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Sökning: WFRF:(Guénot Diego)

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1.
  • Björklund Svensson, Jonas, et al. (författare)
  • Low-divergence femtosecond X-ray pulses from a passive plasma lens
  • 2021
  • Ingår i: Nature Physics. - : Springer Science and Business Media LLC. - 1745-2481 .- 1745-2473. ; 17:5, s. 639-645
  • Tidskriftsartikel (refereegranskat)abstract
    • Electron and X-ray beams originating from compact laser-wakefield accelerators have very small source sizes that are typically on the micrometre scale. Therefore, the beam divergences are relatively high, which makes it difficult to preserve their high quality during transport to applications. To improve on this, tremendous efforts have been invested in controlling the divergence of the electron beams, but no mechanism for generating collimated X-ray beams has yet been demonstrated experimentally. Here we propose and realize a scheme where electron bunches undergoing focusing in a dense, passive plasma lens can emit X-ray pulses with divergences approaching the incoherent limit. Compared with conventional betatron emission, the divergence of this so-called plasma lens radiation is reduced by more than an order of magnitude in solid angle, while maintaining a similar number of emitted photons per electron. This X-ray source offers the possibility of producing brilliant and collimated few-femtosecond X-ray pulses for ultra-fast science, in particular for studies based on X-ray diffraction and absorption spectroscopy. X-ray pulses with low divergences are produced in a laser-wakefield accelerator by focusing electron bunches in a dense passive plasma lens.
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2.
  • Dahlström, J. Marcus, 1982-, et al. (författare)
  • Theory of attosecond delays in laser-assisted photoionization
  • 2013
  • Ingår i: Chemical Physics. - : Elsevier BV. - 0301-0104 .- 1873-4421. ; 414, s. 53-64
  • Tidskriftsartikel (refereegranskat)abstract
    • We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition amplitudes and to make the connection with the time-delays that have been recently measured in experiments. We find that the overall phase contains two distinct types of contributions: one is expressed in terms of the phase-shifts of the photoelectron continuum wavefunction while the other is linked to continuum–continuum transitions induced by the infrared (IR) laser probe. Our formalism applies to both kinds of measurements reported so far, namely the ones using attosecond pulse trains of XUV harmonics and the others based on the use of isolated attosecond pulses (streaking). The connection between the phases and the time-delays is established with the help of finite difference approximations to the energy derivatives of the phases. The observed time-delay is a sum of two components: a one-photon Wigner-like delay and an universal delay that originates from the probing process itself.
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3.
  • Diego, Guénot, et al. (författare)
  • Simultaneous X-ray absorption and two-photon LIF for imaging the spray formation region
  • 2019
  • Ingår i: ILASS–Europe 2019, Proceedings of the 29th Conference on Liquid Atomization and Spray Systems, 2-4 September 2019, Paris, France.
  • Konferensbidrag (refereegranskat)abstract
    • Imaging the spray formation region of atomizing sprays is particularly challenging due to the presence of a variety of irregular liquid structures such as ligaments, liquid blobs, droplets, liquid sheets and a possible liquid core. The number and concentration of those liquid bodies dictate the presence of liquid/air interfaces, which are responsible to undesired scattering effects. The resulting images are blurred, ultimately concealing the real structure of the spray formation region. Due to both, scattering effects and the presence of highly irregular 3D liquid structures, the only reliable measurement of liquid mass in the spray formation region is obtained using X-ray radiography. The generation of collimated X-rays pulsed has been done, in the past, by means of a synchrotron, thus limiting the number of studies that can be performed.In parallel to the use of X-rays, progresses in advanced laser imaging techniques for suppressing multiple scattering issues have been particularly important over the past decade. A very recent solution consists in using 2-photon excitation LIF laser sheet imaging.In this paper, we report for the first time the possibility of simultaneously imaging an atomizing spray using X-ray absorption and 2-photon LIF planar imaging, where the simultaneous single-shot recordings are made over a ~20mmx20mm viewed area. The spray is generated from a commercial fuel port injection system from which, water was injected. The unique illumination/detection scheme proposed here was made possible thanks to the use of X-rays emitted from a laser plasma accelerator (Betatron radiation). For this experiment, we use the High Intensity Laser system at Lund University that provides on target 800mJ, 38fs laser pulses. The emitted X-ray radiation is ranging from 1 to 10keV and peaking at ~2keV. It propagates outside of the vacuum chamber where an X-ray camera records the shadow of the liquid jet. In addition to that, a fraction of the laser pulse ~10mJ is directed on the liquid jet and focuses with a cylindrical lens where it induces fluorescence from a 2-photon excitation process in a dye -here, fluorescein- added to the liquid. The 2p-LIF images provide details on the size and shape of the liquid structures, optically sectioned by the light sheet, while the integrated liquid mass is extracted from the X-ray radiography. This is making the two imaging techniques highly complementary for the characterization of spray systems as well as for further understanding the physics related to liquid atomization.
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4.
  • Gisselbrecht, Mathieu, et al. (författare)
  • Exploring single-photon ionization on the attosecond time scale
  • 2012
  • Ingår i: XXVII International Conference on Photonic, Electronic and Atomic Collisions (Icpeac 2011), Pts 1-15. - : IOP Publishing. - 1742-6588 .- 1742-6596. ; 388, s. 032025-032025
  • Konferensbidrag (refereegranskat)abstract
    • One of the fundamental processes in nature is the photoelectric effect in which an electron is ripped away from its atom via the interaction with a photon. This process was long believed to be instantaneous but with the development of attosecond pulses (1 as 10(-18) s) we can finally get an insight into its dynamic. Here we measure a delay in ionization time between two differently bound electrons. The outgoing electrons are created via ionization with a train of attosecond pulses and we probe their relative delay with a synchronized infrared laser. We demonstrate how this probe field influences the measured delays and show that this contribution can be estimated with a universal formula, which allows us to extract field free atomic data..
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5.
  • Guénot, Diego, et al. (författare)
  • Distribution of Liquid Mass in Transient Sprays Measured Using Laser-Plasma-Driven X-Ray Tomography
  • 2022
  • Ingår i: Physical Review Applied. - 2331-7019. ; 17:6
  • Tidskriftsartikel (refereegranskat)abstract
    • We report, the use of laser-plasma-driven x rays to reveal the three-dimensional (3D) structure of a highly atomizing water spray. Soft x rays approximately 5 keV are generated by means of a laser-plasma accelerator. Transmission radiography measurements are performed at different angles, by rotating a multihole injector. Using computer tomography, the local liquid volume distribution and its spatial variation are retrieved in 3D, showing up to 55% liquid fraction at the nozzle outlet, which decreases to below 7% within only 1 mm. The resolution of the liquid volume fraction is 0.5% while the spatial resolution of the radiographic images is 11.5μm. The x-ray source used here provides successful measurements of liquid mass distribution over a relatively large volume and is very promising for the analysis of a variety of challenging transient spray systems, e.g., the injection of liquid synthetic and biofuels used for future clean-combustion applications.
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6.
  • Guenot, Diego, et al. (författare)
  • Measurements of relative photoemission time delays in noble gas atoms
  • 2014
  • Ingår i: Journal of Physics B. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 47:24, s. 245602-
  • Tidskriftsartikel (refereegranskat)abstract
    • We determine relative photoemission time delays between valence electrons in different noble gas atoms (Ar, Ne and He) in an energy range between 31 and 37 eV. The atoms are ionized by an attosecond pulse train synchronized with an infrared laser field and the delays are measured using an interferometric technique. We compare our results with calculations using the random phase approximation with exchange and multi-configurational Hartree-Fock. We also investigate the influence of the different ionization angular channels.
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7.
  • Guenot, Diego, et al. (författare)
  • Photoemission time delay measurements and calculations close to the 3s ionization cross section minimum in ar
  • 2012
  • Ingår i: Physical Review A. Atomic, Molecular, and Optical Physics. - 1050-2947 .- 1094-1622. ; 85:5, s. 053424-
  • Tidskriftsartikel (refereegranskat)abstract
    • We present experimental measurements and theoretical calculations of photoionization time delays from the 3s and 3p shells in Ar in the photon energy range of 32-42 eV. The experimental measurements are performed by interferometry using attosecond pulse trains and the infrared laser used for their generation. The theoretical approach includes intershell correlation effects between the 3s and 3p shells within the framework of the random-phase approximation with exchange. The connection between single-photon ionization and the two-color two-photon ionization process used in the measurement is established using the recently developed asymptotic approximation for the complex transition amplitudes of laser-assisted photoionization. We compare and discuss the theoretical and experimental results, especially in the region where strong intershell correlations in the 3s -> kp channel lead to an induced Cooper minimum in the 3s ionization cross section.
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8.
  • Guenot, Diego, et al. (författare)
  • Probing electron correlation on the attosecond time scale
  • 2014
  • Ingår i: High Intensity Lasers and High Field Phenomena, HILAS 2014. - 9781557529954
  • Konferensbidrag (refereegranskat)abstract
    • We present experimental measurements and theoretical calculations of single and double ionization time delays in various noble gases using an interferometric method. The measured delays allow us to extract information on the electron correlation.
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9.
  • Guenot, Diego (författare)
  • Probing Electron Correlation on the Attosecond Timescale
  • 2014
  • Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
    • This thesis describes how photoemission stimulated by an attosecond pulse train (APT) can be used to extract information on electron correlation in simple quantum systems such as atoms. The emission of the electron by an APT induces a reorganization of the electrons remaining in the ion core. This reorganization causes a change in the trajectory of the emitted electron. An infrared (IR) field is used to probe the delay induced by the ion's potential and the electron's reorganization via an interferometric technique. This thesis focuses on how the delay can be measured in various atomic systems and on how physical information about the electron correlations may be extracted. The first chapter of the thesis presents a brief overview of the attosecond techniques which have been used. It describes how the APTs are generated via a non-linear process called High Order Harmonic Generation (HHG), and how these pulses are characterized temporally using the so-called RABITT technique (reconstruction of attosecond beating by interference in a two-photon transitions). Finally, the different parts of the experimental set-up are described: the laser system, the APT generation chamber and the different detectors. The second part focuses on a theoretical description of the photo-ionization process. The delays measured in the RABITT technique are derived and interpreted using perturbation theory. The influence of electron correlation on the delay is then investigated in the case of a Fano resonance and in double photoionization. The third chapter describes experimental results obtained in various atomic systems. A comparison is made between the photoemission delays from the outer valence shells of argon, neon, and helium; between the inner and outer valence shells of argon; between the on-resonance and off-resonance delays for argon levels interacting in a Fano resonance; and between the delay induced by single and double photoionization in xenon. The experimental results are compared with calculations using several different atomic codes.
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10.
  • Jimenez-Galan, A., et al. (författare)
  • Phase Measurement of a Fano Resonance Using Tunable Attosecond Pulses
  • 2015
  • Ingår i: Journal of Physics: Conference Series. - : IOP Publishing. - 1742-6588 .- 1742-6596. ; 635, s. 092137-092137
  • Konferensbidrag (refereegranskat)abstract
    • We study photoionization of argon atoms close to the 3s(2)3p(6) -> 3s(1)3p(6)4p Fano resonance using an attosecond pulse train and a weak infrared probe field. An interferometric technique combined with tunable attosecond pulses allows us to determine the phase of the photoionization amplitude as a function of photon energy. We interpret the experimental results using an analytical two-photon model based on the Fano formalism and obtain quantitative agreement.
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11.
  • Klünder, Kathrin, et al. (författare)
  • Probing Single-Photon Ionization on the Attosecond Time Scale
  • 2011
  • Ingår i: Physical Review Letters. - 1079-7114. ; 106:14
  • Tidskriftsartikel (refereegranskat)abstract
    • We study photoionization of argon atoms excited by attosecond pulses using an interferometric measurement technique. We measure the difference in time delays between electrons emitted from the 3s(2) and from the 3p(6) shell, at different excitation energies ranging from 32 to 42 eV. The determination of photoemission time delays requires taking into account the measurement process, involving the interaction with a probing infrared field. This contribution can be estimated using a universal formula and is found to account for a substantial fraction of the measured delay.
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12.
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13.
  • Kotur, Marija, et al. (författare)
  • Spectral phase measurement of a Fano resonance using tunable attosecond pulses
  • 2016
  • Ingår i: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723. ; 7
  • Tidskriftsartikel (refereegranskat)abstract
    • Electron dynamics induced by resonant absorption of light is of fundamental importance in nature and has been the subject of countless studies in many scientific areas. Above the ionization threshold of atomic or molecular systems, the presence of discrete states leads to autoionization, which is an interference between two quantum paths: direct ionization and excitation of the discrete state coupled to the continuum. Traditionally studied with synchrotron radiation, the probability for autoionization exhibits a universal Fano intensity profile as a function of excitation energy. However, without additional phase information, the full temporal dynamics cannot be recovered. Here we use tunable attosecond pulses combined with weak infrared radiation in an interferometric setup to measure not only the intensity but also the phase variation of the photoionization amplitude across an autoionization resonance in argon. The phase variation can be used as a fingerprint of the interactions between the discrete state and the ionization continua, indicating a new route towards monitoring electron correlations in time.
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14.
  • Kroon, David, et al. (författare)
  • Attosecond pulse walk-off in high-order harmonic generation
  • 2014
  • Ingår i: Optics Letters. - 0146-9592. ; 39:7, s. 2218-2221
  • Tidskriftsartikel (refereegranskat)abstract
    • We study the influence of the generation conditions on the group delay of attosecond pulses in high-order harmonic generation in gases. The group delay relative to the fundamental field is found to decrease with increasing gas pressure in the generation cell, reflecting a temporal walk-off due to the dispersive properties of the nonlinear medium. This effect is well reproduced using an on-axis phase-matching model of high-order harmonic generation in an absorbing gas. (C) 2014 Optical Society of America
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15.
  • Louisy, Maite, et al. (författare)
  • Gating attosecond pulses in a noncollinear geometry
  • 2015
  • Ingår i: Optica. - 2334-2536. ; 2:6, s. 563-566
  • Tidskriftsartikel (refereegranskat)abstract
    • The efficient generation of isolated attosecond pulses (IAPs), giving access to ultrafast electron dynamics in various systems, is a key challenge in attosecond science. IAPs can be produced by confining the extreme ultraviolet emission generated by an intense laser pulse to a single field half-cycle or, as shown recently, by employing angular streaking methods. Here, we experimentally demonstrate the angular streaking of attosecond pulse trains in a noncollinear geometry, leading to the emission of angularly separated IAPs. The noncollinear geometry simplifies the separation of the fundamental laser field and the generated pulses, making this scheme promising for intracavity attosecond pulse generation, thus opening new possibilities for high-repetition-rate attosecond sources. (C) 2015 Optical Society of America
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16.
  • Månsson, Erik, et al. (författare)
  • Double ionization probed on the attosecond timescale
  • 2014
  • Ingår i: Nature Physics. - 1745-2473 .- 1745-2481. ; 10:3, s. 207-211
  • Tidskriftsartikel (refereegranskat)abstract
    • Double ionization following the absorption of a single photon is one of the most fundamental processes requiring interaction between electrons(1-3). Information about this interaction is usually obtained by detecting emitted particles without access to real-time dynamics. Here, attosecond light pulses(4,5), electron wave packet interferometry(6) and coincidence techniques(7) are combined to measure electron emission times in double ionization of xenon using single ionization as a clock, providing unique insight into the two-electron ejection mechanism. Access to many-particle dynamics in real time is of fundamental importance for understanding processes induced by electron correlation in atomic, molecular and more complex systems.
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17.
  • Månsson, Erik, et al. (författare)
  • Multi-purpose two- and three-dimensional momentum imaging of charged particles for attosecond experiments at 1 kHz repetition rate.
  • 2014
  • Ingår i: Review of Scientific Instruments. - : AIP Publishing. - 1089-7623 .- 0034-6748. ; 85:12
  • Tidskriftsartikel (refereegranskat)abstract
    • We report on the versatile design and operation of a two-sided spectrometer for the imaging of charged-particle momenta in two dimensions (2D) and three dimensions (3D). The benefits of 3D detection are to discern particles of different mass and to study correlations between fragments from multi-ionization processes, while 2D detectors are more efficient for single-ionization applications. Combining these detector types in one instrument allows us to detect positive and negative particles simultaneously and to reduce acquisition times by using the 2D detector at a higher ionization rate when the third dimension is not required. The combined access to electronic and nuclear dynamics available when both sides are used together is important for studying photoreactions in samples of increasing complexity. The possibilities and limitations of 3D momentum imaging of electrons or ions in the same spectrometer geometry are investigated analytically and three different modes of operation demonstrated experimentally, with infrared or extreme ultraviolet light and an atomic/molecular beam.
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18.
  • Mårsell, Erik, et al. (författare)
  • Secondary electron imaging of nanostructures using Extreme Ultra-Violet attosecond pulse trains and Infra-Red femtosecond pulses
  • 2013
  • Ingår i: Annalen der Physik. - : Wiley. - 0003-3804. ; 525:1-2, s. 162-170
  • Tidskriftsartikel (refereegranskat)abstract
    • Surface electron dynamics unfold at time and length scales down to attoseconds and nanometres, making direct imaging with extreme spatiotemporal resolution highly desirable. However, this has turned out to be a major challenge even with the advent of reliable attosecond light sources. In this paper, photoelectrons from Ag nanowires and nanoparticles excited by extreme ultraviolet (XUV) attosecond pulse trains and infrared femtosecond pulses using a PhotoEmission Electron Microscope (PEEM) are imaged. In addition, the samples were investigated using Scanning Electron Microscopy (SEM) and synchrotron based X-ray photoelectron spectroscopy (XPS). To achieve contrast between the nanostructures and the substrate in the XUV images, three different substrate materials were investigated: Cr, ITO and Au. While plasmonic field enhancement can be observed on all three substrates, only on Au substrates do the Ag nanowires appear significantly brighter than the substrate in XUV-PEEM imaging. 3-photon photoemission imaging of plasmonic hot-spots was performed where the autocorrelation trace is observed in the interference signal between two femtosecond Infra-Red (IR) beams with sub-cycle precision. Finally, using Monte Carlo simulations, it is shown how the secondary electrons imaged in the XUV PEEM can potentially reveal information on the attosecond time scale from the near surface region of the nanostructures.
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19.
  • Permogorov, Alexander, et al. (författare)
  • Effects of pulse chirp on laser-driven proton acceleration
  • 2022
  • Ingår i: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322. ; 12
  • Tidskriftsartikel (refereegranskat)abstract
    • Optimisation and reproducibility of beams of protons accelerated from laser-solid interactions require accurate control of a wide set of variables, concerning both the laser pulse and the target. Among the former ones, the chirp and temporal shape of the pulse reaching the experimental area may vary because of spectral phase modulations acquired along the laser system and beam transport. Here, we present an experimental study where we investigate the influence of the laser pulse chirp on proton acceleration from ultrathin flat foils (10 and 100 nm thickness), while minimising any asymmetry in the pulse temporal shape. The results show a ± 10 % change in the maximum proton energy depending on the sign of the chirp. This effect is most noticeable from 10 nm-thick target foils, suggesting a chirp-dependent influence of relativistic transparency.
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20.
  • Selvander, Madeleine, et al. (författare)
  • Naevi Characterization Using Hyperspectral Imaging : A Pilot Study
  • Ingår i: Current Eye Research. - 0271-3683.
  • Tidskriftsartikel (refereegranskat)abstract
    • Purpose: The prevalence of choroidal naevi is common and has been found to be up to 10%. Little is known regarding the optical properties of choroidal naevi. A novel hyperspectral eye fundus camera was used to investigate choroidal naevi’s optical density spectra in the retina. Methods: In an ophthalmology clinic setting, patients with choroidal naevi were included in the study. Visual acuity and pressure were tested. Following mydriatics, optical coherence tomography and fundus photography were taken as a reference, after which a hyperspectral image with 12 nm spectral resolution at 450–700 nm was taken. The optical density spectra was measured across the area of the naevus. Results: Nine patients with 11 naevi were examined. The visual acuity was not affected by any of the naevi. All the naevi were flat as measured either with the optical coherence tomography and/or on inspection, and only one naevi had a risk factor (orange pigmentation). The Wasserstein distance between the background and the naevi was higher at 695 nm compared to 555 nm (p = .002). The naevi could be grouped into three clusters based on the extracted optical density spectra. Conclusion: Choroidal naevi are better visible in longer wavelengths compared to shorter wavelengths. This finding can be used to contour and follow choroidal naevi. Choroidal naevi expose different optical density spectra that can be grouped into three different clusters. One of these clusters has an optical density spectra resembling the absorption spectra of lipofuscin, which may indicate the content of this pigment.
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21.
  • Svendsen, Kristoffer, et al. (författare)
  • A focused very high energy electron beam for fractionated stereotactic radiotherapy
  • 2021
  • Ingår i: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322. ; 11:1
  • Tidskriftsartikel (refereegranskat)abstract
    • An electron beam of very high energy (50–250 MeV) can potentially produce a more favourable radiotherapy dose distribution compared to a state-of-the-art photon based radiotherapy technique. To produce an electron beam of sufficiently high energy to allow for a long penetration depth (several cm), very large accelerating structures are needed when using conventional radio-frequency technology, which may not be possible due to economical or spatial constraints. In this paper, we show transport and focusing of laser wakefield accelerated electron beams with a maximum energy of 160 MeV using electromagnetic quadrupole magnets in a point-to-point imaging configuration, yielding a spatial uncertainty of less than 0.1 mm, a total charge variation below 1 % and a focal spot of 2.3×2.6mm2. The electron beam was focused to control the depth dose distribution and to improve the dose conformality inside a phantom of cast acrylic slabs and radiochromic film. The phantom was irradiated from 36 different angles to obtain a dose distribution mimicking a stereotactic radiotherapy treatment, with a peak fractional dose of 2.72 Gy and a total maximum dose of 65 Gy. This was achieved with realistic constraints, including 23 cm of propagation through air before any dose deposition in the phantom.
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22.
  • Tomkus, Vidmantas, et al. (författare)
  • Laser wakefield accelerated electron beams and betatron radiation from multijet gas targets
  • 2020
  • Ingår i: Scientific Reports. - : Springer Science and Business Media LLC. - 2045-2322. ; 10:1
  • Tidskriftsartikel (refereegranskat)abstract
    • Laser Plasma Wakefield Accelerated (LWFA) electron beams and efficiency of betatron X-ray sources is studied using laser micromachined supersonic gas jet nozzle arrays. Separate sections of the target are used for the injection, acceleration and enhancement of electron oscillation. In this report, we present the results of LWFA and X-ray generation using dynamic gas density grid built by shock-waves of colliding jets. The experiment was done with the 40 TW, 35 fs laser at the Lund Laser Centre. Electron energies of 30–150 MeV and 1.0 × 108–5.5 × 108 photons per shot of betatron radiation have been measured. The implementation of the betatron source with separate regions of LWFA and plasma density grid raised the efficiency of X-ray generation and increased the number of photons per shot by a factor of 2–3 relative to a single-jet gas target source.
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23.
  • Ulrich, Hannah, et al. (författare)
  • Effects of liquid properties on atomization and spray characteristics studied by planar two-photon fluorescence
  • 2022
  • Ingår i: Physics of Fluids. - : AIP Publishing. - 1070-6631 .- 1089-7666. ; 34:8
  • Tidskriftsartikel (refereegranskat)abstract
    • In this work, planar two-photon laser-induced fluorescence (2p-LIF) is applied for the first time to analyze the fluid dependent spray structure and atomization behavior of water and ethanol in a quantitative way. A commercial six-hole DISI (Direct-Injection Spark-Ignition) injector was studied at different injection pressures, operated with liquids containing the LIF dye fluorescein. Specifically for DISI-injectors, the fluid-dependent atomization is very complex and not fully understood due to the cavitating, turbulent nozzle flow that dominates the spray formation. Optical access and analysis of the near-nozzle spray are often challenging due to multiple light scattering in dense regions which is reduced by 2p-LIF measurements using a femtosecond laser. This allows high-contrast spray imaging close to the nozzle, resulting in an improved identification of single liquid structures of the spray. Thus, a higher accuracy of sizing is possible. Compared to water, the ethanol spray shape shows increased cone angles in the nozzle near-field of about 6%, which cannot be explained by classical atomization theory based on aerodynamic breakup. The larger cone angle of ethanol was attributed to its larger viscosity, which could decelerate the flow at the wall of the injection hole, affecting the velocity profile of the emerging jet. The atomization shows a main jet breakup distance of 7-10 mm in which the structure sizes decreased drastically, specifically for water. For the size of the liquid structures in the near-nozzle region, which show dimensions of about 80-130 μm, ethanol exhibited about 2% smaller Feret's diameters than water for the tested time steps at 20 MPa. This effect is even more distinct for other injection pressures and positions at a further distance to the injector. For all investigated conditions and measurement positions downstream of the nozzle, ethanol showed on average about 24% smaller structures compared to the water spray. Although this trend is in accordance with the classical atomization theory based on the aerodynamic breakup mechanism, other effects, such as cavitation and nozzle-flow induced breakup, contribute to this behavior..
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