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Sökning: WFRF:(Xie Fei)

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5.
  • Deng, Min, et al. (författare)
  • Genome-wide association analyses in Han Chinese identify two new susceptibility loci for amyotrophic lateral sclerosis
  • 2013
  • Ingår i: Nature Genetics. - : Nature Publishing Group. - 1061-4036 .- 1546-1718. ; 45:6, s. 697-
  • Tidskriftsartikel (refereegranskat)abstract
    • To identify susceptibility genes for amyotrophic lateral sclerosis (ALS), we conducted a genome-wide association study (GWAS) in 506 individuals with sporadic ALS and 1,859 controls of Han Chinese ancestry. Ninety top SNPs suggested by the current GWAS and 6 SNPs identified by previous GWAS were analyzed in an independent cohort of 706 individuals with ALS and 1,777 controls of Han Chinese ancestry. We discovered two new susceptibility loci for ALS at 1q32 (CAMK1G, rs6703183, P-combined = 2.92 x 10(-8), odds ratio (OR) = 1.31) and 22p11 (CABIN1 and SUSD2, rs8141797, P-combined = 2.35 x 10(-9), OR = 1.52). These two loci explain 12.48% of the overall variance in disease risk in the Han Chinese population. We found no association evidence for the previously reported loci in the Han Chinese population, suggesting genetic heterogeneity of disease susceptibility for ALS between ancestry groups. Our study identifies two new susceptibility loci and suggests new pathogenic mechanisms of ALS.
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6.
  • Wang, Yuan, et al. (författare)
  • Half-spectrum OFDM to quadruple the spectral efficiency of underwater wireless optical communication with digital power division multiplexing
  • 2024
  • Ingår i: Applied Optics. - : Optica Publishing Group. - 1559-128X .- 2155-3165. ; 63:9, s. 2352-2361
  • Tidskriftsartikel (refereegranskat)abstract
    • Improving the spectrum efficiency (SE) is an effective method to further enhance the data rate of bandwidthmultiplexing (NOFDM) with a compression factor of 0.5 can save half of the bandwidth without introducing any inter-carrier-interference (ICI) only if the total number of subcarriers is large enough, and we termed it as half-spectrum OFDM (HS-OFDM). To the best of our knowledge, this is the first reported work on a closed-form HS-OFDM signal in the discrete domain from the perspective of a correlation matrix. Due to the special mathematical property, no extra complex decoding algorithm is required at the HS-OFDM receiver, making it as simple as the conventional OFDM receiver. Compared with traditional OFDM, HS-OFDM can realize the same data rate, but with a larger signal-to-noise ratio (SNR) margin. To fully use the SNR resource of the communication system, we further propose a digital power division multiplexed HS-OFDM (DPDM-HS-OFDM) scheme to quadruple the SE of conventional OFDM for the bandwidth-starved UWOCs. The experimental results show that HS-OFDM can improve the receiver sensitivity by around 4 dB as opposed to conventional 4QAM-OFDM with the same data rate and SE. With the help of the DPDM-HS-OFDM scheme, the data rate of multi-user UWOC can reach up to 4.5 Gbps under the hard-decision forward error correction (HD-FEC) limit of a bit error rate (BER) of 3.8 x 10-3. Although there is some performance degradation in comparison with single-user HS-OFDM, the BER performance of multi-user DPDM-HS-OFDM is still superior to that of conventional single-user 4QAM-OFDM. Both single-user HS-OFDM and multi-user DPDM-HS-OFDM successfully achieve 2 Gbps/75 m data transmission, indicating that the DPDM-HS-OFDM scheme is of great importance in bandwidth-limited UWOC systems and has guiding significance to underwater wireless optical multiple access.
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7.
  • Wang, Yuan, et al. (författare)
  • Three Gossiping Protocols in Three-Dimensional Underwater Optical Cellular Network
  • 2023
  • Ingår i: 2023 Asia Communications and Photonics Conference/2023 International Photonics and Optoelectronics Meetings, ACP/POEM 2023. - : Institute of Electrical and Electronics Engineers (IEEE).
  • Konferensbidrag (refereegranskat)abstract
    • In this paper, three different low-complexity sector-based Gossiping routing protocols, namely Gossiping with probabilistic selection (Gossiping-PS), Gossiping with visibility priority (Gossiping-VP), and Gossiping with energy priority (Gossiping-EP), are evaluated through the three-dimensional underwater optical cellular network (UOCN). Comprehensive performance comparisons are made among the above three routing protocols in terms of the average hop, end-to-end delay, network lifetime, packet-loss rate, and energy utilization. Numerical analysis shows that Gossiping-PS significantly outperforms the other two schemes, while Gossiping-Vpand Gossiping-EP behave even worse than the standard Gossiping routing protocol under some circumstances, which is owing to the fact that the Greedy algorithm makes the best choice for the current moment instead of taking the global optimality into consideration.
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8.
  • Zhang, Tianyi, et al. (författare)
  • 19.02Gbps/25m Underwater Wireless Optical Communication Adopting Probabilistic Constellation Shaping QAM-DMT Transmission
  • 2023
  • Ingår i: 2023 Asia Communications and Photonics Conference/2023 International Photonics and Optoelectronics Meetings, ACP/POEM 2023. - : Institute of Electrical and Electronics Engineers (IEEE).
  • Konferensbidrag (refereegranskat)abstract
    • We experimentally demonstrated probabilistic constellation shaping quadrature amplitude modulation discrete multitone (PCS QAM-DMT) for 25-m underwater wireless optical communication (UWOC) system with a net data rate of 19.02Gbps. 28.1% capacity improvement is achieved in comparison with conventional bit-power loading DMT scheme. To the best of our knowledge, this is the highest net data rate ever reported for a single LD in current UWOC.
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  • 2019
  • Tidskriftsartikel (refereegranskat)
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10.
  • Arzoumanian, Doris, et al. (författare)
  • Dust polarized emission observations of NGC 6334: BISTRO reveals the details of the complex but organized magnetic field structure of the high-mass star-forming hub-filament network
  • 2021
  • Ingår i: Astronomy and Astrophysics. - : EDP Sciences. - 0004-6361 .- 1432-0746. ; 647
  • Tidskriftsartikel (refereegranskat)abstract
    • Context. Molecular filaments and hubs have received special attention recently thanks to new studies showing their key role in star formation. While the (column) density and velocity structures of both filaments and hubs have been carefully studied, their magnetic field (B-field) properties have yet to be characterized. Consequently, the role of B-fields in the formation and evolution of hub-filament systems is not well constrained. Aims. We aim to understand the role of the B-field and its interplay with turbulence and gravity in the dynamical evolution of the NGC 6334 filament network that harbours cluster-forming hubs and high-mass star formation. Methods. We present new observations of the dust polarized emission at 850 μm toward the 2 pc × 10 pc map of NGC 6334 at a spatial resolution of 0.09 pc obtained with the James Clerk Maxwell Telescope (JCMT) as part of the B-field In STar-forming Region Observations (BISTRO) survey. We study the distribution and dispersion of the polarized intensity (PI), the polarization fraction (PF), and the plane-of-The-sky B-field angle (χB_POS) toward the whole region, along the 10 pc-long ridge and along the sub-filaments connected to the ridge and the hubs. We derived the power spectra of the intensity and χBPOS along the ridge crest and compared them with the results obtained from simulated filaments. Results. The observations span 3 orders of magnitude in Stokes I and PI and 2 orders of magnitude in PF (from 0.2 to 20%). A large scatter in PI and PF is observed for a given value of I. Our analyses show a complex B-field structure when observed over the whole region ( 10 pc); however, at smaller scales (1 pc), χBPOS varies coherently along the crests of the filament network. The observed power spectrum of χBPOS can be well represented with a power law function with a slope of-1.33 ± 0.23, which is 20% shallower than that of I. We find that this result is compatible with the properties of simulated filaments and may indicate the physical processes at play in the formation and evolution of star-forming filaments. Along the sub-filaments, χBPOS rotates frombeing mostly perpendicular or randomly oriented with respect to the crests to mostly parallel as the sub-filaments merge with the ridge and hubs. This variation of the B-field structure along the sub-filaments may be tracing local velocity flows of infalling matter in the ridge and hubs. Our analysis also suggests a variation in the energy balance along the crests of these sub-filaments, from magnetically critical or supercritical at their far ends to magnetically subcritical near the ridge and hubs. We also detect an increase in PF toward the high-column density (NH2 â 1023 cm-2) star cluster-forming hubs. These latter large PF values may be explained by the increase in grain alignment efficiency due to stellar radiation from the newborn stars, combined with an ordered B-field structure. Conclusions. These observational results reveal for the first time the characteristics of the small-scale (down to 0.1 pc) B-field structure of a 10 pc-long hub-filament system. Our analyses show variations in the polarization properties along the sub-filaments that may be tracing the evolution of their physical properties during their interaction with the ridge and hubs. We also detect an impact of feedback from young high-mass stars on the local B-field structure and the polarization properties, which could put constraints on possible models for dust grain alignment and provide important hints as to the interplay between the star formation activity and interstellar B-fields.
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11.
  • Bernardini, M. G., et al. (författare)
  • Scientific prospects for spectroscopy of the gamma-ray burst prompt emission with SVOM
  • 2017
  • Ingår i: Experimental astronomy. - : SPRINGER. - 0922-6435 .- 1572-9508. ; 44:1, s. 113-127
  • Tidskriftsartikel (refereegranskat)abstract
    • SVOM (Space-based multi-band astronomical Variable Objects Monitor) is a Sino-French space mission dedicated to the study of Gamma-Ray Bursts (GRBs) in the next decade, capable to detect and localise the GRB emission, and to follow its evolution in the high-energy and X-ray domains, and in the visible and NIR bands. The satellite carries two wide-field high-energy instruments: a coded-mask gamma-ray imager (ECLAIRs; 4-150 keV), and a gamma-ray spectrometer (GRM; 15-5500 keV) that, together, will characterise the GRB prompt emission spectrum over a wide energy range. In this paper we describe the performances of the ECLAIRs and GRM system with different populations of GRBs from existing catalogues, from the classical ones to those with a possible thermal component superimposed to their non-thermal emission. The combination of ECLAIRs and the GRM will provide new insights also on other GRB properties, as for example the spectral characterisation of the subclass of short GRBs showing an extended emission after the initial spike.
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  • Ching, Tao-Chung, et al. (författare)
  • The JCMT BISTRO-2 Survey: Magnetic Fields of the Massive DR21 Filament
  • 2022
  • Ingår i: Astrophysical Journal. - : American Astronomical Society. - 1538-4357 .- 0004-637X. ; 941:2
  • Tidskriftsartikel (refereegranskat)abstract
    • We present 850 mu m dust polarization observations of the massive DR21 filament from the B-fields In STar-forming Region Observations (BISTRO) survey, using the POL-2 polarimeter and the SCUBA-2 camera on the James Clerk Maxwell Telescope. We detect ordered magnetic fields perpendicular to the parsec-scale ridge of the DR21 main filament. In the subfilaments, the magnetic fields are mainly parallel to the filamentary structures and smoothly connect to the magnetic fields of the main filament. We compare the POL-2 and Planck dust polarization observations to study the magnetic field structures of the DR21 filament on 0.1-10 pc scales. The magnetic fields revealed in the Planck data are well-aligned with those of the POL-2 data, indicating a smooth variation of magnetic fields from large to small scales. The plane-of-sky magnetic field strengths derived from angular dispersion functions of dust polarization are 0.6-1.0 mG in the DR21 filament and similar to 0.1 mG in the surrounding ambient gas. The mass-to-flux ratios are found to be magnetically supercritical in the filament and slightly subcritical to nearly critical in the ambient gas. The alignment between column density structures and magnetic fields changes from random alignment in the low-density ambient gas probed by Planck to mostly perpendicular in the high-density main filament probed by James Clerk Maxwell Telescope. The magnetic field structures of the DR21 filament are in agreement with MHD simulations of a strongly magnetized medium, suggesting that magnetic fields play an important role in shaping the DR21 main filament and subfilaments.
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14.
  • Eswaraiah, Chakali, et al. (författare)
  • The JCMT BISTRO Survey: Revealing the Diverse Magnetic Field Morphologies in Taurus Dense Cores with Sensitive Submillimeter Polarimetry
  • 2021
  • Ingår i: Astrophysical Journal Letters. - : American Astronomical Society. - 2041-8213 .- 2041-8205. ; 912:2
  • Tidskriftsartikel (refereegranskat)abstract
    • We have obtained sensitive dust continuum polarization observations at 850 μm in the B213 region of Taurus using POL-2 on SCUBA-2 at the James Clerk Maxwell Telescope as part of the B-fields in STar-forming Region Observations (BISTRO) survey. These observations allow us to probe magnetic field (B-field) at high spatial resolution (∼2000 au or ∼0.01 pc at 140 pc) in two protostellar cores (K04166 and K04169) and one prestellar core (Miz-8b) that lie within the B213 filament. Using the Davis-Chandrasekhar-Fermi method, we estimate the B-field strengths in K04166, K04169, and Miz-8b to be 38 ± 14, 44 ± 16, and 12 ± 5 μG, respectively. These cores show distinct mean B-field orientations. The B-field in K04166 is well ordered and aligned parallel to the orientations of the core minor axis, outflows, core rotation axis, and large-scale uniform B-field, in accordance with magnetically regulated star formation via ambipolar diffusion taking place in K04166. The B-field in K04169 is found to be ordered but oriented nearly perpendicular to the core minor axis and large-scale B-field and not well correlated with other axes. In contrast, Miz-8b exhibits a disordered B-field that shows no preferred alignment with the core minor axis or large-scale field. We found that only one core, K04166, retains a memory of the large-scale uniform B-field. The other two cores, K04169 and Miz-8b, are decoupled from the large-scale field. Such a complex B-field configuration could be caused by gas inflow onto the filament, even in the presence of a substantial magnetic flux.
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15.
  • Han, Shengyi, et al. (författare)
  • Probiotic Gastrointestinal Transit and Colonization After Oral Administration : A Long Journey
  • 2021
  • Ingår i: Frontiers in Cellular and Infection Microbiology. - : Frontiers Media S.A.. - 2235-2988. ; 11
  • Forskningsöversikt (refereegranskat)abstract
    • Orally administered probiotics encounter various challenges on their journey through the mouth, stomach, intestine and colon. The health benefits of probiotics are diminished mainly due to the substantial reduction of viable probiotic bacteria under the harsh conditions in the gastrointestinal tract and the colonization resistance caused by commensal bacteria. In this review, we illustrate the factors affecting probiotic viability and their mucoadhesive properties through their journey in the gastrointestinal tract, including a discussion on various mucosadhesion-related proteins on the probiotic cell surface which facilitate colonization.
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16.
  • Heckmann, Lea, et al. (författare)
  • Gamma-ray burst localization strategies for the SPHiNX hard x-ray polarimeter
  • 2019
  • Ingår i: JOURNAL OF ASTRONOMICAL TELESCOPES INSTRUMENTS AND SYSTEMS. - : SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS. - 2329-4124. ; 5:1
  • Tidskriftsartikel (refereegranskat)abstract
    • SPHiNX is a proposed gamma-ray burst (GRB) polarimeter mission operating in the energy range 50 to 600 keV with the aim of studying the prompt emission phase. The polarization sensitivity of SPHiNX reduces as the uncertainty on the GRB sky position increases. The stand-alone ability of the SPHiNX design to localize GRB positions is explored via Geant4 simulations. Localization at the level of a few degrees is possible using three different routines. This results in a large fraction (>80%) of observed GRBs having a negligible (<5%) reduction in polarization sensitivity due to the uncertainty in localization. 
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17.
  • Huang, Jingxuan, et al. (författare)
  • Reliable Broadcast Based on Online Fountain Codes
  • 2021
  • Ingår i: IEEE Communications Letters. - : IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC. - 1089-7798 .- 1558-2558. ; 25:2, s. 369-373
  • Tidskriftsartikel (refereegranskat)abstract
    • In this letter, we study wireless broadcast schemes based on online fountain codes. We first propose and analyze an online fountain code based-broadcast scheme, where the coded symbol degree is updated based on the decoding states of all receivers. Then we propose and analyze an improved broadcast scheme by taking advantage of the received coded symbols that are not immediately decodable. Simulation results demonstrate that our proposed scheme has better performance compared to other broadcast schemes based on feedback fountain codes.
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18.
  • Ingram, Adam, et al. (författare)
  • Tracking the X-Ray Polarization of the Black Hole Transient Swift J1727.8-1613 during a State Transition
  • 2024
  • Ingår i: Astrophysical Journal. - : American Astronomical Society. - 0004-637X .- 1538-4357. ; 968:2
  • Tidskriftsartikel (refereegranskat)abstract
    • We report on an observational campaign on the bright black hole (BH) X-ray binary Swift J1727.8-1613 centered around five observations by the Imaging X-ray Polarimetry Explorer. These observations track for the first time the evolution of the X-ray polarization of a BH X-ray binary across a hard to soft state transition. The 2-8 keV polarization degree decreased from ∼4% to ∼3% across the five observations, but the polarization angle remained oriented in the north-south direction throughout. Based on observations with the Australia Telescope Compact Array, we find that the intrinsic 7.25 GHz radio polarization aligns with the X-ray polarization. Assuming the radio polarization aligns with the jet direction (which can be tested in the future with higher-spatial-resolution images of the jet), our results imply that the X-ray corona is extended in the disk plane, rather than along the jet axis, for the entire hard intermediate state. This in turn implies that the long (≳10 ms) soft lags that we measure with the Neutron star Interior Composition ExploreR are dominated by processes other than pure light-crossing delays. Moreover, we find that the evolution of the soft lag amplitude with spectral state does not follow the trend seen for other sources, implying that Swift J1727.8-1613 is a member of a hitherto undersampled subpopulation.
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19.
  • Karoly, Janik, et al. (författare)
  • The JCMT BISTRO Survey: Studying the Complex Magnetic Field of L43
  • 2023
  • Ingår i: Astrophysical Journal. - 1538-4357 .- 0004-637X. ; 952:1
  • Tidskriftsartikel (refereegranskat)abstract
    • We present observations of polarized dust emission at 850 mu m from the L43 molecular cloud, which sits in the Ophiuchus cloud complex. The data were taken using SCUBA-2/POL-2 on the James Clerk Maxwell Telescope as a part of the BISTRO large program. L43 is a dense (N-H2 similar to 10(22) - 10(23) cm(-2)) complex molecular cloud with a submillimeter-bright starless core and two protostellar sources. There appears to be an evolutionary gradient along the isolated filament that L43 is embedded within, with the most evolved source closest to the Sco OB2 association. One of the protostars drives a CO outflow that has created a cavity to the southeast. We see a magnetic field that appears to be aligned with the cavity walls of the outflow, suggesting interaction with the outflow. We also find a magnetic field strength of up to similar to 160 +/- 30 mu G in the main starless core and up to similar to 90 +/- 40 mu G in the more diffuse, extended region. These field strengths give magnetically super- and subcritical values, respectively, and both are found to be roughly trans-Alfvenic. We also present a new method of data reduction for these denser but fainter objects like starless cores.
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20.
  • Kristan, Matej, et al. (författare)
  • The first visual object tracking segmentation VOTS2023 challenge results
  • 2023
  • Ingår i: 2023 IEEE/CVF International conference on computer vision workshops (ICCVW). - : Institute of Electrical and Electronics Engineers Inc.. - 9798350307443 - 9798350307450 ; , s. 1788-1810
  • Konferensbidrag (refereegranskat)abstract
    • The Visual Object Tracking Segmentation VOTS2023 challenge is the eleventh annual tracker benchmarking activity of the VOT initiative. This challenge is the first to merge short-term and long-term as well as single-target and multiple-target tracking with segmentation masks as the only target location specification. A new dataset was created; the ground truth has been withheld to prevent overfitting. New performance measures and evaluation protocols have been created along with a new toolkit and an evaluation server. Results of the presented 47 trackers indicate that modern tracking frameworks are well-suited to deal with convergence of short-term and long-term tracking and that multiple and single target tracking can be considered a single problem. A leaderboard, with participating trackers details, the source code, the datasets, and the evaluation kit are publicly available at the challenge website1
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21.
  • Kristan, Matej, et al. (författare)
  • The Ninth Visual Object Tracking VOT2021 Challenge Results
  • 2021
  • Ingår i: 2021 IEEE/CVF INTERNATIONAL CONFERENCE ON COMPUTER VISION WORKSHOPS (ICCVW 2021). - : IEEE COMPUTER SOC. - 9781665401913 ; , s. 2711-2738
  • Konferensbidrag (refereegranskat)abstract
    • The Visual Object Tracking challenge VOT2021 is the ninth annual tracker benchmarking activity organized by the VOT initiative. Results of 71 trackers are presented; many are state-of-the-art trackers published at major computer vision conferences or in journals in recent years. The VOT2021 challenge was composed of four sub-challenges focusing on different tracking domains: (i) VOT-ST2021 challenge focused on short-term tracking in RGB, (ii) VOT-RT2021 challenge focused on "real-time" short-term tracking in RGB, (iii) VOT-LT2021 focused on long-term tracking, namely coping with target disappearance and reappearance and (iv) VOT-RGBD2021 challenge focused on long-term tracking in RGB and depth imagery. The VOT-ST2021 dataset was refreshed, while VOT-RGBD2021 introduces a training dataset and sequestered dataset for winner identification. The source code for most of the trackers, the datasets, the evaluation kit and the results along with the source code for most trackers are publicly available at the challenge website(1).
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22.
  • Kwon, Woojin, et al. (författare)
  • B-fields in Star-forming Region Observations (BISTRO): Magnetic Fields in the Filamentary Structures of Serpens Main
  • 2022
  • Ingår i: Astrophysical Journal. - : American Astronomical Society. - 1538-4357 .- 0004-637X. ; 926:2
  • Tidskriftsartikel (refereegranskat)abstract
    • We present 850 mu m polarimetric observations toward the Serpens Main molecular cloud obtained using the POL-2 polarimeter on the James Clerk Maxwell Telescope as part of the B-fields In STar-forming Region Observations survey. These observations probe the magnetic field morphology of the Serpens Main molecular cloud on about 6000 au scales, which consists of cores and six filaments with different physical properties such as density and star formation activity. Using the histogram of relative orientation (HRO) technique, we find that magnetic fields are parallel to filaments in less-dense filamentary structures where NH2 < 0.93 x 10(22) cm(-2) (magnetic fields perpendicular to density gradients), while they are perpendicular to filaments (magnetic fields parallel to density gradients) in dense filamentary structures with star formation activity. Moreover, applying the HRO technique to denser core regions, we find that magnetic field orientations change to become perpendicular to density gradients again at NH2 approximate to 4.6 x 10(22) NH2 approximate to 16 x 10(22) cm(-2), magnetic fields change back to being parallel to density gradients once again, which can be understood to be due to magnetic fields being dragged in by infalling material. In addition, we estimate the magnetic field strengths of the filaments (B-POS = 60-300 mu G)) using the Davis-Chandrasekhar-Fermi method and discuss whether the filaments are gravitationally unstable based on magnetic field and turbulence energy densities.
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23.
  • Li, Fei, et al. (författare)
  • Understanding Service Integration of Online Social Networks : A Data-Driven Study
  • 2018
  • Ingår i: 2018 IEEE International Conference on Pervasive Computing and Communications Workshops, PerCom Workshops 2018. - 9781538632277 ; , s. 848-853
  • Konferensbidrag (refereegranskat)abstract
    • The cross-site linking function is widely adopted by online social networks (OSNs). This function allows a user to link her account on one OSN to her accounts on other OSNs. Thus, users are able to sign in with the linked accounts, share contents among these accounts and import friends from them. It leads to the service integration of different OSNs. This integration not only provides convenience for users to manage accounts of different OSNs, but also introduces usefulness to OSNs that adopt the cross-site linking function. In this paper, we investigate this usefulness based on users' data collected from a popular OSN called Medium. We conduct a thorough analysis on its social graph, and find that the service integration brought by the crosssite linking function is able to change Medium's social graph structure and attract a large number of new users. However, almost none of the new users would become high PageRank users (PageRank is used to measure a user's influence in an OSN). To solve this problem, we build a machine-learning-based model to predict high PageRank users in Medium based on their Twitter data only. This model achieves a high F1-score of 0.942 and a high area under the curve (AUC) of 0.986. Based on it, we design a system to assist new OSNs to identify and attract high PageRank users from other well-established OSNs through the cross-site linking function.
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24.
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25.
  • Liao, Xunfan, et al. (författare)
  • The role of dipole moment in two fused-ring electron acceptor and one polymer donor based ternary organic solar cells
  • 2020
  • Ingår i: Materials Chemistry Frontiers. - : Royal Society of Chemistry. - 2052-1537. ; 4:5, s. 1507-1518
  • Tidskriftsartikel (refereegranskat)abstract
    • Fused-ring electron acceptor (FREA) based ternary organic solar cells (OSCs) have made significant progress and attracted considerable attention due to their simple device architecture and broad absorption range in devices. There are three key parameters that need to be fine-tuned in ternary OSCs including absorption, energy level and morphology in order to realize high efficiencies. Herein, a series of FREAs with diverse electron-rich cores or electron-deficient terminals are developed and rationally combined to achieve high performance ternary OSCs. The dipole moment of FREAs' terminals has been unveiled as an important factor and its working mechanism has been thoroughly investigated by systematically studying six ternary OSCs. These ternary blends all exhibit complementary absorption and cascade energy levels, which can facilitate efficient light-harvesting and charge transfer. Additionally, the morphological effects on ternary OSCs are eliminated through comparative studies while demonstrating distinctively different performance. The preliminary results show that compatible dipole moment between two FREAs is critical in ternary blends. Specifically, the performance of the ternary system with two FREAs having quite different dipole moment terminals is worse compared to that with similar terminal dipole moments. The pair with larger difference in the dipole moment will also negatively impact device performance. This interesting phenomenon is likely due to the fact that very different dipole moments of terminals in FREAs can significantly decrease the electron mobility as well as induce unbalanced hole/electron transport. Consequently, it results in increased charge recombination and reduced charge collection efficiency. This finding demonstrates that the dipole moment of FREAs should be taken into account in designing ternary OSCs.
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