidskriftsartikel (refereegranskat)abstract
    • We present numerical calculations of the plasmon properties of single-hole and hole-pair structures in optically thin gold films obtained with the Green's tensor formalism for stratified media. The method can be used to obtain the optical properties of a given hole system, without problems associated with the truncation of the infinite metal film. The calculations are compared with previously published experimental data and an excellent agreement is found. In particular, the calculations are shown to reproduce the evolution of the hole plasmon resonance spectrum as a function of hole diameter, film thickness and hole separation.
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7.
  • Aurand, Bastian, et al. (författare)
  • Radiation pressure-assisted acceleration of ions using multi-component foils in high-intensity laser-matter interactions
  • 2013
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 15
  • Tidskriftsartikel (refereegranskat)abstract
    • Experimental results on the acceleration of protons and carbon ions from ultra-thin polymer foils at intensities of up to 6x10(19)Wcm(-2) are presented revealing quasi-monoenergetic spectral characteristics for different ion species at the same time. For carbon ions and protons, a linear correlation between the cutoff energy and the peak energy is observed when the laser intensity is increased. Particle-in-cell simulations supporting the experimental results imply an ion acceleration mechanism driven by the radiation pressure as predicted for multi-component foils at these intensities.
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8.
  • Favre-Nicolin, V., et al. (författare)
  • Analysis of strain and stacking faults in single nanowires using Bragg coherent diffraction imaging
  • 2010
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 12
  • Tidskriftsartikel (refereegranskat)abstract
    • Coherent diffraction imaging (CDI) on Bragg reflections is a promising technique for the study of three-dimensional (3D) composition and strain fields in nanostructures, which can be recovered directly from the coherent diffraction data recorded on single objects. In this paper, we report results obtained for single homogeneous and heterogeneous nanowires with a diameter smaller than 100 nm, for which we used CDI to retrieve information about deformation and faults existing in these wires. We also discuss the influence of stacking faults, which can create artefacts during the reconstruction of the nanowire shape and deformation.
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9.
  • Foerster, Heidi, et al. (författare)
  • Current-voltage correlations in interferometers
  • 2007
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 9
  • Tidskriftsartikel (refereegranskat)abstract
    • We investigate correlations of current at contacts and voltage fluctuations at voltage probes coupled to interferometers. The results are compared with correlations of current and occupation number fluctuations at dephasing probes. We use a quantum Langevin approach for the average quantities and their fluctuations. For higher order correlations we develop a stochastic path integral approach and find the generating functions of voltage or occupation number fluctuations. We also derive a generating function for the joint distribution of voltage or occupation number at the probe and current fluctuations at a terminal of a conductor. For energy independent scattering we found earlier that the generating function of current cumulants in interferometers with a one-channel dephasing or voltage probe are identical. Nevertheless, the distribution function for voltage and the distribution function for occupation number fluctuations differ, the latter being broader than that of the former in all examples considered here.
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10.
  • Helsing, Johan, et al. (författare)
  • Spectral super-resolution in metamaterial composites
  • 2011
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 13:11
  • Tidskriftsartikel (refereegranskat)abstract
    • We investigate the optical properties of periodic composites containing metamaterial inclusions in a normal material matrix. We consider the case when these inclusions have sharp corners and, following Hetherington and Thorpe, use analytic results to argue that it is then possible to deduce the shape of the corner (its included angle) by measurements of the absorptance of such composites when the scale size of the inclusions and period cell is much finer than the wavelength. These analytic arguments are supported by highly accurate numerical results for the effective permittivity function of such composites as a function of the permittivity ratio of inclusions to the matrix. The results show that this function has a continuous spectral component with limits independent of the area fraction of inclusions, and with the same limits for both square and staggered square arrays. For staggered arrays where the squares are almost touching, the absorption spectrum is an extremely sensitive probe of the inclusion separation distance and acts like a Vernier scale.
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11.
  • Lindblad, Andreas, et al. (författare)
  • Vibrational scattering anisotropy in O-2-dynamics beyond the Born-Oppenheimer approximation
  • 2012
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 14, s. 113018-
  • Tidskriftsartikel (refereegranskat)abstract
    • Born-Oppenheimer and Franck-Condon approximations are two major concepts in the interpretation of electronic excitations and modeling of spectroscopic data in the gas and condensed phases. We report large variations of the anisotropy parameter (beta) for the fully resolved vibrational sub-states of the X-2 Pi(g) electronic ground state of O-2(+) populated by participator resonant Auger decay following excitations of K-shell electrons into the sigma(star) resonance by monochromatic x-rays. Decay spectra for light polarization directions parallel and perpendicular to the electron detection axis recorded at four different excitation energies in the vicinity of the O 1s -> sigma(star) transition are presented. Breakdown of the Born-Oppenheimer approximation is for the first time selectively observed for the lower vibrational sub-states, where two quantum paths-resonant and direct-leading to the same final cationic state exist. The higher vibrational sub-states can only be populated by resonant photoemission; hence no interference between these channels can occur.
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12.
  • Mansten, Erik, et al. (författare)
  • Spectral shaping of attosecond pulses using two-colour laser fields
  • 2008
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 10
  • Tidskriftsartikel (refereegranskat)abstract
    • We use a strong two-colour laser field composed of the fundamental (800 nm) and the second harmonic (400 nm) of an infrared (IR) laser field to generate attosecond pulses with controlled spectral and temporal properties. With a second-harmonic intensity equal to 15% of the IR intensity the second-harmonic field is strong enough to significantly alter and control the electron trajectories in the generation process. This enables us to tune the central photon energy of the attosecond pulses by changing the phase difference between the IR and the second-harmonic fields. In the time domain the radiation is emitted as a sequence of pulses separated by a full IR cycle. We also perform calculations showing that the effect of even stronger second-harmonic fields leads to an extended tunable range under conditions that are experimentally feasible.
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13.
  • Reimann, Stephanie, et al. (författare)
  • Rotating quantum liquids crystallize
  • 2006
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 8
  • Tidskriftsartikel (refereegranskat)abstract
    • Small crystallites form when finite quantal systems are set highly rotating. This crystallization is independent of the statistics of the particles, and occurs for both trapped bosons and fermions. The spin degree of freedom does not change the tendency for localization. In a highly rotating state, the strongly correlated bosonic and fermionic systems approach to that of classical particles.
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14.
  • Stierle, A., et al. (författare)
  • Real time observation of ultrathin epitaxial oxide growth during alloy oxidation
  • 2007
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 9, s. 331-331
  • Tidskriftsartikel (refereegranskat)abstract
    • We have studied the thermal oxidation of the intermetallic alloy CoGa in situ, in real time on the atomic scale, during the growth of an ultrathin, epitaxial Ga oxide layer. On the basis of an extended set of surface x-ray diffraction data, density functional theory calculations and core level spectroscopy data, we find that the oxide film consists of an oxygen ion double layer, which contains the basic building block of bulk beta- Ga2O3. The oxide formation takes place via the nucleation of two- dimensional, anisotropic oxide islands which laterally grow and coalesce. A dramatic increase of the oxide island size is observed for low O-2 pressures in the 10(-8) mbar regime, which we interpret as the onset of a step flow like growth mode. This allows us to conclude that thermal oxidation can be considered as a hetero- epitaxial growth process, that follows similar atomistic growth principles to molecular beam epitaxy. As a consequence, the structural perfection of the oxide layer can be tailored by the appropriate choice of oxygen pressure and temperature.
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15.
  • Söderström, Johan, 1978-, et al. (författare)
  • Angle-resolved electron spectroscopy of the resonant Auger decay in xenon with meV energy resolution
  • 2011
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 13, s. 073014-
  • Tidskriftsartikel (refereegranskat)abstract
    • The angle-resolved resonant Auger spectrum of Xe is investigated with a record high meV energy resolution in the kinetic energy region of 34.45-39.20 eV at hv = 65.110 eV, corresponding to the resonant excitation of the Auger Xe* 4d(5/2)(-1)6p state. New lines have been observed and assigned in the spectra. The results of previous measurements concerning energies, intensities and angular distribution asymmetry parameters have been refined, complemented and, for some of the lines, corrected.
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16.
  • Baba, S., et al. (författare)
  • Cooper-pair splitting in two parallel InAs nanowires
  • 2018
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 20:6
  • Tidskriftsartikel (refereegranskat)abstract
    • We report on the fabrication and electrical characterization of an InAs double-nanowire (NW) device consisting of two closely placed parallel NWs coupled to a common superconducting electrode on one side and individual normal metal leads on the other. In this new type of device we detect Cooper-pair splitting (CPS) with a sizeable efficiency of correlated currents in both NWs. In contrast to earlier experiments, where CPS was realized in a single NW, demonstrating an intrawire electron pairing mediated by the superconductor (SC), our experiment demonstrates an interwire interaction mediated by the common SC. The latter is the key for the realization of zero-magnetic field Majorana bound states, or Parafermions; in NWs and therefore constitutes a milestone towards topological superconductivity. In addition, we observe transport resonances that occur only in the superconducting state, which we tentatively attribute to Andreev bound states and/or Yu-Shiba resonances that form in the proximitized section of one NW.
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17.
  • Bender, P., et al. (författare)
  • Distribution functions of magnetic nanoparticles determined by a numerical inversion method
  • 2017
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 19:7
  • Tidskriftsartikel (refereegranskat)abstract
    • In the present study, we applied a regularized inversion method to extract the particle size, magnetic moment and relaxation-time distribution of magnetic nanoparticles from small-angle x-ray scattering (SAXS), DC magnetization (DCM) and AC susceptibility (ACS) measurements. For the measurements the particles were colloidally dispersed in water. At first approximation the particles could be assumed to be spherically shaped and homogeneously magnetized single-domain particles. As model functions for the inversion, we used the particle form factor of a sphere (SAXS), the Langevin function (DCM) and the Debye model (ACS). The extracted distributions exhibited features/peaks that could be distinctly attributed to the individually dispersed and non-interacting nanoparticles. Further analysis of these peaks enabled, in combination with a prior characterization of the particle ensemble by electron microscopy and dynamic light scattering, a detailed structural and magnetic characterization of the particles. Additionally, all three extracted distributions featured peaks, which indicated deviations of the scattering (SAXS), magnetization (DCM) or relaxation (ACS) behavior from the one expected for individually dispersed, homogeneously magnetized nanoparticles. These deviations could be mainly attributed to partial agglomeration (SAXS, DCM, ACS), uncorrelated surface spins (DCM) and/or intra-well relaxation processes (ACS). The main advantage of the numerical inversion method is that no ad hoc assumptions regarding the line shape of the extracted distribution functions are required, which enabled the detection of these contributions. We highlighted this by comparing the results with the results obtained by standard model fits, where the functional form of the distributions was a priori assumed to be log-normal shaped.
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18.
  • Boeyens, Julia, et al. (författare)
  • Probe thermometry with continuous measurements
  • 2023
  • Ingår i: New Journal of Physics. - 1367-2630. ; 25:12
  • Tidskriftsartikel (refereegranskat)abstract
    • Temperature estimation plays a vital role across natural sciences. A standard approach is provided by probe thermometry, where a probe is brought into contact with the sample and examined after a certain amount of time has passed. In situations where, for example, preparation of the probe is non-trivial or total measurement time of the experiment is the main resource that must be optimized, continuously monitoring the probe may be preferred. Here, we consider a minimal model, where the probe is provided by a two-level system coupled to a thermal reservoir. Monitoring thermally activated transitions enables real-time estimation of temperature with increasing accuracy over time. Within this framework we comprehensively investigate thermometry in both bosonic and fermionic environments employing a Bayesian approach. Furthermore, we explore adaptive strategies and find a significant improvement on the precision. Additionally, we examine the impact of noise and find that adaptive strategies may suffer more than non-adaptive ones for short observation times. While our main focus is on thermometry, our results are easily extended to the estimation of other environmental parameters, such as chemical potentials and transition rates.
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19.
  • Dorsch, Sven, et al. (författare)
  • Characterization of electrostatically defined bottom-heated InAs nanowire quantum dot systems
  • 2021
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:12
  • Tidskriftsartikel (refereegranskat)abstract
    • Conversion of temperature gradients to charge currents in quantum dot systems enables probing various concepts from highly efficient energy harvesting and fundamental thermodynamics to spectroscopic possibilities complementary to conventional bias device characterization. In this work, we present a proof-of-concept study of a device architecture where bottom-gates are capacitively coupled to an InAs nanowire and double function as local joule heaters. The device design combines the ability to heat locally at different locations on the device with the electrostatic definition of various quantum dot and barrier configurations. We demonstrate the versatility of this combined gating- and heating approach by studying, as a function of the heater location and bias, the Seebeck effect across the barrier-free nanowire, fit thermocurrents through quantum dots for thermometry and detect the phonon energy using a serial double quantum dot. The results indicate symmetric heating effects when the device is heated with different gates and we present detection schemes for the electronic and phononic heat transfer contribution across the nanowire. Based on this proof-of-principle work, we propose a variety of future experiments.
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20.
  • Düsterer, S, et al. (författare)
  • Two-color XUV+NIR femtosecond photoionization of neon in the near-threshold region
  • 2019
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 21
  • Tidskriftsartikel (refereegranskat)abstract
    • Results of angle-resolved electron spectroscopy of near-threshold photoionization of Ne atoms by combined femtosecond extreme ultraviolet and near infrared fields are presented. The dressed-electron spectra show an energetic distribution into so-called sidebands, being separated by the photon energy of the dressing laser. Surprisingly, for the low kinetic energy (few eV) sidebands, the photoelectron energy varies as a function of the emission angle. Such behavior has not yet been observed in sideband creation and has not been predicted in commonly used theoretical descriptions such as strong field approximation and soft photon approach. Describing the photoionization with a time-dependent Schrödinger equation allows a qualitative description of the observed effect, as well as the prediction of fine structure in the sideband distribution.
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21.
  • Dzhigaev, D, et al. (författare)
  • Three-dimensional coherent x-ray diffraction imaging of ferroelastic domains in single CsPbBr3 perovskite nanoparticles
  • 2021
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:6
  • Tidskriftsartikel (refereegranskat)abstract
    • Metal halide perovskites attract significant interest due to their remarkable performance in optoelectronic devices. However, the gap in understanding the relationship between their nanoscale structure and properties limits their application towards novel devices. In this work, twinned ferroelastic domains in single 500 nm CsPbBr3 particles are studied with 3D Bragg coherent x-ray diffraction imaging. A preferential double-domain structure is revealed in four identical particles, with one domain oriented along the [110] and the other along the [002] direction. The particles exhibit similar scattering volume ratios of 0.12 0.026 between twin phases, suggesting the possibility of a deterministic formation process. The domains exhibit a difference in lattice tilt of 0.59 degrees, in excellent agreement with calculations of the lattice mismatch at the (112) twin boundary. These results provide important insights both for the fundamental understanding of ferroelastic nanoscale materials and for the performance improvement of perovskite-based devices. Moreover, this work paves the way towards real-time imaging of the domain dynamics in ferroic systems.
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22.
  • Francesco Diotallevi, Giovanni, et al. (författare)
  • Steady-state entanglement production in a quantum thermal machine with continuous feedback control
  • 2024
  • Ingår i: New Journal of Physics. - 1367-2630. ; 26:5
  • Tidskriftsartikel (refereegranskat)abstract
    • Quantum thermal machines can generate steady-state entanglement by harvesting spontaneous interactions with local environments. However, using minimal resources and control, the entanglement is typically weak. Here, we study entanglement generation in a two-qubit quantum thermal machine in the presence of a continuous feedback protocol. Each qubit is measured continuously and the outcomes are used for real-time feedback to control the local system-environment interactions. We show that there exists an ideal operation regime where the quality of entanglement is significantly improved, to the extent that it can violate standard Bell inequalities and uphold quantum teleportation. In agreement with (Khandelwal et al 2020 New J. Phys. 22 073039), we also find, for ideal operation, that the heat current across the system is proportional to the entanglement concurrence. Finally, we investigate the robustness of entanglement production when the machine operates away from the ideal conditions.
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23.
  • Gallardo González, I., et al. (författare)
  • Effects of the dopant concentration in laser wakefield and direct laser acceleration of electrons
  • 2018
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 20:5
  • Tidskriftsartikel (refereegranskat)abstract
    • In this work, we experimentally study the effects of the nitrogen concentration in laser wakefield acceleration of electrons in a gas mixture of hydrogen and nitrogen. A 15 TW peak power laser pulse is focused to ionize the gas, excite a plasma wave and accelerate electrons up to 230 MeV. We find that at dopant concentrations above 2% the total divergence of the electrons is increased and the high energy electrons are emitted preferentially with an angle of ±6 mrad, leading to a forked spatio-spectral distribution associated to direct laser acceleration (DLA). However, electrons can gain more energy and have a divergence lower than 4 mrad for concentrations below 0.5% and the same laser and plasma conditions. Particle-in-cell simulations show that for dopant concentrations above 2%, the amount of trapped charge is large enough to significantly perturb the plasma wave, reducing the amplitude of the longitudinal wakefield and suppressing other trapping mechanisms. At high concentrations the number of trapped electrons overlapping with the laser fields is increased, which rises the amount of charge affected by DLA. We conclude that the dopant concentration affects the quantity of electrons that experience significant DLA and the beam loading of the plasma wave driven by the laser pulse. These two mechanisms influence the electrons final energy, and thus the dopant concentration should be considered as a factor for the optimization of the electron beam parameters.
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24.
  • Gower, Artur, et al. (författare)
  • Effective waves for random three-dimensional particulate materials
  • 2021
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 23:6
  • Tidskriftsartikel (refereegranskat)abstract
    • How do you take a reliable measurement of a material whose microstructure is random? When using wave scattering, the answer is often to take an ensemble average (average over time or space). By ensemble averaging we can calculate the average scattered wave and the effective wavenumber. To date, the literature has focused on calculating the effective wavenumber for a plate filled with particles. One clear unanswered question was how to extend this approach to a material of any geometry and for any source. For example, does the effective wavenumber depend on only the microstructure, or also on the material geometry? In this work, we demonstrate that the effective wavenumbers depend on only microstructure, though beyond the long wavelength limit there are multiple effective wavenumbers for one fixed incident frequency. We show how to calculate the average wave scattered from a random particulate material of any shape, and for broad frequency ranges. As an example, we show how to calculate the average wave scattered from a sphere filled with particles.
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25.
  • Gustafsson, Mats, et al. (författare)
  • Upper bounds on absorption and scattering
  • 2020
  • Ingår i: New Journal of Physics. - : IOP Publishing. - 1367-2630. ; 22:7
  • Tidskriftsartikel (refereegranskat)abstract
    • A general framework for determining fundamental bounds in nanophotonics is introduced in this paper. The theory is based on convex optimization of dual problems constructed from operators generated by electromagnetic integral equations. The optimized variable is a contrast current defined within a prescribed region of a given material constitutive relations. Two power conservation constraints analogous to the optical theorem are utilized to tighten the bounds and to prescribe either losses or material properties. Thanks to the utilization of matrix rank-1 updates, modal decompositions, and model order reduction techniques, the optimization procedure is computationally efficient even for complicated scenarios. No dual gaps are observed. The method is well-suited to accommodate material anisotropy and inhomogeneity. To demonstrate the validity of the method, bounds on scattering, absorption, and extinction cross sections are derived first and evaluated for several canonical regions. The tightness of the bounds is verified by comparison to optimized spherical nanoparticles and shells. The next metric investigated is bi-directional scattering studied closely on a particular example of an electrically thin slab. Finally, the bounds are established for Purcell's factor and local field enhancement where a dimer is used as a practical example.
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