| 1. |
- Echle, Georg, et al.
(författare)
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Optimized spectral microwindows for data analysis of the Michelson Interferometer for Passive Atmospheric Sounding on the Environmental Satellite
- 2000
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Ingår i: Applied Optics. - 1559-128X .- 2155-3165. ; 39:30, s. 5531-
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Tidskriftsartikel (refereegranskat)abstract
- For data analysis of the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) atmospheric limb emission spectroscopic experiment on Environmental Satellite microwindows, i.e., small spectral regions for data analysis, have been defined and optimized. A novel optimization scheme has been developed for this purpose that adjusts microwindow boundaries such that the total retrieval error with respect to measurement noise, parameter uncertainties, and systematic errors is minimized. Dedicated databases that contain optimized microwindows for retrieval of vertical profiles of pressure and temperature, H2O, O3, HNO3, CH4, N2O, and NO2 have been generated. Furthermore, a tool for optimal selection of subsets of predefined microwindows for specific retrieval situations has been provided. This tool can be used further for estimating total retrieval errors for a selected microwindow subset. It has been shown by use of this tool that an altitude-dependent definition of microwindows is superior to an altitude-independent definition. For computational efficiency a dedicated microwindow-related list of spectral lines has been defined that contains only those spectral lines that are of relevance for MIPAS limb sounding observations.
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| 2. |
- Funke, Bernd, et al.
(författare)
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New non-LTE retrieval method for atmospheric parameters from MIPAS/ENVISAT emission spectra at 5.3 μm
- 2002
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Ingår i: Proceedings of SPIE, the International Society for Optical Engineering. - : SPIE. - 0277-786X .- 1996-756X. ; 4539, s. 396-405
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Tidskriftsartikel (refereegranskat)abstract
- Atmospheric emissions at 5.3 μm will be measured by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), a high-resolution limb sounder on board the European polar platform ENVISAT, scheduled to be launched in 2001. Measured spectra at 5.3 μm contain information on important atmospheric quantities such as NO volume mixing ratio, thermospheric temperature, and chemical NO production rates. However, the scientific analysis of this spectral region has to deal with complex non-local thermodynamic equilibrium (non-LTE) effects. A conventional non-LTE retrieval approach using ab initio vibrational temperatures cannot be applied due to rotational and spin-orbit non-LTE of NO in the thermosphere, and the dependence of NO state populations on the NO abundance itself caused by chemical excitations. An innovative non-LTE retrieval method enabling the treatment of vibrational, rotational, and spin non-LTE as well as a dependence of the non-LTE state distribution on the retrieval target quantities has thus been developed for the MIPAS data analysis. The ability of the developed non-LTE inversion tool to retrieve NO abundance profiles, thermospheric temperature profiles, and NO mean production rates by NO2 photolysis in the stratosphere and N+O2 combination in the thermosphere is demonstrated by means of a feasibility study.
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| 3. |
- Grieco, Francesco, 1992, et al.
(författare)
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Recovery and validation of Odin/SMR long-term measurements of mesospheric carbon monoxide
- 2020
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 13:9, s. 5013-5031
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Tidskriftsartikel (refereegranskat)abstract
- The Sub-Millimetre Radiometer (SMR) on board the Odin satellite performs limb sounding measurements of the middle atmosphere to detect molecular emission from different species. Carbon monoxide (CO) is an important tracer of atmospheric dynamics at these altitudes, due to its long photochemical lifetime and high vertical concentration gradient. In this study, we have successfully recovered over 18 years of SMR observations, providing the only dataset to date being so extended in time and stretching out to the polar regions, with regards to satellite-measured mesospheric CO. This new dataset is part of the Odin/SMR version 3.0 level 2 data. Much of the level 1 dataset - except the October 2003 to October 2004 period - was affected by a malfunctioning of the phase-lock loop (PLL) in the front end used for CO observations. Because of this technical issue, the CO line could be shifted away from its normal frequency location, causing the retrieval to fail or leading to an incorrect estimation of the CO concentration. An algorithm was developed to locate the CO line and shift it to its correct location. Nevertheless, another artefact causing an underestimation of the concentration, i.e. a line broadening, stemmed from the PLL malfunctioning. This was accounted for by using a broader response function. The application of these corrections resulted in the recovery of a large amount of data that was previously being flagged as problematic and therefore not processed. A validation study has been carried out, showing how SMR CO volume mixing ratios are in general in good accordance with the other instruments considered in the study. Overall, the agreement is very good between 60 and 80 km altitude, with relative differences close to zero. A positive bias at low altitudes (50-60 km) up to +20% and a negative bias up to -20% at high altitudes (80-100 km) were found with respect to the comparison instruments.
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| 4. |
- Hegglin, Michaela I., et al.
(författare)
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Overview and update of the SPARC Data Initiative: comparison of stratospheric composition measurements from satellite limb sounders
- 2021
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Ingår i: Earth System Science Data. - : Copernicus GmbH. - 1866-3516 .- 1866-3508. ; 13:5, s. 1855-1903
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Forskningsöversikt (refereegranskat)abstract
- The Stratosphere-troposphere Processes and their Role in Climate (SPARC) Data Initiative (SPARC, 2017) performed the first comprehensive assessment of currently available stratospheric composition measurements obtained from an international suite of space-based limb sounders. The initiative's main objectives were (1) to assess the state of data availability, (2) to compile time series of vertically resolved, zonal monthly mean trace gas and aerosol fields, and (3) to perform a detailed intercomparison of these time series, summarizing useful information and highlighting differences among datasets. The datasets extend over the region from the upper troposphere to the lower mesosphere (300-0.1 hPa) and are provided on a common latitude-pressure grid. They cover 26 different atmospheric constituents including the stratospheric trace gases of primary interest, ozone (O-3) and water vapor (H2O), major long-lived trace gases (SF6, N2O, HF, CCl3F, CCl2F2, NO y), trace gases with intermediate lifetimes (HCl, CH4, CO, HNO3), and shorter-lived trace gases important to stratospheric chemistry including nitrogen-containing species (NO, NO2, NOx, N2O5, HNO4), halogens (BrO, ClO, ClONO2, HOCl), and other minor species (OH, HO2, CH2O, CH3CN), and aerosol. This overview of the SPARC Data Initiative introduces the updated versions of the SPARC Data Initiative time series for the extended time period 1979-2018 and provides information on the satellite instruments included in the assessment: LIMS, SAGE I/II/III, HALOE, UARS-MLS, POAM II/III, OSIRIS, SMR, MIPAS, GOMOS, SCIAMACHY, ACE-FTS, ACEMAESTRO, Aura-MLS, HIRDLS, SMILES, and OMPS-LP. It describes the Data Initiative's top-down climatological validation approach to compare stratospheric composition measurements based on zonal monthly mean fields, which provides upper bounds to relative inter-instrument biases and an assessment of how well the instruments are able to capture geophysical features of the stratosphere. An update to previously published evaluations of O-3 and H2O monthly mean time series is provided. In addition, example trace gas evaluations of methane (CH4), carbon monoxide (CO), a set of nitrogen species (NO, NO2, and HNO3), the reactive nitrogen family (NOy), and hydroperoxyl (HO2) are presented. The results highlight the quality, strengths and weaknesses, and representativeness of the different datasets. As a summary, the current state of our knowledge of stratospheric composition and variability is provided based on the overall consistency between the datasets. As such, the SPARC Data Initiative datasets and evaluations can serve as an atlas or reference of stratospheric composition and variability during the "golden age" of atmospheric limb sounding. The updated SPARC Data Initiative zonal monthly mean time series for each instrument are publicly available and accessible via the Zenodo data archive (Hegglin et al., 2020).
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| 5. |
- Hendrickx, Koen, 1990-
(författare)
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Solar Forcing of Nitric Oxide in the Upper Atmosphere
- 2018
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Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- The forcing of the Sun on Earth's atmosphere manifests itself via solar radiation and energetic particle precipitation (EPP), which variations are most noticeable in the upper regions of the atmosphere. A key species in the lower thermosphere, which is influenced by solar forcing, is nitric oxide (NO). An NO reservoir is present in the lower thermosphere, from which NO-rich air can be transported downward into the mesosphere and stratosphere, where it takes part in catalytic ozone destruction cycles. For climate models to correctly simulate the solar forcing on our climate, the processes of NO production and destruction, as well as the descent into the lower atmosphere, must be understood and accurately represented.In this thesis, observations from the Solar Occultation For Ice Experiment (SOFIE) instrument onboard the Aeronomy of Ice in the Mesosphere (AIM) satellite are used to investigate temporal characteristics of NO in the mesosphere and lower thermosphere. We have developed a diagnostic method to determine the relative importance of the NO physical drivers throughout the lower thermosphere. The method shows that, at high latitudes, precipitating auroral electrons dominantly drive NO variations. Comparisons with NO measurements by the Student Nitric Oxide Experiment (SNOE), made almost a decade earlier, reveal that the impact of this forcing on NO appears to be invariant throughout the 11 year solar cycle.On shorter timescales, we have shown a clear signature of the reoccurring 27 day geomagnetic impact on NO concentrations during summer and winter, with subsequent descent into the lower mesosphere during winter. The occurrence of medium energy electrons, which precipitate to mesospheric altitudes, results in a further increase of the descending NO flux. This complicates the determination of the relative contribution of the EPP direct and indirect effect on NO, i.e. separating direct NO production from downwards transported NO, respectively, in NO enhancements at a certain altitude. Using a full-range energy spectrum from the Polar-orbiting Operational Environmental Satellites (POES), we have been able to disentangle the direct and indirect EPP effect on Southern hemispheric NO during a geomagnetic storm in 2010.Simulations of NO by the Whole Atmosphere Community Climate Model with Specified Dynamics (SD-WACCM) model reveal that the model predicts a too high climatological mean, while the short term variability is too low, as compared to SOFIE. However, even though the dynamical transport in both model and observations agrees very well, the descending NO fluxes are too low in the model.In conclusion, the results of this thesis provide a better understanding of NO variability from an observational standpoint and will enable better model representations in the future.
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| 6. |
- Lahtinen, Atte K., et al.
(författare)
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Decreased spermatogonial numbers in boys with severe haematological diseases
- 2024
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Ingår i: British Journal of Haematology. - : John Wiley & Sons. - 0007-1048 .- 1365-2141. ; 205:1, s. 229-235
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Tidskriftsartikel (refereegranskat)abstract
- This study examines spermatogonial numbers in testicular samples from 43 prepubertal patients undergoing haematopoietic stem cell transplantation (HSCT). High-dose chemotherapy and/or radiation during HSCT can impact spermatogenesis requiring fertility preservation. Results show that 49% of patients have decreased and 19% severely depleted spermatogonial pool prior to HSCT. Patients with Fanconi anaemia exhibit significantly reduced spermatogonial numbers. Patients with immunodeficiency or aplastic anaemia generally present within the normal range, while results in patients with myelodysplastic syndrome or myeloproliferative neoplasm vary. The study emphasizes the importance of assessing spermatogonial numbers in patients with severe haematological diseases for informed fertility preservation decisions.
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| 7. |
- Larsson, Richard
(författare)
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Modeling the Zeeman Effect in Planetary Atmospheric Radiative Transfer
- 2014
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Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
- There are special effects in spectroscopy that must be considered in order to fullyexplain how molecular oxygen interacts with radiation in planetary atmospheres.One of these, the Zeeman effect, is described in this thesis. The Zeeman effect is the theory by which energy levels of atoms and molecules are altered by magnetism, and it causes both polarization and line shape to change. The first publication attached to this thesis, Paper I, details the technical and practical implementation of the Zeeman effect in a radiative transfer model. One potential use of magnetically altered spectroscopy is to remotely measure magnetism. Paper II discuss a method for such measurements on weakly magnetized planets by measuring the polarization caused by the Zeeman effect. The article brings up Mars as one potential candidate to utilize the method. To introduce the articles properly, the thesis starts with a shortdescription of the underlying basic theory for radiative transfer and spectroscopy.After the theory chapter, a short description of input necessary to utilize the theory on operational and experimental platforms is presented.
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| 8. |
- Mlynczak, Martin G., et al.
(författare)
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Energy transport in the thermosphere during the solar storms of April 2002
- 2005
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Ingår i: Journal of Geophysical Research - Space Physics. - 2169-9380 .- 2169-9402. ; 110:A12
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Tidskriftsartikel (refereegranskat)abstract
- The dramatic solar storm events of April 2002 deposited a large amount of energy into the Earth's upper atmosphere, substantially altering the thermal structure, the chemical composition, the dynamics, and the radiative environment. We examine the flow of energy within the thermosphere during this storm period from the perspective of infrared radiation transport and heat conduction. Observations from the SABER instrument on the TIMED satellite are coupled with computations based on the ASPEN thermospheric general circulation model to assess the energy flow. The dominant radiative response is associated with dramatically enhanced infrared emission from nitric oxide at 5.3 μm from which a total of ∼7.7 × 1023 ergs of energy are radiated during the storm. Energy loss rates due to NO emission exceed 2200 Kelvin per day. In contrast, energy loss from carbon dioxide emission at 15 μm is only ∼2.3% that of nitric oxide. Atomic oxygen emission at 63 μm is essentially constant during the storm. Energy loss from molecular heat conduction may be as large as 3.8% of the NO emission. These results confirm the “natural thermostat” effect of nitric oxide emission as the primary mechanism by which storm energy is lost from the thermosphere below 210 km.
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| 9. |
- Mlynczak, Marty, et al.
(författare)
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The natural thermostat of nitric oxide emission at 5.3 μm in the thermosphere observed during the solar storms of April 2002
- 2003
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Ingår i: Geophysical Research Letters. - 0094-8276 .- 1944-8007. ; 30:21
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Tidskriftsartikel (refereegranskat)abstract
- The Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) experiment on the Thermosphere-Ionosphere Mesosphere Energetics and Dynamics (TIMED) satellite observed the infrared radiative response of the thermosphere to the solar storm events of April 2002. Large radiance enhancements were observed at 5.3 μm, which are due to emission from the vibration-rotation bands of nitric oxide (NO). The emission by NO is indicative of the conversion of solar energy to infrared radiation within the atmosphere and represents a "natural thermostat" by which heat and energy are efficiently lost from the thermosphere to space and to the lower atmosphere. We describe the SABER observations at 5.3 μm and their interpretation in terms of energy loss. The infrared enhancements remain only for a few days, indicating that such perturbations to the thermospheric state, while dramatic, are short-lived. Copyright 2003 by the American Geophysical Union.
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| 10. |
- Risi, Camille, et al.
(författare)
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Process-evaluation of tropospheric humidity simulated by general circulation models using water vapor isotopic observations : 2. Using isotopic diagnostics to understand the mid and upper tropospheric moist bias in the tropics and subtropics
- 2012
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Ingår i: Journal of Geophysical Research. - 0148-0227 .- 2156-2202. ; 117, s. D05304-
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Tidskriftsartikel (refereegranskat)abstract
- Evaluating the representation of processes controlling tropical and subtropical tropospheric relative humidity (RH) in atmospheric general circulation models (GCMs) is crucial to assess the credibility of predicted climate changes. GCMs have long exhibited a moist bias in the tropical and subtropical mid and upper troposphere, which could be due to the mis-representation of cloud processes or of the large-scale circulation, or to excessive diffusion during water vapor transport. The goal of this study is to use observations of the water vapor isotopic ratio to understand the cause of this bias. We compare the three-dimensional distribution of the water vapor isotopic ratio measured from space and ground to that simulated by several versions of the isotopic GCM LMDZ. We show that the combined evaluation of RH and of the water vapor isotopic composition makes it possible to discriminate the most likely cause of RH biases. Models characterized either by an excessive vertical diffusion, an excessive convective detrainment or an underestimated in situ cloud condensation will all produce a moist bias in the free troposphere. However, only an excessive vertical diffusion can lead to a reversed seasonality of the free tropospheric isotopic composition in the subtropics compared to observations. Comparing seven isotopic GCMs suggests that the moist bias found in many GCMs in the mid and upper troposphere most frequently results from an excessive diffusion during vertical water vapor transport. This study demonstrates the added value of water vapor isotopic measurements for interpreting shortcomings in the simulation of RH by climate models.
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| 11. |
- Risi, Camille, et al.
(författare)
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Process-evaluation of tropospheric humidity simulated by general circulation models using water vapor isotopologues : 1. Comparison between models and observations
- 2012
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Ingår i: Journal of Geophysical Research. - 0148-0227 .- 2156-2202. ; 117, s. D05303-
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Tidskriftsartikel (refereegranskat)abstract
- The goal of this study is to determine how H2O and HDO measurements in water vapor can be used to detect and diagnose biases in the representation of processes controlling tropospheric humidity in atmospheric general circulation models (GCMs). We analyze a large number of isotopic data sets (four satellite, sixteen ground-based remote-sensing, five surface in situ and three aircraft data sets) that are sensitive to different altitudes throughout the free troposphere. Despite significant differences between data sets, we identify some observed HDO/H2O characteristics that are robust across data sets and that can be used to evaluate models. We evaluate the isotopic GCM LMDZ, accounting for the effects of spatiotemporal sampling and instrument sensitivity. We find that LMDZ reproduces the spatial patterns in the lower and mid troposphere remarkably well. However, it underestimates the amplitude of seasonal variations in isotopic composition at all levels in the subtropics and in midlatitudes, and this bias is consistent across all data sets. LMDZ also underestimates the observed meridional isotopic gradient and the contrast between dry and convective tropical regions compared to satellite data sets. Comparison with six other isotope-enabled GCMs from the SWING2 project shows that biases exhibited by LMDZ are common to all models. The SWING2 GCMs show a very large spread in isotopic behavior that is not obviously related to that of humidity, suggesting water vapor isotopic measurements could be used to expose model shortcomings. In a companion paper, the isotopic differences between models are interpreted in terms of biases in the representation of processes controlling humidity.
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| 12. |
- Vandaele, Ann Carine, et al.
(författare)
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Martian dust storm impact on atmospheric H2O and D/H observed by ExoMars Trace Gas Orbiter
- 2019
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Ingår i: Nature. - : Springer. - 1476-4687 .- 1476-4687 .- 0028-0836. ; 568:7753, s. 521-525
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Tidskriftsartikel (övrigt vetenskapligt/konstnärligt)abstract
- Global dust storms on Mars are rare1,2 but can affect the Martian atmosphere for several months. They can cause changes in atmospheric dynamics and inflation of the atmosphere3, primarily owing to solar heating of the dust3. In turn, changes in atmospheric dynamics can affect the distribution of atmospheric water vapour, with potential implications for the atmospheric photochemistry and climate on Mars4. Recent observations of the water vapour abundance in the Martian atmosphere during dust storm conditions revealed a high-altitude increase in atmospheric water vapour that was more pronounced at high northern latitudes5,6, as well as a decrease in the water column at low latitudes7,8. Here we present concurrent, high-resolution measurements of dust, water and semiheavy water (HDO) at the onset of a global dust storm, obtained by the NOMAD and ACS instruments onboard the ExoMars Trace Gas Orbiter. We report the vertical distribution of the HDO/H2O ratio (D/H) from the planetary boundary layer up to an altitude of 80 kilometres. Our findings suggest that before the onset of the dust storm, HDO abundances were reduced to levels below detectability at altitudes above 40 kilometres. This decrease in HDO coincided with the presence of water-ice clouds. During the storm, an increase in the abundance of H2O and HDO was observed at altitudes between 40 and 80 kilometres. We propose that these increased abundances may be the result of warmer temperatures during the dust storm causing stronger atmospheric circulation and preventing ice cloud formation, which may confine water vapour to lower altitudes through gravitational fall and subsequent sublimation of ice crystals3. The observed changes in H2O and HDO abundance occurred within a few days during the development of the dust storm, suggesting a fast impact of dust storms on the Martian atmosphere.
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| 13. |
- von Clarmann, Thomas, et al.
(författare)
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Overview: Estimating and reporting uncertainties in remotely sensed atmospheric composition and temperature
- 2020
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Ingår i: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 13:8, s. 4393-4436
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Tidskriftsartikel (refereegranskat)abstract
- Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. Reported characterization data should be intercomparable between different instruments, empirically validatable, grid-independent, usable without detailed knowledge of the instrument or retrieval technique, traceable and still have reasonable data volume. The latter may force one to work with representative rather than individual characterization data. Many errors derive from approximations and simplifications used in real-world retrieval schemes, which are reviewed in this paper, along with related error estimation schemes. The main sources of uncertainty are measurement noise, calibration errors, simplifications and idealizations in the radiative transfer model and retrieval scheme, auxiliary data errors, and uncertainties in atmospheric or instrumental parameters. Some of these errors affect the result in a random way, while others chiefly cause a bias or are of mixed character. Beyond this, it is of utmost importance to know the influence of any constraint and prior information on the solution. While different instruments or retrieval schemes may require different error estimation schemes, we provide a list of recommendations which should help to unify retrieval error reporting.
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